Photonics Research, Volume. 5, Issue 5, 473(2017)

Tunable luminescent CsPb2Br5 nanoplatelets: applications in light-emitting diodes and photodetectors

Ceng Han1, Cunlong Li1, Zhigang Zang1、*, Ming Wang1, Kuan Sun2, Xiaosheng Tang1, and Jihe Du1
Author Affiliations
  • 1Key Laboratory of Optoelectronic Technology & Systems (Ministry of Education), Chongqing University, Chongqing 400044, China
  • 2Key Laboratory of Low-Grade Energy Utilization Technologies and Systems (Ministry of Education), Chongqing University, Chongqing 400044, China
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    Figures & Tables(9)
    Study of the influence of reaction temperature on CsPb2Br5 NPLs. (a)–(c) SEM images, (d)–(f) AFM topography images, and (g)–(i) line profiles of layers.
    Morphology and EDS of an individual CsPb2Br5 NPL synthesized at 140°C. (a) TEM image and (b) HRTEM image. (c)–(f) Element mapping and (g) EDS spectrum.
    (a) XRD pattern. (b) Crystal structures of CsPb2Br5 and CsPbBr3. (c) PL and UV–vis absorption spectra. (d) PL decay traces of CsPb2Br5 NPLs.
    (a) Schematic of LEDs coated with CsPb2Br5 NPLs. (b) Emission spectra and (c) chromaticity coordinate variations of LEDs coated with different amount of CsPb2Br5 NPLs. (d) Emission spectra and (e) chromaticity coordinates of coated LEDs under different driving currents. The inset shows photographs of coated LEDs without and with injection current.
    (a) I–V curve of bare LEDs and coated LEDs. (b) Variation of FWHM and emission peak of coated LEDs under different injection currents. Luminous flux and luminous efficiency of (c) bare LEDs and (d) coated LEDs.
    (a) Schematic diagram of the fabricated photodetector device. (b) SEM image and (c) magnified SEM image of the device. (d) Band profile of the CsPb2Br5 NPL photodetector. (e)–(g) Current–voltage (I–V) characteristics of CsPb2Br5 NPL photodetectors without and with incident light of 405 nm by changing the bias voltage from −10 to 10 V.
    (a), (c), and (e) Current–time (I–T) curves of the photodetectors. (b), (d), and (f) Rise times and the decay times of the photodetectors with incident light of 405 nm at the bias of 6 V.
    • Table 1. Lifetimes and PLQYs of CsPb2Br5 NPLs Synthesized at Different Temperatures

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      Table 1. Lifetimes and PLQYs of CsPb2Br5 NPLs Synthesized at Different Temperatures

      Temp (°C)τ1 (ns)τ2 (ns)τave (ns)PLQY (%)
      1005.29.25.911
      1204.816.36.524
      1404.232.99.763
    • Table 2. Performances of CsPb2Br5 NPL Photodetectors

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      Table 2. Performances of CsPb2Br5 NPL Photodetectors

      Temp (°C)Rise Time(s)Decay Time(s)The Ratio of Current with and without Irradiation (%)Responsivity (μA/W)
      1000.4260.422364340
      1200.8520.62817974
      1400.8520.63959146
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    Ceng Han, Cunlong Li, Zhigang Zang, Ming Wang, Kuan Sun, Xiaosheng Tang, Jihe Du, "Tunable luminescent CsPb2Br5 nanoplatelets: applications in light-emitting diodes and photodetectors," Photonics Res. 5, 473 (2017)

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    Paper Information

    Category: Materials

    Received: Jul. 11, 2017

    Accepted: Aug. 14, 2017

    Published Online: Sep. 20, 2017

    The Author Email: Zhigang Zang (zangzg@cqu.edu.cn)

    DOI:10.1364/PRJ.5.000473

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