Journal of Quantum Optics, Volume. 29, Issue 1, 10002(2023)
Research Progress of Rydberg Molecules
[1] [1] SCHLAGMLLER M, LIEBISCH T C, ENGEL F K, et al. Ultracold Chemical Reactions of a Single Rydberg Atom in a Dense Gas[J]. Phys Rev X, 2016, 6(3):031020. DOI: 10.1103/PhysRevX.6.031020.
[2] [2] SECKER T, GERRITSMA R, GLAETZLE A W, et al. Controlled long-range interactions between Rydberg atoms and ions[J]. Phys Rev A, 2016 94(1):013420. DOI: 10.1103/PhysRevA.94.013420.
[3] [3] BOISSEAU C, SIMBOTIN I, CT R. Macrodimers: Ultralong range Rydberg molecules[J]. Phys Rev Lett, 2002, 88(13):133004. DOI: 10.1103/PhysRevLett.88.133004.
[4] [4] OVERSTREET K R, SCHWETTMANN A, TALLANT J, et al. Observation of electric-field-induced Cs Rydberg atom macrodimers[J]. Nat Phys, 2009, 5(8):581-585. DOI:10.1038/nphys1307.
[5] [5] DEIGLMAYR J, SAMANNSHAUSEN H, PILLET P, et al. Observation of Dipole-Quadrupole Interaction in an Ultracold Gas of Rydberg Atoms[J]. Phys Rev Lett, 2014, 113(19):193001. DOI:10.1103/physrevlett.113.193001.
[6] [6] SAMANNSHANSEN H, DEIGLMAYR J. Observation of Rydberg-Atom Macrodimers: Micrometer-Sized Diatomic Molecules[J]. Phys Rev Lett, 2016, 117(8):083401. DOI:10.1103/physrevlett.117.083401.
[7] [7] HAN X, BAI S, JIAO Y, et al. Cs 62DJ Rydberg-atom macrodimers formed by long-range multipole interaction[J]. Phys Rev A, 2018, 97(3):031403(R). DOI:10.1103/physreva.97.031403.
[8] [8] HAN X, BAI S, JIAO Y, et al. Adiabatic potentials of cesium (nDJ)2 Rydberg-Rydberg macrodimers[J]. J Phys B: At Mol Opt Phys, 2019, 52(13):135102. DOI:10.1088/1361-6455/ab1371.
[10] [10] SHAFFER J P, RITTENHOUSE S T, SADEGHPOUR H R. Ultracold Rydberg molecules[J]. Nat Commu, 2018, 9:1965. DOI: 10.1038/s41467-018-04135-6.
[11] [11] BORN M, OPPENHEIMER J R. Zur Quantentheorie der Molekeln[J]. Ann Phys, 1927, 84:457-484. DOI: 10.1002/andp.19273892002.
[12] [12] SCHWETTMANN A, CRAWFORD J, OVERSTREET K R, et al. Cold Cs Rydberg-gas interactions[J]. Phys Rev A, 2006, 74(2):020701(R). DOI: 10.1103/PhysRevA.74.020701.
[13] [13] DEIGLMAYR J. Long-range interactions between Rydberg atoms[J]. Phys Scr, 2016, 91(10):104007. DOI:10.1088/0031-8949/91/10/104007.
[14] [14] HOLLERITH S, ZEIHER J, RUI J, et al. Quantum gas microscopy of Rydberg macrodimers[J]. Science, 2019, 364(6441):664-667. DOI:10.1126/science.aaw4150.
[15] [15] OMONT A. On the theory of collisions of atoms in Rydberg states with neutral particles[J]. J Phys, 1977, 38(11):1343-1359. DOI: 10.1051/ jphys: 0197700380110134300.
[16] [16] GREENE C H, DICKINSON A S, SADEGHPOUR H R. Creation of Polar and Nonpolar Ultra-Long-Range Rydberg molecules[J]. Phys Rev Lett, 2000, 85(12):2458-2461. DOI: 10.1103/PhysRevLett.85.2458.
[17] [17] CHIBISOV M I, KHUSKIVADZE A A, FABRIKANT I I. Energies and dipole moments of long-range molecular Rydberg states[J]. J Phys B: At Mol Opt Phys, 2002, 35(10):L193-L198. DOI: 10.1088/0953-4075/35/10/101.
[18] [18] HAMILTON E L, GREENE C H, SADEGHPOUR H R. Shape-resonance-induced long-range molecular Rydberg states[J]. J Phys B: At Mol Opt Phys, 2002, 35(10):L199-L206. DOI: 10.1088/0953-4075/35/10/102.
[19] [19] BENDKOWSKY V, BUTSCHER B, NIPPER J, et al. Observation of ultralong-range Rydberg molecules[J]. Nature, 2009, 458(7241):1005-1008. DOI: 10.1038/nature07945.
