Journal of Synthetic Crystals, Volume. 54, Issue 7, 1100(2025)

Review on Impact of Film Preparation Method and Crystallization Behavior on the Imaging Performance of Halide Perovskite X-Ray Detectors

Hang XIE1,2,3,4,5 and Zhiwen JIN1,2,3,4,5、*
Author Affiliations
  • 1School of Physical Science and Technology,Lanzhou University,Lanzhou 730000,China
  • 2Lanzhou Center for Theoretical Physics,Lanzhou 730000,China
  • 3Key Laboratory of Theoretical Physics of Gansu Province,Lanzhou 730000,China
  • 4Key Laboratory of Quantum Theory and Applications of MoE,Lanzhou 730000,China
  • 5Gansu Provincial Research Center for Basic Disciplines of Quantum Physics,Lanzhou 730000,China
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    X-ray detectors play a vital role in medical diagnostics, security screening, industrial nondestructive testing, and scientific research. Halide perovskites (HPs) have garnered significant attention for high-performance X-ray detection due to their large X-ray absorption coefficient, long carrier diffusion length, and superior optical properties. Notably, the flexible synthesis of HPs enables facile fabrication into polycrystalline films, wafers, and other forms. However, differences in crystallization behavior induced by fabrication methods result in varied defect distributions within the active layer, such as crystallographic orientation, grain boundaries, cracks, and pinholes, which critically impact charge carrier transport and scintillation efficiency and degrade the device performance. Therefore, elucidating crystallization mechanisms under different fabrication conditions and developing tailored control strategies are imperative. Here we systematically review the recent advances in HPs X-ray detectors: 1) wet chemical synthesis approaches and crystallization regulation strategies; 2) crystallization regulation in pressing methods, ion migration suppression, and scintillator wafer development; 3) analyzing crystallization mechanisms in vapor deposition processes, strategies for enhancing scintillator performance, and exploratory efforts toward direct X-ray detection applications. Finally, we highlight existing challenges and future prospects for advancing HPs X-ray detectors.

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    Hang XIE, Zhiwen JIN. Review on Impact of Film Preparation Method and Crystallization Behavior on the Imaging Performance of Halide Perovskite X-Ray Detectors[J]. Journal of Synthetic Crystals, 2025, 54(7): 1100

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    Paper Information

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    Received: Jan. 17, 2025

    Accepted: --

    Published Online: Aug. 28, 2025

    The Author Email: Zhiwen JIN (jinzw@lzu.edu.cn)

    DOI:10.16553/j.cnki.issn1000-985x.2025.0016

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