NUCLEAR TECHNIQUES, Volume. 47, Issue 1, 010302(2024)
Separation of rare earth fission products from LiF-BeF2 molten salt by sulfide precipitation
Fig. 1. LiF-BeF2 and REF3-LiF-BeF2 mixed molten salts (color online)(a) LiF-BeF2, (b) NdF3-LiF-BeF2, (c) CeF3-LiF-BeF2, (d) SmF3-LiF-BeF2, (e) YbF3-LiF-BeF2
Fig. 3. Removal ratios when the ratio of NdF3 to Na2S∙5H2O content is 1:2 under different temperatures for 5 h
Fig. 4. Photograph of Salt after adding Na2S·5H2O to REF3-LiF-BeF2 at 600 °C (a) NdF3, (b) CeF3, (c) SmF3, (d) YbF3
Fig. 5. XRD patterns of the precipitates after adding Na2S·5H2O to REF3-LiF-BeF2(a) NdF3, (b) CeF3, (c) SmF3, (d) EuF3
Fig. 6. SEM images of the precipitates after adding Na2S·5H2O to NdF3 (a), SmF3 (b)-LiF-BeF2 molten salt
Fig. 7. EDS images of precipitates after adding Na2S·5H2O to EuF3-LiF-BeF2 molten salt
Fig. 8. S 2p XPS spectra of precipitate after adding Na2S∙5H2O to NdF3-LiF-BeF2
Fig. 9. Removal ratio comparison of two systems for RE elements (Nd, Ce, Sm, and Eu)
Fig. 10. Snapshots of distillation equipment (a) and quartz tube with nickel foil collection device (b)[28]
Fig. 11. Photograph of ThF4-LiF-BeF2 salt (a) and mixed molten salt after adding Na2S∙5H2O (b)
Fig. 12. XRD patterns of precipitates after adding Na2S·5H2O to ThF4-LiF-BeF2
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Yujiao WANG, Yaxin QU, Haiying FU, Ming CHENG, Qiang DOU, Yu GONG. Separation of rare earth fission products from LiF-BeF2 molten salt by sulfide precipitation[J]. NUCLEAR TECHNIQUES, 2024, 47(1): 010302
Category: Research Articles
Received: Jul. 23, 2023
Accepted: --
Published Online: Mar. 7, 2024
The Author Email: FU Haiying (付海英)