Photonics Research, Volume. 8, Issue 10, 1605(2020)

Room temperature synthesis of stable silica-coated CsPbBr3 quantum dots for amplified spontaneous emission

Qionghua Mo1、†, Tongchao Shi2、†, Wensi Cai1, Shuangyi Zhao1、*, Dongdong Yan1, Juan Du2,3,4, and Zhigang Zang1,5
Author Affiliations
  • 1Key Laboratory of Optoelectronic Technology & Systems (Ministry of Education), Chongqing University, Chongqing 400044, China
  • 2State Key Laboratory of High Field Laser Physics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, China
  • 3Hangzhou Institute for Advanced Study, University of Chinese Academy of Sciences, Hangzhou 310024, China
  • 4e-mail: dujuan@mail.siom.ac.cn
  • 5e-mail: zangzg@cqu.edu.cn
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    Figures & Tables(6)
    Reaction process schematics of the formation of CsPbBr3@SiO2 QDs.
    (a) XRD patterns, (b) FTIR spectra, (c) XPS full scan of CsPbBr3@SiO2 QDs and the high-resolution XPS profiles of (d) Cs 3d, (e) Pb 4f, (f) Br 3d, (g) Si 2p, and (h) O 1s.
    (a), (c) TEM images and (b), (d) HRTEM images of pure CsPbBr3 and CsPbBr3@SiO2 QDs. (e) Element distribution of CsPbBr3@SiO2 QDs.
    (a) Photographs of CsPbBr3 and CsPbBr3@SiO2 QDs solution with/without UV light and films with UV light. (b) PL intensity, (c) Absorption and PL spectra, and (d) PL decay curves of CsPbBr3 and CsPbBr3@SiO2 QDs.
    PL spectra of (a) CsPbBr3 and (b) CsPbBr3@SiO2. (c) Normalized PL intensity of CsPbBr3 and CsPbBr3@SiO2 under continuous heating at 60°C.
    (a) Pump-intensity dependence of the emission from the CsPbBr3 film under an 800 nm femtosecond laser excitation. (b) Output intensity (red) and linewidth (black) as functions of pump energy density for CsPbBr3 film under a femtosecond laser excitation of 800 nm. (c) Pump-intensity dependence of the emission from the CsPbBr3@SiO2 film under an 800 nm femtosecond laser excitation. (d) Output intensity (red) and linewidth (black) as functions of pump energy density for CsPbBr3@SiO2 film under a femtosecond laser excitation of 800 nm.
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    Qionghua Mo, Tongchao Shi, Wensi Cai, Shuangyi Zhao, Dongdong Yan, Juan Du, Zhigang Zang, "Room temperature synthesis of stable silica-coated CsPbBr3 quantum dots for amplified spontaneous emission," Photonics Res. 8, 1605 (2020)

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    Paper Information

    Category: Optical and Photonic Materials

    Received: Jun. 10, 2020

    Accepted: Aug. 3, 2020

    Published Online: Sep. 23, 2020

    The Author Email: Shuangyi Zhao (shyzhao@cqu.edu.cn)

    DOI:10.1364/PRJ.399845

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