Acta Optica Sinica, Volume. 45, Issue 6, 0601003(2025)

Point Source Carbon Emission Measurement Using Portable EM27/SUN Spectrometer: A Case Study of Hefei Wanneng Power Plant

Chao Li1,2,3, Xianhua Wang1,2,3、*, Hanhan Ye1,3, Shichao Wu1,3, Hailiang Shi1,2,3, Erchang Sun1,2,3, and Yuan An1,2,3
Author Affiliations
  • 1Anhui Institute of Optics and Fine Mechanics, Hefei Institutes of Physical Science, Chinese Academy of Sciences, Hefei 230031, Anhui , China
  • 2University of Science and Technology of China, Hefei 230026, Anhui , China
  • 3Key Laboratory of General Optical Calibration and Characterization Technology, Chinese Academy of Sciences, Hefei 230031, Anhui , China
  • show less
    Figures & Tables(20)
    Diagram of smoke plume dispersion principle
    Schematic of measurement instruments[18]. (a) Outdoor photograph of a single measurement experiment; (b) external structure of EM27/SUN instrument; (c) internal structure of EM27/SUN instrument
    Spectra measured by EM27/SUN. (a) 0.625‒2.5 μm; (b) around 1.6 μm (6300‒6400 cm-1)
    Diagram of synchronous observation locations of EM27/SUN and TCCON stations
    XCO2 results from EM27/SUN compared to TCCON before and after correction (2021‒2023). (a) In 2021; (b) in 2022; (c) in 2023
    Location map of WN Power Plant
    Distribution of measurement point locations based on EM27/SUN instrument. (a) Distribution of measurement points; (b) surrounding environment of an upper-wind measurement point; (c) surrounding environment of a down-wind measurement point
    Impact of lightpath obstruction on EM27/SUN measurements. (a) Spectral curves around 1.6 μm for measurement points P01‒P04; (b) sun intensity at P01‒P04
    Variations in incident sun intensity for EM27/SUN measurement on April 2, 2022. (a) Before filtering; (b) after filtering
    XCO2 results at the upper-wind and down-wind outlets of WN Power Plant at different time. (a) In 2021; (b) in 2022; (c) in 2023
    Relationship between XCO2 variation characteristics and the distance from emission source
    Simulation results of XCO2, wind direction, and wind speed at Points 1 and 2 with and without buildings. (a) Geographic location of measurement points; (b) XCO2; (c) wind direction; (d) wind speed
    XCO2 results of EM27/SUN at different measurement points. (a) Scatter plot; (b) box plot
    Estimated CO2 emission intensity over time. (a) Point 1; (b) Point 2
    Estimated CO2 emission intensity at different distances from the emission source
    Measurement distance and estimated emission intensity from 2021 to 2023. (a) Statistics between measurement sections and emission source distances; (b) estimated results of annual average CO2 emission intensity
    • Table 1. Parameters of EM27/SUN instrument

      View table

      Table 1. Parameters of EM27/SUN instrument

      ParameterInformation
      DetectorInGaS, extended InGaAs
      Spectral range0.625‒2.5 μm
      Spectral resolution<0.5 cm-1
      Maximum optical path difference1.8 cm
      Field of view (FOV)1.1 mrad
      Operating temperature-20‒50 
    • Table 2. XCO2results from EM27/SUN before and after correction based on TCCON

      View table

      Table 2. XCO2results from EM27/SUN before and after correction based on TCCON

      YearCorrection formulaBefore correctionAfter correction
      R2RMSE /10-6R2RMSE /10-6
      2021y=0.67x+134.610.850.410.980.27
      2022y=0.64x+148.500.830.360.980.26
      2023y=0.66x+142.760.820.350.970.19
    • Table 3. Collection information in the measurement experiment at WN Power Plant

      View table

      Table 3. Collection information in the measurement experiment at WN Power Plant

      LocationTime
      YearDate
      Upper-wind2021November 24‒27
      2022October 17‒20
      2023March 28‒29, April 2‒3
      Down-wind2021November 25‒26
      2022October 18‒19
      2023March 29, April 2
    • Table 4. Estimated CO2 emission intensity at Points 1 and 2

      View table

      Table 4. Estimated CO2 emission intensity at Points 1 and 2

      PointCO2 emission intensity /(kg/s)Retrieval error /(kg/s)
      Point 1228.47±18.69
      Point 2235.18±28.73
    Tools

    Get Citation

    Copy Citation Text

    Chao Li, Xianhua Wang, Hanhan Ye, Shichao Wu, Hailiang Shi, Erchang Sun, Yuan An. Point Source Carbon Emission Measurement Using Portable EM27/SUN Spectrometer: A Case Study of Hefei Wanneng Power Plant[J]. Acta Optica Sinica, 2025, 45(6): 0601003

    Download Citation

    EndNote(RIS)BibTexPlain Text
    Save article for my favorites
    Paper Information

    Category: Atmospheric Optics and Oceanic Optics

    Received: Jul. 2, 2024

    Accepted: Aug. 6, 2024

    Published Online: Mar. 26, 2025

    The Author Email: Xianhua Wang (xhwang@aiofm.ac.cn)

    DOI:10.3788/AOS241235

    CSTR:32393.14.AOS241235

    Topics