<trans-title xml:lang="en">Progress on Large-area Organic-inorganic Hybrid Perovskite Films and Its Photovoltaic Application</trans-title>

Hui ZHANG; Zhipeng XU; Congtan ZHU; Xueyi GUO; Ying YANG

doi:10.15541/jim20230448

Journal of Inorganic Materials, Volume. 39, Issue 5, 457(2024)

Progress on Large-area Organic-inorganic Hybrid Perovskite Films and Its Photovoltaic Application

Hui ZHANG^1,2, Zhipeng XU^1,2, Congtan ZHU^1,2, Xueyi GUO^1,2, and Ying YANG^1,2、*

Author Affiliations

¹1. School of Metallurgy and Environment, Central South University, Changsha 410083, China

²2. Hunan Key Laboratory of Nonferrous Metal Resources Recycling, Central South University, Changsha 410083, China

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Figures & Tables(6)

1. Scalable-deposition techniques of large-area PSCs

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2. Film-forming mechanism of perovskite layer

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3. Composition engineering of perovskite material ABX₃

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4. Additive engineering of perovskite precursor ink

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Table 1. Summary of large area (≥1 cm²) perovskite layer composition, deposition techniques and corresponding PSCs performance

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Table 1. Summary of large area (≥1 cm²) perovskite layer composition, deposition techniques and corresponding PSCs performance

Perovskite layer composition	Deposition technique	V_OC/V	J_SC/(mA·cm^-2)	FF/%	PCE/%	Area/cm²	Ref.
FA_0.88Cs_0.12PbI₃	One-step blade-coating	1.00	21.21	72	15.30	205	[3]
MAPbI₃	One-step blade-coating	1.08	23.17	68	17.06	1	[16]
FAPbI₃	Two-step blade-coating	6.71	3.47	71	16.54	25	[17]
FAPbI₃	Two-step blade-coating	6.65	3.72	75	18.65	25	[18]
(FACs)Pb(IBr)	Vacuum evaporation+blade-coating	1.204.72	24.425.59	8276	24.0320.02	116	[19]
FA_0.15MA_0.85PbI₃	Screen printing	1.10	23.93	69	18.12	1	[23]
MAPbI₃	Co-evaporation	6.71	3.68	73	18.13	21	[24]
FA_0.81MA_0.15PbI_2.51Br_0.45	Two-step spin-coating+VASP	1.14	23.19	76	20.38	1	[26]
FA_0.995MA_0.005Pb(I_0.995Br_0.005)₃	Vacuum evaporation+spin-coating	1.18	24.55	77	22.26	1	[30]

Table 2. Summary of large area (≥1 cm²) perovskite layer composition, factors influencing the crystallinity (solvent system and additive type) and performance of corresponding PSCs

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Table 2. Summary of large area (≥1 cm²) perovskite layer composition, factors influencing the crystallinity (solvent system and additive type) and performance of corresponding PSCs

Perovskite layer composition	Factor affecting perovskite crystallinity		V_OC/V	J_SC/(mA·cm^-2)	FF/%	PCE/%	Area/cm²	Ref.
FA_0.83Cs_0.17PbI₃	Solvent system	DMF/NMP	15.35	1.67	76	19.54	65	[45]
MA_0.6FA_0.4PbI₃		2-ME/DMSO/CBH	5.8116.07	4.251.53	7878	18.12619.15	1850	[46]
(FAPbI₃)_0.875(CsPbBr₃)_0.125		DMF/DMPU	6.69	3.70	72	17.71	10	[47]
(FAPbI₃)_0.95(CsPbBr₃)_0.05		DMF/DMPU	10.82	2.15	77	17.94	20	[48]
FA_0.83Cs_0.17PbI_2.83Br_0.17		DMF/NMP/DPSO	1.08	20.63	74	16.63	21	[49]
(FAPbI₃)_0.95(MAPbBr₃)_0.05		2-ME/DMI	15.46	1.71	76	20.15	81	[50]
(FAPbI₃)_0.95(MAPbBr₃)_0.05		2-ME/CHP	5.7911.79	4.542.14	8081	20.9920.40	1531	[51]
MAPbI₃		2-ME/DMSO	3.19	7.19	70	14.57	2	[52]
FAPbI₃		2-ME/ACN	8.36	3.06	67	17.10	13	[53]
MAPbI₃		2-ME/DMSO/ACN	18.90	1.17	76	16.90	64	[54]
FAPbI₃		DMF/DMSO/ACN	9.00	3.14	76	21.90	16	[55]
Cs_0.03(FA_0.97MA_0.03)_0.97Pb(I_0.97Br_0.03)₃		DMF/DMSO/EtOH	1.193.50	23.987.57	7472	21.0418.95	13	[57]
(FAMA)PbI₃	Type of additive	NH₄Cl^a	7.31	2.96	67	14.55	25	[60]
(FAMA)PbI₃		NpMAI^a	1.19	24.53	76	22.26	1	[61]
(FACs)PbI₃		Crown	5.6314.29	4.171.67	7158	16.6913.84	16100	[63]
MAPbI₃		Sulfolane	7.44	3.04	71	16.06	37	[64]
FAPbI₃		Hexaflorobenzene	1.21	25.2	80	25.12	1	[65]
FAPbI₃		NAMHI	6.61	3.85	79	20.10	10	[66]
MAPbI₃		BTAI	6.52	3.51	80	18.57	12	[67]
FA_0.9MA_0.03Cs_0.07Pb(I_0.92Br_0.08)₃		PMA-AA	11.54	2.37	80	21.95	14	[68]

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Hui ZHANG, Zhipeng XU, Congtan ZHU, Xueyi GUO, Ying YANG. Progress on Large-area Organic-inorganic Hybrid Perovskite Films and Its Photovoltaic Application[J]. Journal of Inorganic Materials, 2024, 39(5): 457

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Paper Information

Category:

Received: Sep. 28, 2023

Accepted: --

Published Online: Jul. 8, 2024

The Author Email: Ying YANG (muyicaoyang@csu.edu.cn)

DOI:10.15541/jim20230448

Topics

laser devices and laser physics

Lasers and Laser Optics

Laser physics

laser manufacturing

Instrumentation, Measurement and Metrology

Table 1. Summary of large area (≥1 cm2) perovskite layer composition, deposition techniques and corresponding PSCs performance

Table 1. Summary of large area (≥1 cm2) perovskite layer composition, deposition techniques and corresponding PSCs performance

Table 2. Summary of large area (≥1 cm2) perovskite layer composition, factors influencing the crystallinity (solvent system and additive type) and performance of corresponding PSCs

Table 2. Summary of large area (≥1 cm2) perovskite layer composition, factors influencing the crystallinity (solvent system and additive type) and performance of corresponding PSCs

Table 1. Summary of large area (≥1 cm²) perovskite layer composition, deposition techniques and corresponding PSCs performance

Table 1. Summary of large area (≥1 cm²) perovskite layer composition, deposition techniques and corresponding PSCs performance

Table 2. Summary of large area (≥1 cm²) perovskite layer composition, factors influencing the crystallinity (solvent system and additive type) and performance of corresponding PSCs

Table 2. Summary of large area (≥1 cm²) perovskite layer composition, factors influencing the crystallinity (solvent system and additive type) and performance of corresponding PSCs