Researching | Size matters: quantum confinement-driven dynamics in CsPbI3 quantum dot light-emitting diodes

Journal of Semiconductors, Volume. 46, Issue 4, 042103(2025)

Size matters: quantum confinement-driven dynamics in CsPbI₃ quantum dot light-emitting diodes

Shuo Li... Wenxu Yin, Weitao Zheng and Xiaoyu Zhang* |Show fewer author(s)

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School of Materials Science and Engineering, Jilin University, Changchun 130012, China

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[1] A P Alivisatos. Semiconductor clusters, nanocrystals, and quantum dots. Science, 271, 933(1996).

[2] O Chen, J Zhao, V P Chauhan et al. Compact high-quality CdSe-CdS core-shell nanocrystals with narrow emission linewidths and suppressed blinking. Nat Mater, 12, 445(2013).

[3] K S Cho, E K Lee, W J Joo et al. High-performance crosslinked colloidal quantum-dot light-emitting diodes. Nat Photonics, 3, 341(2009).

[4] X L Dai, Y Z Deng, X G Peng et al. Quantum-dot light-emitting diodes for large-area displays: Towards the dawn of commercialization. Adv Mater, 29, 1607022(2017).

[5] X Y Li, Y B Zhao, F J Fan et al. Bright colloidal quantum dot light-emitting diodes enabled by efficient chlorination. Nat Photonics, 12, 159(2018).

[6] Y Shirasaki, G J Supran, M G Bawendi et al. Emergence of colloidal quantum-dot light-emitting technologies. Nat Photonics, 7, 13(2013).

[7] Y X Yang, Y Zheng, W R Cao et al. High-efficiency light-emitting devices based on quantum dots with tailored nanostructures. Nat Photonics, 9, 259(2015).

[8] J Yoo, K Lee, U J Yang et al. Highly efficient printed quantum dot light-emitting diodes through ultrahigh-definition double-layer transfer printing. Nat Photonics, 18, 1105(2024).

[9] Y K Wang, H Y Wan, S Teale et al. Long-range order enabled stability in quantum dot light-emitting diodes. Nature, 629, 586(2024).

[10] P L Gao, Z N Chen, S M Chen. Electron-induced degradation in blue quantum-dot light-emitting diodes. Adv Mater, 36, e2309123(2024).

[11] D C Kim, H Seung, J Yoo et al. Intrinsically stretchable quantum dot light-emitting diodes. Nat Electron, 7, 365(2024).

[12] Y R Su, W B Ma, Y Yang. Perovskite semiconductors for direct X-ray detection and imaging. J Semicond, 41, 051204(2020).

[13] P Tamarat, E Prin, Y Berezovska et al. Universal scaling laws for charge-carrier interactions with quantum confinement in lead-halide perovskites. Nat Commun, 14, 229(2023).

[14] W G Chi, S K Banerjee. Application of perovskite quantum dots as an absorber in perovskite solar cells. Angew Chem Int Ed, 61, e202112412(2022).

[15] Y M Li, M Deng, X Y Zhang et al. Stable and efficient CsPbI3 quantum-dot light-emitting diodes with strong quantum confinement. Nat Commun, 15, 5696(2024).

[16] D Bera, L Qian, T K Tseng et al. Quantum dots and their multimodal applications: A review. Materials, 3, 2260(2010).

[17] L Polavarapu, B Nickel, J Feldmann et al. Advances in quantum-confined perovskite nanocrystals for optoelectronics. Adv Energy Mater, 7, 1700267(2017).

[18] W Z Li, J D Fan, L M Ding. Multidimensional perovskites enhance solar cell performance. J Semicond, 42, 020201(2021).

[19] F J Ye, W Q Yang, D Y Luo et al. Applications of cesium in the perovskite solar cells. J Semicond, 38, 011003(2017).

[20] W K Bae, Y S Park, J Lim et al. Controlling the influence of Auger recombination on the performance of quantum-dot light-emitting diodes. Nat Commun, 4, 2661(2013).

