Laser & Optoelectronics Progress, Volume. 59, Issue 7, 0700001(2022)

Principle and Research Progress of Atmospheric Remote Sensing by Intense Femtosecond Lasers

Tiejun Wang1,2、*, Na Chen1,2, Hao Guo1,2, Yaoxiang Liu1,2, Yuxin Leng1,2, and Ruxin Li1,2
Author Affiliations
  • 1State Key Laboratory of High Field Laser Physics and Chinese Academy of Sciences, Center for Excellence in Ultra-Intense Laser Science, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, China
  • 2Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing , 100049, China
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    Figures & Tables(13)
    Dominant physical processes during intense femtosecond laser nonlinear filamentation. (a) Beam self-focusing induced by optical Kerr effect; (b) beam self-defocusing induced by laser ionized plasma[7]
    Schematic setup for remote femtosecond laser filament induced breakdown spectroscopy
    R-FIBS experiments by Teramobile at a distance up 90 m. (a) Experimental schematic setup for R-FIBS and beam cross section containing 30 filaments; (b) fluorescence signal of metallic target of Fe at the remote distance of 90 m[33]
    Experimental setups for spatio-temporally chirped femtosecond laser filamentation. (a) Principal demonstration; (b) application on R-FIBS[53]
    Fluorescence spectra of neutral (a) Fe and (b) Al induced by spatio-temporally chirped femtosecond laser filamentation at a distance of 22 m (solid lines), and fluorescence spectra excited by normal 50 fs laser filamentation under same focusing condition (dashed lines)[53]
    R-FIBS measurements of radioactive uranium. (a) Intensity of atomic line (U I 591.54 nm) and molecular spectral band (UO 593.55 nm) as a function of second-order dispersion of incident laser pulse (inset is the initial laser beam profile); (b) beam cross-sections under different second-order dispersion pulse widths recorded by interaction between beam and optical disc (accumulated 40 laser pulses)[57]
    Supercontinuum spectrum of 200 nm‒14 μm produced by terawatt femtosecond laser filamentation in air[26]
    Polarization dependent supercontinuum generation by filamentation. (a) Supercontinuum spectra from air filamentation under different laser polarizations (laser pulse energy is 4.75 mJ); (b) laser filament induced supercontinuum spectral intensity as a function of angle of quarter wave plate[24]
    White light laser generation by tuning the incident angle between different laser incident directions and normal direction of focusing filament lens. (a) Side fluorescence images of femtosecond laser filaments in air; (b)‒(e) corresponding real color images of forward white light lasers[60]
    Atmospheric sensing of filament induced supercontinuum Lidar. (a) Schematically experimental setup of femtosecond laser filament based supercontinuum Lidar; (b) range-corrected Lidar signals at 270 nm, 300 nm, and 600 nm as a function of vertical distance to the ground; (c) high resolution atmospheric absorption spectra at the vertical distance of 4.5 km to the ground recorded by filament induced supercontinuum Lidar[4]
    Single pulse signal of filament induced supercontinuum Lidar in the spectral range of 300‒470 nm[65]
    Schematic model of atmospheric sensing based on spaceborne filament induced supercontinuum Lidar[71]
    • Table 1. Comparison of the advantages and application scenario of FIBS at different central wavelengths

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      Table 1. Comparison of the advantages and application scenario of FIBS at different central wavelengths

      Central wavelength of pump laser pulsePhoton energy of pump laserAdvantagesApplication scenarios
      UVHighHigh photon energy, better resolution spectroscopy, better ablation efficiency

      Cultural heritage items: different metal and stones types41

      Explosives: DNT and ammonium perchlorate42

      IRLowMature technology to reach high laser energy, higher clamped intensity, reach longer atmospheric distance

      Widely investigated in many applications:

      atmospheric remote sensing with sample phases from gas, liquid to aerosol and solid618-1937

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    Tiejun Wang, Na Chen, Hao Guo, Yaoxiang Liu, Yuxin Leng, Ruxin Li. Principle and Research Progress of Atmospheric Remote Sensing by Intense Femtosecond Lasers[J]. Laser & Optoelectronics Progress, 2022, 59(7): 0700001

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    Paper Information

    Category: Reviews

    Received: Aug. 10, 2021

    Accepted: Sep. 24, 2021

    Published Online: Mar. 8, 2022

    The Author Email: Tiejun Wang (tiejunwang@siom.ac.cn)

    DOI:10.3788/LOP202259.0700001

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