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Acta Optica Sinica, Volume. 38, Issue 8, 0816002(2018)

Radioluminescence Properties of Sn 2+-Doped Borosilicate Glass with High Gd2O3

Xiaobo Jiang1,2、*, Ya Zou1,2, Shuai Han2,3, Congjuan Wang2, Danping Chen2、*, and Qiuhong Yang1
Author Affiliations
  • 1 School of Materials Science and Engineering, Shanghai University, Shanghai 200444, China
  • 2 Laboratory of High Power Laser Components, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, China
  • 3 University of Chinese Academy of Sciences, Beijing 100049, China
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    Absorption spectra and XPS spectra. (a) Absorption spectra of un-doped Si-B glass and Si-B glasses doped with different Sn2+ concentrations; (b) absorption spectra of Si-B glasses with different Gd2O3 concentrations; (c) XPS spectra of Sn1 prepared in CO and air atmospheres; (d) absorption spectra of Sn1 prepared in CO and air atmospheres

    Fig. 1. Absorption spectra and XPS spectra. (a) Absorption spectra of un-doped Si-B glass and Si-B glasses doped with different Sn2+ concentrations; (b) absorption spectra of Si-B glasses with different Gd2O3 concentrations; (c) XPS spectra of Sn1 prepared in CO and air atmospheres; (d) absorption spectra of Sn1 prepared in CO and air atmospheres

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    Excitation spectra and emission spectra of un-doped Si-B glass and Si-B glasses doped with different Sn2+ concentrations. (a) Excitation spectra at detection wavelength of 409 nm; (b) emission spectra at excitation wavelength of 252 nm

    Fig. 2. Excitation spectra and emission spectra of un-doped Si-B glass and Si-B glasses doped with different Sn2+ concentrations. (a) Excitation spectra at detection wavelength of 409 nm; (b) emission spectra at excitation wavelength of 252 nm

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    Excitation spectra and emission spectra of Si-B glasses with different Gd2O3 concentrations. (a) Excitation spectra at detection wavelength of 409 nm; (b) emission spectra at excitation wavelength of 275 nm

    Fig. 3. Excitation spectra and emission spectra of Si-B glasses with different Gd2O3 concentrations. (a) Excitation spectra at detection wavelength of 409 nm; (b) emission spectra at excitation wavelength of 275 nm

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    Absorption spectra and ultraviolet absorption cut-off wavelengths of glass samples doped with different Sn2+ concentrations. (a) Absorption spectra of Si-B glass; (b) absorption spectra of B-Sn glass; (c) absorption spectra of Si-Sn glass;(d) ultraviolet absorption cut-off wavelength of Si-B, B-Sn and Si-Sn glasses

    Fig. 4. Absorption spectra and ultraviolet absorption cut-off wavelengths of glass samples doped with different Sn2+ concentrations. (a) Absorption spectra of Si-B glass; (b) absorption spectra of B-Sn glass; (c) absorption spectra of Si-Sn glass;(d) ultraviolet absorption cut-off wavelength of Si-B, B-Sn and Si-Sn glasses

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    Luminescence decay curves for different samples. (a) Si-B glasses doped with different Sn2+ concentrations; (b) Si-B glasses with different Gd2O3 concentrations

    Fig. 5. Luminescence decay curves for different samples. (a) Si-B glasses doped with different Sn2+ concentrations; (b) Si-B glasses with different Gd2O3 concentrations

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    Radioluminescence spectra for different samples. (a) Un-doped Si-B glass and Si-B glasses doped with different Sn2+ concentrations; (b) Si-B glasses with different Gd2O3 concentrations

    Fig. 6. Radioluminescence spectra for different samples. (a) Un-doped Si-B glass and Si-B glasses doped with different Sn2+ concentrations; (b) Si-B glasses with different Gd2O3 concentrations

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    Energy level diagrams of Gd3+ and Sn2+

    Fig. 7. Energy level diagrams of Gd3+ and Sn2+

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    • Table 1. Compositions and density of Si-B glass

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      Table 1. Compositions and density of Si-B glass

      Sample No.Mole fraction /%Density /(g∙cm-3)
      SiO2B2O3La2O3Gd2O3SnO
      Sn0353530003.92
      Sn135353000.13.94
      Sn235353000.23.96
      Sn335353000.33.97
      Sn435353000.43.97
      Sn-Gd035353000.33.97
      Sn-Gd1353527.52.50.34.02
      Sn-Gd2353522.57.50.34.13
      Sn-Gd3353515150.34.20
      Sn-Gd435350300.34.33

    • Table 2. Compositions of B-Sn and Si-Sn glasses

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      Table 2. Compositions of B-Sn and Si-Sn glasses

      Sample No.Mole fraction /%
      B2O3Si2O3Al2O3La2O3SnO
      B-Sn170010200.1
      B-Sn270010200.2
      B-Sn370010200.3
      B-Sn470010200.4
      Si-Sn105020300.1
      Si-Sn205020300.2
      Si-Sn305020300.3
      Si-Sn405020300.4
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    Xiaobo Jiang, Ya Zou, Shuai Han, Congjuan Wang, Danping Chen, Qiuhong Yang. Radioluminescence Properties of Sn 2+-Doped Borosilicate Glass with High Gd2O3[J]. Acta Optica Sinica, 2018, 38(8): 0816002

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    Paper Information

    Category: Materials

    Received: Feb. 7, 2018

    Accepted: Apr. 9, 2018

    Published Online: May. 9, 2019

    The Author Email:

    DOI:10.3788/AOS201838.0816002

    Topics

    laser devices and laser physics
    Lasers and Laser Optics
    Laser physics
    laser manufacturing
    Instrumentation, Measurement and Metrology