Journal of the Chinese Ceramic Society, Volume. 53, Issue 8, 2320(2025)
Effect of Side Chain Ionizability on Sulfate Tolerance of Polycarboxylate Superplasticizer
[1] [1] MEZHOV A, BEN SHIR I, SCHMIDT A, et al. Retardation mechanism of cement hydration by a comb polyphosphate superplasticizer[J]. Constr Build Mater, 2022, 352: 128698.
[2] [2] KAPELUSZNA E, KOTWICA . The effect of various grinding aids on the properties of cement and its compatibility with acrylate-based superplasticizer[J]. Materials, 2022, 15(2): 614.
[3] [3] FLATT R J, HOUST Y F. A simplified view on chemical effects perturbing the action of superplasticizers[J]. Cem Concr Res, 2001, 31(8): 1169-1176.
[4] [4] AGARWAL S K, MASOOD I, MALHOTRA S K. Compatibility of superplasticizers with different cements[J]. Constr Build Mater, 2000, 14(5): 253-259.
[5] [5] HARUNA S, FALL M. Time- and temperature-dependent rheological properties of cemented paste backfill that contains superplasticizer[J]. Powder Technol, 2020, 360: 731-740.
[6] [6] HANEHARA S, YAMADA K. Interaction between cement and chemical admixture from the point of cement hydration, absorption behaviour of admixture, and paste rheology[J]. Cem Concr Res, 1999, 29(8): 1159-1165.
[7] [7] HE Y, ZHANG X, SHUI L L, et al. Effects of PCEs with various carboxylic densities and functional groups on the fluidity and hydration performances of cement paste[J]. Constr Build Mater, 2019, 202: 656-668.
[8] [8] ALONSO M M, PALACIOS M, PUERTAS F. Compatibility between polycarboxylate-based admixtures and blended-cement pastes[J]. Cem Concr Compos, 2013, 35(1): 151-162.
[9] [9] YAMADA K, HANEHARA S. Interaction mechanism of cement and superplasticizers - the roles of polymer adsorption and ionic conditions of aqueous phase[J]. Concr Sci Eng, 2001, 3: 135-145.
[10] [10] ANDERSEN P J, KUMAR A, ROY D M, et al. The effect of calcium sulphate concentration on the adsorption of a superplasticizer on a cement: Methods, zeta potential and adsorption studies[J]. Cem Concr Res, 1986, 16(2): 255-259.
[11] [11] HAN S, PLANK J. Mechanistic study on the effect of sulfate ions on polycarboxylate superplasticisers in cement[J]. Adv Cem Res, 2013, 25(4): 200-207.
[12] [12] YAMADA K, OGAWA S, HANEHARA S. Controlling of the adsorption and dispersing force of polycarboxylate-type superplasticizer by sulfate ion concentration in aqueous phase[J]. Cem Concr Res, 2001, 31(3): 375-383.
[13] [13] FAN W, STOFFELBACH F, RIEGER J, et al. A new class of organosilane-modified polycarboxylate superplasticizers with low sulfate sensitivity[J]. Cem Concr Res, 2012, 42(1): 166-172.
[14] [14] HE Y, ZHANG X, HOOTON R D. Effects of organosilane-modified polycarboxylate superplasticizer on the fluidity and hydration properties of cement paste[J]. Constr Build Mater, 2017, 132: 112-123.
[15] [15] DALAS F, NONAT A, POURCHET S, et al. Tailoring the anionic function and the side chains of comb-like superplasticizers to improve their adsorption[J]. Cem Concr Res, 2015, 67: 21-30.
[16] [16] MARCHON D, SULSER U, EBERHARDT A, et al. Molecular design of comb-shaped polycarboxylate dispersants for environmentally friendly concrete[J]. Soft Matter, 2013, 9(45): 10719-10728.
[17] [17] FLATT R J, ZIMMERMANN J, HAMPEL C, et al. The role of adsorption energy in the sulfate-polycarboxylate competition[C]// SP-262: Ninth ACI International Conference on Superplasticizers and Other Chemical Admixtures. American Concrete Institute, 2009: 153-164.
[18] [18] BOUKENDAKDJI O, KADRI E H, KENAI S. Effects of granulated blast furnace slag and superplasticizer type on the fresh properties and compressive strength of self-compacting concrete[J]. Cem Concr Compos, 2012, 34(4): 583-590.
[19] [19] GUO Y D, HAN K D, GUO T F, et al. Synthesis and effect of polycarboxylate superplasticizer-contained silica-matrix-microcapsules on the flow behavior of cement paste[J]. Constr Build Mater, 2024, 443: 137697.
[20] [20] MADSEN F, PEPPAS N A. Complexation graft copolymer networks: Swelling properties, calcium binding and proteolytic enzyme inhibition[J]. Biomaterials, 1999, 20(18): 1701-1708.
[21] [21] RAVIV U, GIASSON S, KAMPF N, et al. Lubrication by charged polymers[J]. Nature, 2003, 425(6954): 163-165.
