Journal of Bioresources and Bioproducts, Volume. 10, Issue 2, 209(2025)
Robust MXene aerogel assisted by cellulose nanofiber for efficient crude oil spill remediation
[1] [1] Cai, C.Y., Wei, Z.C., Huang, Y.Z., Fu, Y., 2021. Wood-inspired superelastic MXene aerogels with superior photothermal conversion and durable superhydrophobicity for clean-up of super-viscous crude oil. Chem. Eng. J. 421, 127772.
[2] [2] Cao, W.T., Feng, W., Jiang, Y.Y., Ma, C., Zhou, Z.F., Ma, M.G., Chen, Y., Chen, F., 2019. Two-dimensional MXene-reinforced robust surface superhydrophobicity with self-cleaning and photothermal-actuating binary effects. Mater. Horiz. 6, 1057-1065.
[3] [3] Chaudhuri, K., Alhabeb, M., Wang, Z.X., Shalaev, V.M., Gogotsi, Y., Boltasseva, A., 2018. Highly broadband absorber using plasmonic titanium carbide (MXene). ACS Photonics 5, 1115-1122.
[4] [4] Cheng, Q.F., Huang, C.J., Tomsia, A.P., 2017. Freeze casting for assembling bioinspired structural materials. Adv. Mater. 29, 1703155.
[5] [5] Ding, M.C., Lu, H., Sun, Y.B., He, Y.J., Yu, J.H., Kong, H.J., Shao, C.X., Liu, C.Y., Li, C.W., 2022. Superelastic 3D assembled clay/graphene aerogels for continuous solar desalination and oil/organic solvent absorption. Adv. Sci. 9, e2205202.
[6] [6] Fan, X.Q., Liu, L., Jin, X., Wang, W.T., Zhang, S.F., Tang, B.T., 2019. MXene Ti3C2Tx for phase change composite with superior photothermal storage capability. J. Mater. Chem. A 7, 14319-14327.
[7] [7] Ge, J., Shi, L., Wang, Y.C., Zhao, H.Y., Yao, H.B., Zhu, Y.B., Zhang, Y., Zhu, H.W., Wu, H.G., Yu, S.H., 2017. Joule-heated graphene-wrapped sponge enables fast clean-up of viscous crude-oil spill. Nat. Nanotechnol. 12, 434-440.
[8] [8] Gong, X.Y., Wang, Y.X., Zeng, H.B., Betti, M., Chen, L.Y., 2019. Highly porous, hydrophobic, and compressible cellulose nanocrystals/poly(vinyl alcohol) aerogels as recyclable absorbents for oil-water separation. ACS Sustain. Chem. Eng. 7, 11118-11128.
[9] [9] Guan, Y.H., Wang, Z.N., Bao, M.T., Chen, X.P., Dong, L.M., Shen, Y., Li, Y.M., 2023. Multi-energies assisted and all-weather recovery of crude oil by superhydrophobic melamine sponge. J. Hazard. Mater. 443, 130131.
[10] [10] Ji, C., Wang, Y., Ye, Z.Q., Tan, L.Y., Mao, D.S., Zhao, W.G., Zeng, X.L., Yan, C.Z., Sun, R., Kang, D.J., Xu, J.B., Wong, C.P., 2020. Ice-templated MXene/Ag-epoxy nanocomposites as high-performance thermal management materials. ACS Appl. Mater. Interfaces 12, 24298-24307.
[11] [11] Kang, Y.L., Zhang, J., Wu, G., Zhang, M.X., Chen, S.C., Wang, Y.Z., 2018. Full-biobased nanofiber membranes toward decontamination of wastewater containing multiple pollutants. ACS Sustain. Chem. Eng. 6, 11783-11792.
[12] [12] Li, H., Du, Z.Q., 2019. Preparation of a highly sensitive and stretchable strain sensor of MXene/silver nanocomposite-based yarn and wearable applications. ACS Appl. Mater. Interfaces 11, 45930-45938.
[13] [13] Li, R.Y., Zhang, L.B., Shi, L., Wang, P., 2017. MXene Ti3C2: An effective 2D light-to-heat conversion material. ACS Nano. 11, 3752-3759.
[14] [14] Li, K.R., Chang, T.H., Li, Z.P., Yang, H.T., Fu, F.F., Li, T.T., Ho, J.S., Chen, P.Y., 2019. Biomimetic MXene textures with enhanced light-to-heat conversion for solar steam generation and wearable thermal management. Adv. Energy Mater. 9, 1901687.
[15] [15] Li, S.S., Gu, B., Li, X.Y., Tang, S.W., Zheng, L., Ruiz-Hitzky, E., Sun, Z.Y., Xu, C.L., Wang, X.Y., 2022. MXene-enhanced chitin composite sponges with antibacterial and hemostatic activity for wound healing. Adv. Healthc. Mater. 11, 2102367.
