Journal of Atmospheric and Environmental Optics, Volume. 20, Issue 2, 188(2025)

Investigation of photolysis of glyoxal/ammonium sulfate aqueous secondary organic aerosol

FAN Jiafu1, YU Yuanqin1, GU Xuejun2、*, and TANG Xiaofeng2
Author Affiliations
  • 1School of Physicals and Optoelectronics Engineering of Anhui University, Hefei 230601, China
  • 2Anhui Institute of Optics and Fine Mechanics Basic Science Physics Research Center, HFIPS,Chinese Academy of Sciences, Hefei 230031, China
  • show less
    References(30)

    [1] Seinfeld J H, Pandis S N[M]. Atmospheric Chemistry and Physics: From Air Pollution to Climate Change(2006).

    [2] Suda S R, Petters M D, Yeh G K et al. Influence of functional groups on organic aerosol cloud condensation nucleus activity[J]. Environmental Science & Technology, 48, 10182-10190(2014).

    [3] Fu T M, Jacob D J, Wittrock F et al. Global budgets of atmospheric glyoxal and methylglyoxal, and implications for formation of secondary organic aerosols[J]. Journal of Geophysical Research Atmospheres, 113, 303-320(2008).

    [4] Lacoste C, Basso M C, Pizzi A et al. Bioresourced pine tannin/furanic foams with glyoxal and glutaraldehyde[J]. Industrial Crops and Products, 45, 401-405(2013).

    [5] Nishino N, Arey J, Atkinson R. Formation yields of glyoxal and methylglyoxal from the gas-phase OH radical-initiated reactions of toluene, xylenes, and trimethylbenzenes as a function of NO2 concentration[J]. Journal of Physical Chemistry A, 114, 10140-10147(2010).

    [6] Kaiser J, Wolfe G M, Min K E et al. Reassessing the ratio of glyoxal to formaldehyde as an indicator of hydrocarbon precursor speciation[J]. Atmospheric Chemistry & Physics, 15, 7571-7583(2015).

    [7] Kawamura K, Okuzawa K, Aggarwal S G et al. Determination of gaseous and particulate carbonyls (glycolaldehyde, hydroxyacetone, glyoxal, methylglyoxal, nonanal and decanal) in the atmosphere at Mt. Tai[J]. Atmospheric Chemistry and Physics, 13, 5369-5380(2013).

    [8] Hastings W P, Koehler C A, Bailey E L et al. Secondary organic aerosol formation by glyoxal hydration and oligomer formation: Humidity effects and equilibrium shifts during analysis[J]. Environmental Science & Technology, 39, 8728-8735(2005).

    [9] Lu Z, Hao J, Takekawa H et al. Effect of high concentrations of inorganic seed aerosols on secondary organic aerosol formation in the m-xylene/NOx photooxidation system[J]. Atmospheric Environment, 43, 897-904(2009).

    [10] Laskin A, Laskin J, Nizkorodov S A. Chemistry of atmospheric brown carbon[J]. Chemical Reviews, 115, 4335-4382(2015).

    [11] Grace D N, Lugos E N, Ma S Q et al. Brown carbon formation potential of the biacetyl-ammonium sulfate reaction system[J]. ACS Earth and Space Chemistry, 4, 1104-1113(2020).

    [12] Yu G, Bayer A R, Galloway M M et al. Glyoxal in aqueous ammonium sulfate solutions: Products, kinetics and hydration effects[J]. Environmental Science & Technology, 45, 6336-6342(2011).

    [13] Heald C L, Ridley D A, Kreidenweis S M et al. Satellite observations cap the atmospheric organic aerosol budget[J]. Geophysical Research Letters, 37, 808-812(2010).

    [14] Wildt J, Surratt J D, Seinfeld J H et al. The formation, properties and impact of secondary organic aerosol: Current and emerging issues[J]. Atmospheric Chemistry and Physics, 9, 5155-5236(2009).

    [15] Docherty K S, Wu W, Lim Y B et al. Contributions of organic peroxides to secondary aerosol formed from reactions of monoterpenes with O3[J]. Environmental Science & Technology, 39, 4049-4059(2005).

