NUCLEAR TECHNIQUES, Volume. 46, Issue 6, 060504(2023)

Influence of wall effect on detection efficiency of β-emitters in TDCR-Čerenkov method

Zihao FAN1,2, Juncheng LIANG2, Haoran LIU2, Daqing YUAN1、*, Yang XIAO2, Changhao SUN2, Zhijie YANG2, and Meiling LIU2
Author Affiliations
  • 1China Institute of Atomic Energy, Beijing 102413, China
  • 2National Institute of Metrology, Beijing 100029, China
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    Figures & Tables(7)
    Schematic diagram of sample preparation
    TDCR counting system (a) Physical object diagram, (b) System diagram
    Deposition spectra of β emitters in hydrochloric acid (a) 700 keV, (b) 2 800 keV
    Deposition spectra of β emitters of the wall of counting vial (a) 700 keV, (b) 2 800 keV
    Čerenkov photon numbers k(E) vs. energy
    • Table 1. Comparison of results

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      Table 1. Comparison of results

      核素

      Nuclide

      比活度 Specific activity / Bq·g-1

      TDCR-切伦科夫(无壁效应)

      TDCR-Čerenkov (without wall effect)

      TDCR-切伦科夫(有壁效应)

      TDCR-Čerenkov (with wall effect)

      TDCR-LS
      90Y25.60(10)×10325.44(10)×10325.44(12)×103
      32P24.99(16)×10424.79(16)×10424.83(5)×104
      204Tl1.03(2)×1051.03(2)×1051.04(1)×105
    • Table 2. Evaluation of the combined uncertainties for method including wall effect (%)

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      Table 2. Evaluation of the combined uncertainties for method including wall effect (%)

      分量 ComponentTDCR-切伦科夫 TDCR-ČerenkovTDCR-LS
      90Y32P204Tl90Y32P204Tl
      测量变异性 Measurement variability0.100.060.650.480.100.36
      死时间 Dead-time0.030.030.010.020.020.01
      符合分辨时间 Resolving-time0.040.050.160.030.030.04
      半衰期修正 Decay correction0.050.03<0.010.050.03<0.01
      本底 Background0.060.060.060.040.040.04
      称重 Mass0.060.170.130.050.170.25
      β谱 β spectrum0.010.010.02<0.01<0.01<0.01
      各向异性系数 Anisotropy coefficient0.360.561.4
      kBkB value0.020.010.04
      合成 Combined0.390.601.60.490.210.44
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    Zihao FAN, Juncheng LIANG, Haoran LIU, Daqing YUAN, Yang XIAO, Changhao SUN, Zhijie YANG, Meiling LIU. Influence of wall effect on detection efficiency of β-emitters in TDCR-Čerenkov method[J]. NUCLEAR TECHNIQUES, 2023, 46(6): 060504

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    Paper Information

    Category: Research Articles

    Received: Dec. 29, 2022

    Accepted: --

    Published Online: Jul. 5, 2023

    The Author Email:

    DOI:10.11889/j.0253-3219.2023.hjs.46.060504

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