[22] [22] KOBAYASHI M, TAKAHARA A. Tribological properties of hydrophilic polymer brushes under wet conditions[J]. Chem Rec, 2010, 10(4): 208-216.
[23] [23] KOBAYASHI M, ISHIHARA K, TAKAHARA A. Neutron reflectivity study of the swollen structure of polyzwitterion and polyeletrolyte brushes in aqueous solution[J]. J Biomater Sci Polym Ed, 2014, 25(14-15): 1673-1686.
[24] [24] COLLEPARDI M. Admixtures used to enhance placing characteristics of concrete[J]. Cem Concr Compos, 1998, 20(2-3): 103-112.
[25] [25] LI C Z, FENG N Q, LI Y D, et al. Effects of polyethlene oxide chains on the performance of polycarboxylate-type water-reducers[J]. Cem Concr Res, 2005, 35(5): 867-873.
[26] [26] NAWA T. Effect of chemical structure on steric stabilization of polycarboxylate-based superplasticizer[J]. J Adv Concr Technol, 2006, 4(2): 225-232.
[27] [27] KJELDSEN A M, FLATT R J, BERGSTRM L. Relating the molecular structure of comb-type superplasticizers to the compression rheology of MgO suspensions[J]. Cem Concr Res, 2006, 36(7): 1231-1239.
[28] [28] GUAN J N, LIU X, LIU S J, et al. Comb polymer with ionic side chains as a novel dispersant for cement slurries: Synthesis, characterization and working mechanism[J]. Adv Powder Technol, 2024, 35(2): 104323.
[29] [29] GUAN J N, LIU S J, LIU X, et al. Effect of side chain ionizability on the adsorption behavior of polycarboxylate superplasticizer[J]. Colloids Surf A Physicochem Eng Aspects, 2025, 708: 136058.
[30] [30] FENEUIL B, PITOIS O, ROUSSEL N. Effect of surfactants on the yield stress of cement paste[J]. Cem Concr Res, 2017, 100: 32-39.
[32] [32] LEWIS J A, MATSUYAMA H, KIRBY G, et al. Polyelectrolyte effects on the rheological properties of concentrated cement suspensions[J]. J Am Ceram Soc, 2006, 83: 1905-1913.
[33] [33] BAYLY C I, CIEPLAK P, CORNELL W, et al. A well-behaved electrostatic potential based method using charge restraints for deriving atomic charges: The RESP model[J]. J Phys Chem, 1993, 97(40): 10269-10280.
[34] [34] JORGENSEN W L, MAXWELL D S, TIRADO-RIVES J. Development and testing of the OPLS all-atom force field on conformational energetics and properties of organic liquids[J]. J Am Chem Soc, 1996, 118(45): 11225-11236.
[35] [35] HESS B, KUTZNER C, VAN DER SPOEL D, et al. GROMACS 4: Algorithms for highly efficient, load-balanced, and scalable molecular simulation[J]. J Chem Theory Comput, 2008, 4(3): 435-447.
[36] [36] BERENDSEN H J C, POSTMA J P M, VAN GUNSTEREN W F, et al. Molecular dynamics with coupling to an external bath[J]. J Chem Phys 1984, 81(8): 3684-3690.
[37] [37] ESSMANM U, PERERA L, BERKOWITZ M L, et al. A smooth particle mesh Ewald method [J]. J Chem Phys, 1995, 103 (19): 8577-8593.
[38] [38] ASTRAKAS L G, GOUSIAS C, TZAPHLIDOU M. Structural destabilization of chignolin under the influence of oscillating electric fields[J]. J Appl Phys 2012, 111(7): 074702.
[39] [39] HESS B, BEKKER H, BERENDSEN H J C, et al. LINCS: A linear constraint solver for molecular simulations[J]. J Comput Chem, 18(12): 1463-1472.
[40] [40] VAN GUNSTEREN W F, BERENDSEN H J C. A leap-frog algorithm for stochastic dynamics[J]. Mol Simul, 1988, 1(3): 173-185.
[41] [41] SHU X, RAN Q P, LIU J P, et al. Tailoring the solution conformation of polycarboxylate superplasticizer toward the improvement of dispersing performance in cement paste[J]. Constr Build Mater, 2016, 116: 289-298.
[42] [42] YAO G, ZHAO J, RAMISETTI S, et al. Atomistic molecular dynamic simulation of dilute poly(acrylic acid) solution: Effects of simulation size sensitivity and ionic strength[J]. Ind Eng Chem Res, 2018, 57(50): 17129-17141.
Get Citation
Copy Citation Text
GUAN Jianan, CHENG Bo, LIU Xiao, ZHU Haitang, QIAN Shanshan, SHI Jianjun. Effect of Side Chain Ionizability on Sulfate Tolerance of Polycarboxylate Superplasticizer[J]. Journal of the Chinese Ceramic Society, 2025, 53(8): 2320
Category:
Received: Jan. 6, 2025
Accepted: Sep. 5, 2025
Published Online: Sep. 5, 2025
The Author Email: LIU Xiao (liux@bjut.edu.cn)