[20] [20] BELLOS M A, CAROLLO R, BANERJEE J, et al. Excitation of weakly-bound molecules to trilobite-like Rydberg states[J]. Phys Rev Lett, 2013, 111(5):053001. DOI: 10.1103/PhysRevLett.111.053001.
[21] [21] ANDERSON D A, MILLER S A, RAITHEL G. Photoassociation of long-range nD Rydberg molecules[J]. Phys Rev Lett, 2014, 112(16):163201. DOI: 10.1103/PhysRevLett.112.163201.
[22] [22] KRUPP A T, GAJ A, BALEWSKI J B, et al. Alignment of D-State Rydberg Molecules[J]. Phys Rev Lett, 2014, 112(14):143008. DOI: 10.1103/physrevlett.112.143008.
[23] [23] MACLENNAN J L, CHEN Y J, RAITHEL G. Deeply bound (24DJ+5S1/2) 87Rb and 85Rb molecules for eight spin couplings[J]. Phys Rev A, 2019, 99(3):033407. DOI: 10.1103/physreva.99.033407.
[24] [24] BOOTH D, RITTENHOUSE S T, YANG J, et al. Production of trilobite Rydberg molecule dimers with kilo-Debye permanent electric dipole moments[J]. Science, 2015, 348(6230):99-102. DOI:10.1126/science.1260722.
[25] [25] TALLANT J, RITTENHOUSE S T, BOOTH D, et al. Observation of blue-shifted ultralong-range Cs2 Rydberg molecules[J]. Phys Rev Lett, 2012, 109(17):173202. DOI: 10.1103/PhysRevLett.109.173202.
[26] [26] SAMANNSHAUSEN H, MERKT F, DEIGLMAYR J. Experimental Characterization of Singlet Scattering Channels in Long-Range Rydberg Molecules[J]. Phys Rev Lett, 2015, 114(13):133201. DOI: 10.1103/PhysRevLett. 114.133201.
[27] [27] FEY C, YANG J, RITTENHOUSE S T, et al. Effective Three-Body Interactions in Cs(6s)-Cs(nd) Rydberg Trimers[J]. Phys Rev Lett, 2019, 122(10):103001. DOI: 10.1103/PhysRevLett.122.103001.
[28] [28] BAI S, HAN X, BAI J, et al. Cesium nDJ+6S1/2 Rydberg molecules and their permanent electric dipole moments[J]. Phys Rev Research, 2020, 2(3):033525. DOI: 10.1103/PhysRevResearch.2.033525.
[29] [29] BAI S, HAN X, BAI J, et al. Observation of photoassociation spectroscopy of ultralong 37D5/2+6S1/2 Cs2 Rydberg molecules[J]. J Chem Phys, 2020, 152(8):084302. DOI:10.1063/1.5132993.
[30] [30] BENDKOWSKY V. Ultralong-range Rydberg molecules: investigation of a novel binding[D]. Universitt Stuttgart. 2010.
[32] [32] ANDERSON D A, MILLER S A, RAITHEL G. Angular-momentum couplings in long-range Rb2 Rydberg molecules[J]. Phys Rev A, 2014, 90(6):062518. DOI: 10.1103/PhysRevA.90.062518.
[33] [33] YANG Y, KHN O. A concise method for kinetic energy quantisation[J]. Mol Phys, 2008, 106(21):2445-2457. DOI: 10.1080/00268970802562117.
[34] [34] YANG Y, MEUWLY M. A generalized reactive force field for nonlinear hydrogen bonds: Hydrogen dynamics and transfer in malonaldehyde[J]. J Chem Phys, 2010, 133(6):064503. DOI: 10.1063/1.3447701.
[35] [35] YANG Y, LIU X, MEUWLY M, et al. Harmonic Bath Averaged Hamiltonian: An efficient Tool To Capture Quantum Effects of Large Systems[J]. J. Phys. Chem. A, 2012, 116(46):11134-11139. DOI:10.1021/jp304498h.
[36] [36] LI W, POHL T, ROST J M, et al. A Homonuclear Molecule with a Permanent Electric Dipole Moment[J]. Science, 2011, 334(6059):1110-1114. DOI:10.1126/science.1211255.
[37] [37] NIEDERPRM T, THOMAS O, EICHERT T, et al. Observation of pendular butterfly Rydberg molecules[J]. Nat Commun, 2016, 7(1):12820. DOI: 10.1038/ncomms12820.
[38] [38] MARKSON S, RITTENHOUSE S T, SCHMIDT R, et al. Theory of Ultralong-Range Rydberg Molecule Formation Incorporating Spin-Dependent Relativistic Effects: Cs(6s) -Cs(np) as Case Study[J]. Chem Phys Chem, 2016, 17(22):3683-3691. DOI: doi:10.1002/cphc.201600932.
