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Journal of Semiconductors, Volume. 46, Issue 5, 052803(2025)

Compositional engineering for lead-free antimony bismuth alloy-based halide perovskite solar cells

Ziyu Cai1、†, Junchi Zhu1、†, Chenyuan Ding1, Tao Dong1, Boyang Yu1, Wenzheng Hu1, Jiayi Xie1, Feng Ye2、*, Qiufeng Ye1、**, and Zebo Fang1、***
Author Affiliations
  • 1Zhejiang Engineering Research Center of MEMS, Shaoxing University, Shaoxing 312000, China
  • 2School of Textile Science and Engineering, Shaoxing University, Shaoxing 312000, China
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    [1] Z Liang, Y Zhang, H F Xu et al. Homogenizing out-of-plane cation composition in perovskite solar cells. Nature, 624, 557(2023).

    [2] Z H Wang, Z Y Han, X B Chu et al. Regulation of wide bandgap perovskite by rubidium thiocyanate for efficient silicon/perovskite tandem solar cells. Adv Mater, 36, 2407681(2024).

    [3] X Y Chin, D Turkay, J A Steele et al. Interface passivation for 31.25%-efficient perovskite/silicon tandem solar cells. Science, 381, 59(2023).

    [4] B W Park, B Philippe, X L Zhang et al. Bismuth based hybrid perovskites A3Bi2I9 (A: Methylammonium or cesium) for solar cell application. Adv Mater, 27, 6806(2015).

    [5] C F Lan, G X Liang, S Zhao et al. Lead-free formamidinium bismuth perovskites (FA)3Bi2I9 with low bandgap for potential photovoltaic application. Sol Energy, 177, 501(2019).

    [6] B B Yu, M Liao, J X Yang et al. Alloy-induced phase transition and enhanced photovoltaic performance: The case of Cs3Bi2I9–xBrx perovskite solar cells. J Mater Chem A, 7, 8818(2019).

    [7] P C Harikesh, H K Mulmudi, B Ghosh et al. Rb as an alternative cation for templating inorganic lead-free perovskites for solution processed photovoltaics. Chem Mater, 28, 7496(2016).

    [8] F Y Jiang, D W Yang, Y Y Jiang et al. Chlorine-incorporation-induced formation of the layered phase for antimony-based lead-free perovskite solar cells. J Am Chem Soc, 140, 1019(2018).

    [9] Y F Zhang, F Z Liu, H H Su et al. Controlling the intermediate phase to improve the crystallinity and orientation of Cs3Sb2ClxI9-x films for efficient solar cells. Adv Funct Materials, 33, 2304063(2023).

    [10] F Bai, Y H Hu, Y Q Hu et al. Lead-free, air-stable ultrathin Cs3Bi2I9 perovskite nanosheets for solar cells. Sol Energy Mater Sol Cells, 184, 15(2018).

    [11] F Umar, J Zhang, Z X Jin et al. Dimensionality controlling of Cs3Sb2I9 for efficient all-inorganic planar thin film solar cells by HCl-assisted solution method. Adv Opt Mater, 7, 1801368(2019).

    [12] M Shi, P Fu, W M Tian et al. Tuning the optoelectronic property of all-inorganic lead-free perovskite via finely microstructural modulation for photovoltaics. Small Meth, 8, 2300405(2024).

    [13] J Kang, S Chen, M M Hao et al. Alloying Sb into all inorganic lead-free CsBi3I10 for improving the crystal growth and photovoltaic performance. J Mater Chem A, 10, 19618(2022).

    [14] B Al-Anesi, G K Grandhi, A Pecoraro et al. Antimony-bismuth alloying: The key to a major boost in the efficiency of lead-free perovskite-inspired photovoltaics. Small, 19, 2303575(2023).

    [15] G Q Chen, P Wang, Y Q Wu et al. Lead-free halide perovskite Cs3Bi2xSb2–2xI9 (x ≈ 0.3) possessing the photocatalytic activity for hydrogen evolution comparable to that of (CH3NH3)PbI3. Adv Mater, 32, 2001344(2020).

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    Ziyu Cai, Junchi Zhu, Chenyuan Ding, Tao Dong, Boyang Yu, Wenzheng Hu, Jiayi Xie, Feng Ye, Qiufeng Ye, Zebo Fang. Compositional engineering for lead-free antimony bismuth alloy-based halide perovskite solar cells[J]. Journal of Semiconductors, 2025, 46(5): 052803

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    Paper Information

    Category: Research Articles

    Received: Dec. 9, 2024

    Accepted: --

    Published Online: Jun. 4, 2025

    The Author Email: Feng Ye (FYe), Qiufeng Ye (QFYe), Zebo Fang (ZBFang)

    DOI:10.1088/1674-4926/24120038

    Topics

    laser devices and laser physics
    Lasers and Laser Optics
    Laser physics
    laser manufacturing
    Instrumentation, Measurement and Metrology