[21] Q Y Li, K F Wu, H M Zhu et al. Charge transfer from quantum-confined 0D, 1D, and 2D nanocrystals. Chem Rev, 124, 5695(2024).

[22] X F Liu, Q Zhang, G C Xing et al. Size-dependent exciton recombination dynamics in single CdS nanowires beyond the quantum confinement regime. J Phys Chem C, 117, 10716(2013).

[23] M V Kovalenko, L Protesescu, M I Bodnarchuk. Properties and potential optoelectronic applications of lead halide perovskite nanocrystals. Science, 358, 745(2017).

[24] M Lu, Y Zhang, S X Wang et al. Metal halide perovskite light-emitting devices: Promising technology for next-generation displays. Adv Funct Materials, 29, 1902008(2019).

[25] T H Han, K Y Jang, Y T Dong et al. A roadmap for the commercialization of perovskite light emitters. Nat Rev Mater, 7, 757(2022).

[26] B N Han, Q S Shan, F J Zhang et al. Giant efficiency and color purity enhancement in multicolor inorganic perovskite light-emitting diodes via heating-assisted vacuum deposition. J Semicond, 41, 052205(2020).

[27] J S Du, D Shin, T K Stanev et al. Halide perovskite nanocrystal arrays: Multiplexed synthesis and size-dependent emission. Sci Adv, 6, eabc4959(2020).

[28] Y Z Jiang, K Y Wei, C J Sun et al. Unraveling size-dependent ion-migration for stable mixed-halide perovskite light-emitting diodes. Adv Mater, 35, e2304094(2023).

[29] Y H Kim, C Wolf, Y T Kim et al. Highly efficient light-emitting diodes of colloidal metal-halide perovskite nanocrystals beyond quantum size. ACS Nano, 11, 6586(2017).

[30] A B Feng, X M Jiang, X Y Zhang et al. Shape control of metal halide perovskite single crystals: From bulk to nanoscale. Chem Mater, 32, 7602(2020).

[31] X M Jiang, S Q Xia, J Zhang et al. Exploring organic metal halides with reversible temperature-responsive dual-emissive photoluminescence. ChemSusChem, 12, 5228(2019).

[32] H J Li, Y F Feng, M Y Zhu et al. Nanosurface-reconstructed perovskite for highly efficient and stable active-matrix light-emitting diode display. Nat Nanotechnol, 19, 638(2024).

[33] Y Wang, T Y Zhang, M Kan et al. Bifunctional stabilization of all-inorganic α-CsPbI3 perovskite for 17% efficiency photovoltaics. J Am Chem Soc, 140, 12345(2018).

[34] Y Q Hu, F Bai, X B Liu et al. Bismuth incorporation stabilized α-CsPbI3 for fully inorganic perovskite solar cells. ACS Energy Lett, 2, 2219(2017).

[35] I L Aleiner, P W Brouwer, L I Glazman. Quantum effects in coulomb blockade. Phys Rep, 358, 309(2002).

[36] S R Patel, S M Cronenwett, D R Stewart et al. Statistics of coulomb blockade peak spacings. Phys Rev Lett, 80, 4522(1998).

[37] L M Kong, X Y Zhang, C X Zhang et al. Stability of perovskite light-emitting diodes: Existing issues and mitigation strategies related to both material and device aspects. Adv Mater, 34, e2205217(2022).

[38] J E Jeong, J H Park, C H Jang et al. Multifunctional charge transporting materials for perovskite light-emitting diodes. Adv Mater, 32, e2002176(2020).

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Shuo Li, Wenxu Yin, Weitao Zheng, Xiaoyu Zhang. Size matters: quantum confinement-driven dynamics in CsPbI₃ quantum dot light-emitting diodes[J]. Journal of Semiconductors, 2025, 46(4): 042103

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Paper Information

Category: Research Articles

Received: Dec. 14, 2024

Accepted: --

Published Online: May. 21, 2025

The Author Email: Xiaoyu Zhang (XYZhang)

DOI:10.1088/1674-4926/24120018

Topics

laser devices and laser physics

Lasers and Laser Optics

laser manufacturing

Instrumentation, Measurement and Metrology