[16] [16] Ma, X.Z., Zhang, C., Gnanasekar, P., Xiao, P., Luo, Q., Li, S.Q., Qin, D.D., Chen, T., Chen, J., Zhu, J., Yan, N., 2021. Mechanically robust, solar-driven, and degradable lignin-based polyurethane adsorbent for efficient crude oil spill remediation. Chem. Eng. J. 415, 128956.
[17] [17] Navarathna, C.M., Dewage, N.B., Keeton, C., Pennisson, J., Henderson, R., Lashley, B., Zhang, X.F., Hassan, E.B., Perez, F., Mohan, D., Pittman, C.U., Mlsna, T., 2020. Biochar adsorbents with enhanced hydrophobicity for oil spill removal. ACS Appl. Mater. Interfaces 12, 9248-9260.
[18] [18] Qin, L.Y., Yang, D.Z., Zhang, M., Zhao, T.Y., Luo, Z., Yu, Z.Z., 2021. Superelastic and ultralight electrospun carbon nanofiber/MXene hybrid aerogels with anisotropic microchannels for pressure sensing and energy storage. J. Colloid Interface Sci. 589, 264-274.
[19] [19] Song, X., Huang, X.W., Luo, J.C., Long, B., Zhang, W.M., Wang, L., Gao, J.F., Xue, H.G., 2021. Flexible, superhydrophobic and multifunctional carbon nanofiber hybrid membranes for high performance light driven actuators. Nanoscale 13, 12017-12027.
[20] [20] Tang, S.W., Wu, Z.G., Feng, G.X., Wei, L.S., Weng, J.Y., Ruiz-Hitzky, E., Wang, X.Y., 2023a. Multifunctional sandwich-like composite film based on superhydrophobic MXene for self-cleaning, photodynamic and antimicrobial applications. Chem. Eng. J. 454, 140457.
[21] [21] Tang, S.W., Wu, Z.G., Li, X.Y., Xie, F.W., Ye, D.D., Ruiz-Hitzky, E., Wei, L.S., Wang, X.Y., 2023b. Nacre-inspired biodegradable nanocellulose/MXene/AgNPs films with high strength and superior gas barrier properties. Carbohydr. Polym. 299, 120204.
[22] [22] Wang, N.N., Wang, H., Wang, Y.Y., Wei, Y.H., Si, J.Y., Yuen, A.C.Y., Xie, J.S., Yu, B., Zhu, S.E., Lu, H.D., Yang, W., Chan, Q.N., Yeoh, G.H., 2019. Robust, lightweight, hydrophobic, and fire-retarded polyimide/MXene aerogels for effective oil/water separation. ACS Appl. Mater. Interfaces 11, 40512-40523.
[23] [23] Wang, P.L., Ma, C., Yuan, Q., Mai, T., Ma, M.G., 2022. Novel Ti3C2Tx MXene wrapped wood sponges for fast cleanup of crude oil spills by outstanding Joule heating and photothermal effect. J. Colloid Interface Sci. 606, 971-982.
[24] [24] Wang, X.J., Wang, C., Cheng, L., Lee, S.T., Liu, Z., 2012. Noble metal coated single-walled carbon nanotubes for applications in surface enhanced raman scattering imaging and photothermal therapy. J. Am. Chem. Soc. 134, 7414-7422.
[25] [25] Wang, Y.Q., Xie, W.H., Liu, H., Gu, H.B., 2020. Hyperelastic magnetic reduced graphene oxide three-dimensional framework with superb oil and organic solvent adsorption capability. Adv. Compos. Hybrid Mater. 3, 473-484.
[26] [26] Wang, Z.X., Han, X.S., Han, X.W., Chen, Z.B., Wang, S.J., Pu, J.W., 2021. MXene/wood-derived hierarchical cellulose scaffold composite with superior electromagnetic shielding. Carbohydr. Polym. 254, 117033.
[27] [27] Wang, T., Wang, W., Hu, C.Y., Zheng, J., Zhu, Z.J., Liu, B.J., 2024a. Design of carboxymethyl cellulose/alginate aerogels with anti-fouling and light-driven self-cleaning for enhanced oily wastewater remediation. Carbohydr. Polym. 342, 122358.
[28] [28] Wang, T., Wang, W., Wang, J.J., Hu, C.Y., Zheng, J., Zhu, Z.J., Liu, B.J., 2024b. Development of biomass aerogels with aligned channels: for continuous treatment of oily wastewater and solar-powered oil evaporation. Bioresour. Technol. 412, 131344.
[29] [29] Wang, T., Wang, W., Hu, C.Y., Zheng, J., Liu, B.J., Zhu, Z.J., 2024c. Mechanically durable, recyclable polyvinyl alcohol/lignin-based aerogel for efficient oil/water separation and solar-powered removal of high-viscosity oil. Ind. Crops Prod. 219, 119131.
