Optical Instruments, Volume. 44, Issue 4, 57(2022)

Surface energy transfer and metal regulated spontaneous emission of single fluorescent molecules in bimetallic core-shell nanostructures

Zhao LI1, Jun ZHOU2, and Xiantong YU2、*
Author Affiliations
  • 1Shanghai Jingpu Information Technology Co., Ltd., Shanghai 200433, China
  • 2School of Optical-Electrical and Computer Engineering, University of Shanghai for Science and Technology, Shanghai 200093, China
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    Figures & Tables(9)
    Schematic model of the SET and spontaneous emission for single fluorescent molecule in Au/SiO2/Ag core-shell nanostructures
    Schematic diagram of LSPR hybridization of gold core and silver shell in Au/SiO2/Ag structure
    Normalized optical characteristic curve of ASA structure and the near-field distribution at the plasma resonance frequency
    Non-radiative decay rate as a function of molecular-gold surface distance dwhen the LSPR resonance energy is 2.2 eV
    Non-radiative decay rate as a function of molecular-gold surface distance dwhen the LSPR resonance energy is 2.9 eV
    Non-radiative decay rate as a function of molecular-gold surface distance dwhen the LSPR resonance energy is 3.6 eV
    Non-radiative decay rate changes with molecular orientation θ
    Radiative decay rate as a function of the distance d from the molecule to the gold core surface
    Fluorescence quantum efficiency as a function of the distance d
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    Zhao LI, Jun ZHOU, Xiantong YU. Surface energy transfer and metal regulated spontaneous emission of single fluorescent molecules in bimetallic core-shell nanostructures[J]. Optical Instruments, 2022, 44(4): 57

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    Paper Information

    Category: DESIGN AND RESEARCH

    Received: Dec. 24, 2021

    Accepted: --

    Published Online: Oct. 19, 2022

    The Author Email: Xiantong YU (xtyu@usst.edu.cn)

    DOI:10.3969/j.issn.1005-5630.2022.004.008

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