Acta Optica Sinica, Volume. 39, Issue 8, 0830003(2019)

Photoluminescence Lifetime of CdSxSe1-x/ZnS (Core/Shell) Quantum Dot

Cheng Cheng and Xujun Deng*
Author Affiliations
  • Institute of Intelligent Optoelectronic Technology, Zhejiang University of Technology, Hangzhou, Zhejiang 310023, China
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    Figures & Tables(15)
    TEM images of CdSxSe1-x/ZnS quantum dot in water (sample No.6). (a) Low power; (b) high power
    Size distribution of QD (No.6 sample)
    Spectrogram of No.6 sample
    Absorption spectra of each sample
    PL radiation of each sample at room temperature. (a) PL wavelength of each samples; (b) PL-peaking wavelength varying with QD size
    Effect of temperature on PL radiation. (a) PL spectra at different temperatures of No. 6 sample; (b) PL-peaking wavelength varying with temperature of each samples
    PL-peaking wavelength varying with x
    PL versus time and fitting results. (a) Measured luminescence decay curves of QD; (b) original life data and fitting curve of No. 6 sample
    Fitting results of PL lifetime. (a) Weights ?1 and ?2 of PL lifetime of QD; (b) short lifetime τ1, long lifetime τ2, and average lifetime τ
    PL lifetime varying with size of CdSxSe1-x/ZnS QD
    Effect of element component ratio on PL lifetime. (a) Measured luminescence decay curves for different x values; (b) PL lifetime varying with x
    Effect of temperature on PL lifetime of No. 6 sample. (a) luminescence decay curves of QD at different temperatures; (b) PL lifetime varying with temperature
    • Table 1. Estimated size of CdSxSe1-x/ZnS QD

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      Table 1. Estimated size of CdSxSe1-x/ZnS QD

      No.123456
      Diameter d /nm4.064.896.757.888.119.22
    • Table 2. x of each sample

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      Table 2. x of each sample

      Sample No.123456
      x0.9450.7810.7010.6500.4330.366
    • Table 3. Element-component ratio calculated by PL-peaking wavelength

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      Table 3. Element-component ratio calculated by PL-peaking wavelength

      No.123456
      λp /nm506532546557598612
      x0.9340.7770.6990.6450.4400.383
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    Cheng Cheng, Xujun Deng. Photoluminescence Lifetime of CdSxSe1-x/ZnS (Core/Shell) Quantum Dot[J]. Acta Optica Sinica, 2019, 39(8): 0830003

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    Paper Information

    Category: Spectroscopy

    Received: Mar. 21, 2019

    Accepted: May. 5, 2019

    Published Online: Aug. 7, 2019

    The Author Email: Xujun Deng (dxujun@foxmail.com)

    DOI:10.3788/AOS201939.0830003

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