[30] [30] Wei, Y.H., Li, J.J., Sun, F.R., Wu, J.R., Zhao, L.J., 2018. Leakage-proof phase change composites supported by biomass carbon aerogels from succulents. Green Chem 20, 1858-1865.
[31] [31] Wu, N., Yang, Y.F., Wang, C.X., Wu, Q.L., Pan, F., Zhang, R.N., Liu, J.R., Zeng, Z.H., 2023. Ultrathin cellulose nanofiber assisted ambient-pressure-dried, ultralight, mechanically robust, multifunctional MXene aerogels. Adv. Mater. 35, e2207969.
[32] [32] Yi, L.F., Yang, J.Y., Fang, X., Xia, Y., Zhao, L.J., Wu, H., Guo, S.Y., 2020. Facile fabrication of wood-inspired aerogel from chitosan for efficient removal of oil from water. J. Hazard. Mater. 385, 121507.
[33] [33] Yun, T., Kim, H., Iqbal, A., Cho, Y.S., Lee, G.S., Kim, M.K., Kim, S.J., Kim, D., Gogotsi, Y., Kim, S.O., Koo, C.M., 2020. Electromagnetic shielding of monolayer MXene assemblies. Adv. Mater. 32, 1906769.
[34] [34] Zhang, Y.L., Mu, Z.J., Lai, J.P., Chao, Y.G., Yang, Y., Zhou, P., Li, Y.J., Yang, W.X., Xia, Z.H., Guo, S.J., 2019. MXene/Si@SiOx@C layer-by-layer superstructure with autoadjustable function for superior stable lithium storage. ACS Nano. 13, 2167-2175.
[35] [35] Zhang, J., Huang, D., Wu, G., Chen, S.C., Wang, Y.Z., 2020a. Highly-efficient, rapid and continuous separation of surfactant-stabilized oil/Water emulsions by selective under-liquid adhering emulsified droplets. J. Hazard. Mater. 400, 123132.
[36] [36] Zhang, S.C., Liu, H., Tang, N., Zhou, S., Yu, J.Y., Ding, B., 2020b. Spider-web-inspired PM0.3 filters based on self-sustained electrostatic nanostructured networks. Adv. Mater. 32, e2002361.
[37] [37] Zhang, J.Y., Cheng, Y.H., Xu, C.J., Gao, M.Y., Zhu, M.F., Jiang, L., 2021. Hierarchical interface engineering for advanced nanocellulosic hybrid aerogels with high compressibility and multifunctionality. Adv. Funct. Mater. 31, 2009349.
[38] [38] Zhao, X., Peng, L.M., Tang, C.Y., Pu, J.H., Zha, X.J., Ke, K., Bao, R.Y., Yang, M.B., Yang, W., 2020a. All-weather-available, continuous steam generation based on the synergistic photo-thermal and electro-thermal conversion by MXene-based aerogels. Mater. Horiz. 7, 855-865.
[39] [39] Zhao, X., Wang, L.Y., Tang, C.Y., Zha, X.J., Liu, Y., Su, B.H., Ke, K., Bao, R.Y., Yang, M.B., Yang, W., 2020b. Smart Ti3C2Tx MXene fabric with fast humidity response and joule heating for healthcare and medical therapy applications. ACS Nano. 14, 8793-8805.
[40] [40] Zhou, Z.H., Song, Q.C., Huang, B.X., Feng, S.Y., Lu, C.H., 2021. Facile fabrication of densely packed Ti3C2 MXene/nanocellulose composite films for enhancing electromagnetic interference shielding and electro-/photothermal performance. ACS Nano. 15, 12405-12417.
[41] [41] Zhou, G.Q., Li, M.C., Liu, C.Z., Wu, Q.L., Mei, C.T., 2022a. 3D printed Ti3C2Tx MXene/cellulose nanofiber architectures for solid-state supercapacitors: Ink rheology, 3D printability, and electrochemical performance. Adv. Funct. Mater. 32, 2109593.
[42] [42] Zhou, J., Li, X.L., Hou, T., Zhang, X.G., Yang, B., 2022b. Biodegradable, biomimetic, and nanonet-engineered membranes enable high-flux and highly-efficient oil/water separation. J. Hazard. Mater. 434, 128858.
[43] [43] Zhu, M., Yan, X.X., Xu, H.L., Xu, Y.J., Kong, L., 2021. Highly conductive and flexible bilayered MXene/cellulose paper sheet for efficient electromagnetic interference shielding applications. Ceram. Int. 47, 17234-17244.
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Tang Shuwei, Wei Lansheng, Wu Zhengguo, Weng Jiayao, Luo Jiwen, Wang Xiaoying. Robust MXene aerogel assisted by cellulose nanofiber for efficient crude oil spill remediation[J]. Journal of Bioresources and Bioproducts, 2025, 10(2): 209
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Accepted: Aug. 26, 2025
Published Online: Aug. 26, 2025
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