Acta Optica Sinica, Volume. 43, Issue 13, 1326002(2023)

High-Harmonic Spectral Shift of Water Under Two-Color Laser Fields

Xulin Zhao1,2, Lihua Bai1、**, Ya Bai2,3、*, and Peng Liu2,3
Author Affiliations
  • 1Department of Physics, Shanghai University, Shanghai 200444, China
  • 2State Key Laboratory of High Field Laser Physics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, China
  • 3Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing 100049, China
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    Figures & Tables(7)
    Electric field intensity of driving pulse and the band structure. (a) Electric field intensity of driving pulse at relative phase of ϕ=0.2π; (b) band structure used in the calculation
    High-order harmonic spectra from liquid water at the relative phase of ϕ=0.2π
    Time-frequency analysis spectra of the calculated high harmonic current at the relative phase of ϕ=0.2π, and time zero is the peak value of the electric field envelope
    High-order harmonic spectra changed with relative phase
    Contributions to harmonic spectra from positive half-cycle and negative half-cycle. (a) Positive half-cycle; (b) negative half-cycle
    Frequency shift of H9 and H11 from positive half-cycle and negative half-cycle. (a) H9; (b) H11
    • Table 1. Recombination time of H9 with positive and negative half-cycles at different ϕ

      View table

      Table 1. Recombination time of H9 with positive and negative half-cycles at different ϕ

      ϕtr in negative half-cycle /T0High harmonic order in negative half-cycletr in positive half-cycle /T0High harmonic order in positive half-cycleΔtrϕ /T0
      00.81899.17300.13839.51360.6806
      0.1π0.81139.27060.14109.51420.6703
      0.2π0.80509.34450.14069.48710.6644
      0.3π0.80109.38760.13799.44540.6631
      0.4π0.79879.39940.13299.39020.6658
      0.5π0.79969.37110.12579.31980.6739
      0.6π0.80239.30900.11769.24290.6847
      0.7π0.80739.21280.10879.15570.6986
      0.8π0.81409.09070.10019.06920.7139
      0.9π0.82168.95900.09298.99230.7287
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    Xulin Zhao, Lihua Bai, Ya Bai, Peng Liu. High-Harmonic Spectral Shift of Water Under Two-Color Laser Fields[J]. Acta Optica Sinica, 2023, 43(13): 1326002

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    Paper Information

    Category: Physical Optics

    Received: Dec. 22, 2022

    Accepted: Mar. 6, 2023

    Published Online: Jul. 12, 2023

    The Author Email: Bai Lihua (lhbai@163.com), Bai Ya (pipbear@siom.ac.cn)

    DOI:10.3788/AOS222167

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