    [16] Russell L M, Bahadur R, Ziemann P J. Identifying organic aerosol sources by comparing functional group composition in chamber and atmospheric particles[J]. Proceedings of the National Academy of Sciences, 108, 3516-3521(2011).

    [17] Zhao R, Lee A K Y, Huang L et al. Photochemical processing of aqueous atmospheric brown carbon[J]. Atmospheric Chemistry and Physics, 15, 6087-6100(2015).

    [18] Hoyle C R, Boy M, Donahue N M et al. A review of the anthropogenic influence on biogenic secondary organic aerosol[J]. Atmospheric Chemistry and Physics, 11, 321-343(2011).

    [19] Kroll J H, Seinfeld J H. Chemistry of secondary organic aerosol: Formation and evolution of low-volatility organics in the atmosphere[J]. Atmospheric Environment, 42, 3593-3624(2008).

    [20] Hodzic A, Madronich S, Kasibhatla P S et al. Organic photolysis reactions in tropospheric aerosols: Effect on secondary organic aerosol formation and lifetime[J]. Atmospheric Chemistry & Physics, 15, 8113-8149(2015).

    [21] Epstein S A, Blair S L, Nizkorodov S A et al. Direct photolysis of a-pinene ozonolysis secondary organic aerosol: Effect on particle mass and peroxide content[J]. Environmental Science and Technology, 48, 11251-11258(2014).

    [22] Mang S A, Henricksen D K, Bateman A P et al. Contribution of carbonyl photochemistry to aging of atmospheric secondary organic aerosol[J]. The Journal of Physical Chemistry A, 112, 8337-8344(2008).

    [23] Grace D N, Sharp J R, Holappa R E et al. Heterocyclic product formation in aqueous brown carbon systems[J]. ACS Earth and Space Chemistry, 3, 2472-2481(2019).

    [24] Sareen N, Moussa S G, McNeill V F. Photochemical aging of light-absorbing secondary organic aerosol material[J]. The Journal of Physical Chemistry A, 117, 2987-2996(2013).

    [25] Maxut A, Nozière B, Fenet B et al. Formation mechanisms and yields of small imidazoles from reactions of glyoxal with NH4+ in water at neutral pH[J]. Physical Chemistry Chemical Physics, 17, 20416-20424(2015).

    [26] Fan M J, Ma S Q, Ferdousi N et al. Modeling of carbonyl/ammonium sulfate aqueous brown carbon chemistry via UV/vis spectral decomposition[J]. Atmosphere, 11, 358-369(2020).

    [27] Renbaum-Wolff L, Grayson J W, Bateman A P et al. Viscosity of α-pinene secondary organic material and implications for particle growth and reactivity[J]. Proceedings of the National Academy of Sciences, 110, 8014-8019(2013).

    [28] Gomez M E, Lin Y, Guo S et al. Heterogeneous chemistry of glyoxal on acidic solutions. An oligomerization pathway for secondary organic aerosol formation[J]. Journal of Physical Chemistry A, 119, 4457-4463(2015).

    [29] Lin X, Huang M Q, Zhang W et al. Effects of ammonium sulfate fine particle on the optical properties of benzene secondary organic aerosol[J]. Acta Scientiae Circumstantiae, 41, 2560-2568(2021).

    [30] Nakao S, Liu Y, Tang P et al. Chamber studies of SOA formation from aromatic hydrocarbons: Observation of limited glyoxal uptake[J]. Atmospheric Chemistry and Physics, 12, 3927-3937(2012).

    Tools

    Get Citation

    Copy Citation Text

    Jiafu FAN, Yuanqin YU, Xuejun GU, Xiaofeng TANG. Investigation of photolysis of glyoxal/ammonium sulfate aqueous secondary organic aerosol[J]. Journal of Atmospheric and Environmental Optics, 2025, 20(2): 188

    Download Citation

    EndNote(RIS)BibTexPlain Text
    Save article for my favorites
    Paper Information

    Category:

    Received: Feb. 23, 2022

    Accepted: --

    Published Online: May. 30, 2025

    The Author Email: Xuejun GU (xjgu@aiofm.ac.cn)

    DOI:10.3969/j.issn.1673-6141.2025.02.007

    Topics