Laser & Optoelectronics Progress, Volume. 58, Issue 11, 1100001(2021)

Research Progresses, Opportunities, and Challenges of Perovskite Light-Emitting Diodes

Ruyan Kang1,2, Lili Yan1,2, Ziqi Zhang1,2, Zhiyuan Zuo1,2、*, and Zhiqiang Li1,2、**
Author Affiliations
  • 1Center for Optics Research and Engineering, Shandong University, Qingdao , Shandong 266237, China
  • 2Key Laboratory of Laser & Infrared System, Ministry of Education, Shandong University, Qingdao , Shandong 266237, China
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    Figures & Tables(10)
    PeLEDs structure and operation mechanism diagram[31]. (a) Inverted LED structure (n-i-p); (b) normal LED structure (p-i-n); (c) operation mechanism of the two structures
    Band gap width of quantum well increases with decrease of quantum well thickness[32]
    Energy-band alignment of methylammonium halide perovskites and various ETLs and HTLs[35]
    Temperature-dependent PL and FWHM of MAPbBr3 in amorphous nanoparticles and polycrystalline film[38]. (a) PL spectral intensity; (b) FWHM
    Fabrication process of devices with submicron structure in the perovskite layer [14]
    EQE and current efficiency curves of NiOx, NiOx-PSSNa, and NiOx-PSSNa-KBr PeLEDs[51]. (a) EQE; (b) current efficiency
    Temperature-dependent (BA)2CsPb2Br7 single crystal structure evolution[60]
    Schematic illustration of fabrication process for 2D tin-based perovskite thin films[88]
    Schematic diagrams of PeLEDs with dual functions of luminescence and light detection[97]
    • Table 1. Performance parameters of PeLEDs reported in recent years

      View table

      Table 1. Performance parameters of PeLEDs reported in recent years

      Type of PeLEDsPerovskite materialor concentration ratioDevice structureEL peak /nmTurn on voltage /VMaximal EQE /%Maximal luminanceLifetime (L50)@operation conditionPublication dateRef. No
      Red PeLEDsFA0.87Cs0.13PbI3 PNCsITO/ZnO-PEI/Pero/CBP/MoO3/Au6921.915.8218 cd·m-2-2019-07[86]
      FA0.33Cs0.67Pb(I0.7Br0.3)3ITO/poly-TPD/Pero/TPBi/LiF/Al694-20.9-

      14 h@2.5 mA·cm-2,

      L0=25 cd·m-2

      [13]
      PEA2SnI4ITO/PEDOT∶PSS/Pero/TPBi/LiF/Al633-0.370 cd·m-21.1 ns@18 mA·cm-22020-03[66]
      CsPbI3 QDsITO/Ag/ZnO/PEI/Pero/TCTA/MoO3/Au6862.113.714725 cd·m-2-2020-03[87]
      Near-infrared PeLEDsc(NMAI)∶ c(Fal)∶ c(PbI2)=2∶1.9∶2ITO/ZnO/PEIE/Pero/TFB/MoOx/Au7801.312.7254 cd·m-2≈30 min@100 mA·cm-22018-02[32]
      5AVA-FAPbI3ITO/ZnO-PEIE/Pero/TFB/MoOx/Au8031.2520.7390 cd·m-2≈20 h@100 mA·cm-22018-10[14]
      c(NMAI)∶ c(FAI)∶ c(PbI2)∶c(poly-HEMA)= 5∶3∶8∶4ITO/MZO-PEIE/Pero/TFB-PFO/MoOx/Au790-20.1-≈46 h@0.1 mA·cm-22018-11[15]
      FAPbl3ITO/ZnO∶PEIE/Pero/TFB/MoOx/Au8003.321.6308 cd·m-220 h@25 mA·cm-22019-03[16]
      FAPbI3ITO/ZnO/Pero/TFB/MoOx/Au8041.314.2131.2 cd·m-223.7 h@100 mA·cm-22019-18[6]
      FAPbI3ITO/ZnO/PEIE/Pero/poly-TPD/MoO3/Al7994.020.257 cd·m-220 h (L80)@57 mA·cm-22019-12[17]
      Cs0.17FA0.83PbI2.5Br0.5ITO/ZnO/PEIE/Pero/TFB/MoO3/Au8001.517.4965 cd·m-220 h@10 mA·cm-22019-11[68]
      FAPbI3 NCsITO/PEIE-ZnO/PMC/TFB/MoOx/Au8022.217.3100 h@20 mA·m-22020-02[69]
      MAPbI3 MQWITO/Au/ZnO/Pero/TFB/MoO3/Au~8001.620.2114.9 mW·cm-2-2020-05[47]
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    Ruyan Kang, Lili Yan, Ziqi Zhang, Zhiyuan Zuo, Zhiqiang Li. Research Progresses, Opportunities, and Challenges of Perovskite Light-Emitting Diodes[J]. Laser & Optoelectronics Progress, 2021, 58(11): 1100001

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    Paper Information

    Category: Reviews

    Received: Jul. 13, 2020

    Accepted: Aug. 25, 2020

    Published Online: Jun. 7, 2021

    The Author Email: Zhiyuan Zuo (zuozhiyuan@sdu.edu.cn), Zhiqiang Li (lzq@sdu.edu.cn)

    DOI:10.3788/LOP202158.1100001

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