[39] [39] BUTSCHER B, BENDKOWSKY V, NIPPER J, et al. Lifetimes of ultralong-range Rydberg molecules in vibrational ground and excited states[J]. J Phys B: At Mol Opt Phys, 2011, 44(18):184004. DOI: 10.1088/0953-4075/44/18/184004.
[40] [40] CAMARGO F, WHALEN J D, DING R, et al. Lifetimes of ultra-long-range strontium Rydberg molecules[J]. Phys Rev A, 2016, 93(2):022702. DOI: 10.1103/PhysRevA.93.022702.
[41] [41] WEIMER H, MLLER M, LESANOVSKY I, et al. A Rydberg quantum simulator[J]. Nat Phys, 2010, 6(5):382-388. DOI: 10.1038/nphys1614.
[42] [42] LUKIN M D, FLEISCHHAUER M, COTE R, et al. Dipole Blockade and Quantum Information Processing in Mesoscopic Atomic Ensembles[J]. Phys Rev Lett, 2001, 87(3):037901. DOI: 10.1103/PhysRevLett.87.037901.
[43] [43] DEMILLE D. Quantum computation with trapped polar molecules[J]. Phys Rev Lett, 2002, 88(6):067901. DOI: 10.1103/PhysRevLett.88.067901.
[44] [44] RABL P, DEMILLE D, DOYLE J. M, et al. Hybrid Quantum Processors: molecular ensembles as quantum memory for solid state circuits[J]. Phys Rev Lett, 2006, 97(3):033003. DOI: 10.1103/PhysRevLett.97.033003.
[45] [45] ALIZADEH E, ORLANDO T M, SANCHE L. Biomolecular Damage Induced by Ionizing Radiation: The Direct and Indirect Effects of Low-Energy Electrons on DNA[J]. Annu Rev Phys Chem, 2015, 66(1):379-398. DOI: 10.1146/annurev-physchem-040513-103605.
[46] [46] BALD I, KOPYRA J, ILLENBERGER E. Selective Excision of C5 from D-Ribose in the Gas Phase by Low-Energy Electrons (0 -1 eV): Implications for the Mechanism of DNA Damage[J]. Angew Chem Int Ed, 2006, 45(29):4851-4855. DOI: 10.1002/anie.200600303.
[47] [47] SIMONS J. How Do Low-Energy (0.1 -2 eV) Electrons Cause DNA-Strand Breaks? [J]Acc Chem Res, 2006, 39(10):772-779. DOI: 10.1021/AR0680769.
[48] [48] MARTIN F, P BURROW D, CAI Z, et al. DNA Strand Breaks Induced by 0 -4 eV Electrons: The Role of Shape Resonances[J]. Phys Rev Lett, 2004, 93(6):068101. DOI: 10.1103/PhysRevLett.93.068101
[49] [49] CARON L G, SANCHE L. Low-Energy Electron Diffraction and Resonances in DNA and other Helical Macromolecules[J]. Phys Rev Lett, 2003, 91(11):113201. DOI: 10.1103/PhysRevLett.91.113201.
[50] [50] DUSPAYEV A, HAN X, VIRAY M, et al. Long-range Rydberg-atom-ion molecules of Rb and Cs[J]. Phys Rev Research, 2021, 3(2):023114. DOI: 10.1103/PhysRevResearch.3.023114.
[51] [51] DEI M, HAZE S, DENSCHLAG J H. Long-range atom-ion Rydberg molecule: a novel molecular binding mechanism[J]. Atoms, 2021, 9:34. DOI: 10.3390/atoms9020034.
[52] [52] JACKSON J D. Classical Electrodynamics[M]. 3rd ed. New Jersey: Wiley, 1999.
[53] [53] WEBER S, TRESP C, MENKE H, et al. Calculation of Rydberg interaction potentials[J]. J Phys B: At Mol Opt Phys, 2017, 50(13):133001. DOI:10.1088/1361-6455/aa743a.
[54] [54] ZUBER N, ANASURI V S V, BERNGRUBER M. et al. Observation of a molecular bond between ions and Rydberg atoms[J]. Nature, 2022, 605:453-456. DOI: 10.1038/s41586-022-04577-5.
Get Citation
Copy Citation Text
GUO Shu-rong, HAN Xiao-xuan, PENG Peng, QIAO Xiao-fei. Research Progress of Rydberg Molecules[J]. Journal of Quantum Optics, 2023, 29(1): 10002
Received: Aug. 22, 2022
Accepted: --
Published Online: Nov. 17, 2023
The Author Email: HAN Xiao-xuan (xxhan21@163.com)