Acta Optica Sinica, Volume. 44, Issue 16, 1627003(2024)
Size Control of CsPbBr3 Quantum Dots by Aluminum Doping Enabling Single-Photon Emission
Fig. 1. Schematic diagram of the synthesis process for CsPbBr3 quantum dot solution
Fig. 2. XRD and XPS spectra of Al∶CsPbBr3 quantum dots and CsPbBr3 quantum dots. (a) XRD spectrum; (b) XPS diagram; (c) Cs 3d; (d) Pb 4f; (e) Br 3d; (f) Al 2p
Fig. 3. TEM images of Al∶CsPbBr3 quantum dots and CsPbBr3 quantum dots. (a) Al∶CsPbBr3 quantum dots; (b) CsPbBr3 quantum dots; (c) size distribution plot of Al∶CsPbBr3 quantum dots; (d) size distribution plot of CsPbBr3 quantum dots
Fig. 4. HRTEM image and EDS maps of Al∶CsPbBr3 quantum dots. (a) HRTEM image; (b) Al element map; (c) Pb element map; (d) Cs element map; (e) Br element map
Fig. 5. Fluorescence (PL) and absorption spectra of CsPbBr3 quantum dots and Al∶CsPbBr3 quantum dots. (a) PL spectra at different Al/Pb molar ratios; (b) absorption spectra at different Al/Pb molar ratios; (c) emission linewidth of CsPbBr3 quantum dots; (d) emission linewidth of Al∶CsPbBr3 quantum dots; (e) PL spectra of Al∶CsPbBr3 quantum dots compared to CsPbBr3 quantum dots; (f) PL evolution of CsPbBr3 quantum dots at different storage time
Fig. 6. Fluorescence intensity plots and the second-order correlation function statistical histograms of CsPbBr3 quantum dots and Al∶CsPbBr3 quantum dots. (a) Real-time fluorescence intensity plot of CsPbBr3 quantum dots; (b) single-photon statistics histogram of CsPbBr3 quantum dots under 439 nm light excitation; (c) real-time fluorescence intensity plot of Al∶CsPbBr3 quantum dots; (d) single-photon statistical histogram of Al∶CsPbBr3 quantum dots under 439 nm light excitation
Get Citation
Copy Citation Text
Lü Xin, Guohui Li, Ting Guo, Shaoding Liu, Hong Sun, Yanxia Cui, Rong Wen. Size Control of CsPbBr3 Quantum Dots by Aluminum Doping Enabling Single-Photon Emission[J]. Acta Optica Sinica, 2024, 44(16): 1627003
Category: Quantum Optics
Received: Mar. 5, 2024
Accepted: Apr. 29, 2024
Published Online: Jul. 31, 2024
The Author Email: Guohui Li (liguohui@tyut.edu.cn), Rong Wen (wenrong@tyut.edu.cn)
CSTR:32393.14.AOS240694