Chinese Journal of Lasers, Volume. 45, Issue 9, 903001(2018)

Optical Properties of Dithienylethene and Its Applications in Super-Resolution Optical Storage

Liu Tiecheng1,2, Zhang Li3, Sun Jing3, Zhong Yuwu4, Wang Zhongyang3, Guo Xinjun1, and Ruan Hao1
Author Affiliations
  • 1[in Chinese]
  • 2[in Chinese]
  • 3[in Chinese]
  • 4[in Chinese]
  • show less
    Figures & Tables(7)
    Optical paths. (a) Optical path for Z-scan; (b) optical path for detection of fluorescence spectrum
    Spectrum versus time and cycle diagram of fluorescence switch. (a) Ultraviolet-visible absorption spectrum versus UV irradiation time (inset: structure of diarylethene D1); (b) fluorescence spectrum versus time; (c) fluorescence spectrum conversed by ring-opening versus time under irradiation by 375 nm laser; (d) cycle diagram of fluorescence switch under alternating irradiation by ultraviolet and visible light
    Test results. (a) Fluorescence spectrum conversed by ring-opening via two-photon absorption versus time (inset: fluorescence intensity contrast versus ring-opening two-photon absorption conversion power density; (b) data and fitting results from ring-opening Z-scan; (c) schematic of photon-erasing effect of diarylethene D1 in super-resolution optical storage; (d) fluorescence-quenching spectrum of diarylethene D1
    Calculation results of effective absorption intensity of two-photon-dual-beam and absorption intensity resolution. (a) Effective absorption intensity when inhibition ratio is 2; (b) effective absorption intensity resolution under different fluorescence intensity contrast; (c) simulated longitudinal resolution of linear energy absorption intensity; (d) simulated longitudinal resolution of effective absorption intensity; (e) simulated effective absorption intensity after threshold control; (f) eff
    Schematic of optical recording and reading of diarylethene D1. (a) Super-resolution; (b) original
    • Table 1. Conversion power density threshold of ring-opening two-photon absorption and photon energy threshold versus wavelength

      View table

      Table 1. Conversion power density threshold of ring-opening two-photon absorption and photon energy threshold versus wavelength

      Wavelength /nm740760780800
      Power density threshold /(GW·cm-2)107.36173.53198.75251.87
      Photon energy threshold /(1022 GJ·mol-1·cm-3)1.8962.913.1753.92
    • Table 2. Fluorescence quenching contrast versus power density

      View table

      Table 2. Fluorescence quenching contrast versus power density

      Power density /(GW·cm-2)Initial value /photonQuenchingvalue /photonAStable value under375 nm irradiation /photonB
      1.441963126607.4147071.3
      2.531475018687.958452.5
      2.751253516297.734523.6
      2.891993224868.049704.0
      3.371528218208.435724.3
      3.861438078118.418477.8
    Tools

    Get Citation

    Copy Citation Text

    Liu Tiecheng, Zhang Li, Sun Jing, Zhong Yuwu, Wang Zhongyang, Guo Xinjun, Ruan Hao. Optical Properties of Dithienylethene and Its Applications in Super-Resolution Optical Storage[J]. Chinese Journal of Lasers, 2018, 45(9): 903001

    Download Citation

    EndNote(RIS)BibTexPlain Text
    Save article for my favorites
    Paper Information

    Category: materials and thin films

    Received: Feb. 9, 2018

    Accepted: --

    Published Online: Sep. 8, 2018

    The Author Email:

    DOI:10.3788/CJL201845.0903001

    Topics