Laser & Optoelectronics Progress, Volume. 62, Issue 11, 1127005(2025)

2D Material-Micro/Nano-Photonic Cavity Coupling Quantum Systems and Their Control in Multiple Degrees of Freedom (Invited)

Yuhang Li1,2, Xiulai Xu3,4,5、**, and Chenjiang Qian1,2、*
Author Affiliations
  • 1Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China
  • 2School of Physical Sciences, University of Chinese Academy of Sciences, Beijing 100049, China
  • 3School of Physics, Peking University, Beijing 100871, China
  • 4Yangtze Delta Institute of Optoelectronics, Peking University, Nantong 226010, Jiangsu , China
  • 5Collaborative Innovation Center of Extreme Optics, Shanxi University, Taiyuan 030006, Shanxi , China
  • show less
    Figures & Tables(9)
    Schematic diagrams of 2D material-micro/nano-photonic cavity coupling systems. (a) Monolayer 2D material; (b) multilayer 2D material; (c) twist angle and Moiré fringe; (d) DBR microcavity; (e) grating cavity; (f) defect photonic crystal
    Interactions of exciton-photon. (a) Temperature-dependent photoluminescence (PL) spectra[52]; (b) multi-peak Lorentzian fitting of the PL spectra at temperature of 95 K[52]; (c) interaction strengths obtained experimentally (dot) and theoretically (solid line) at different temperatures[52]; (d) schematic diagram of the valley-polarized exciton-polaritons of TMDs in a microcavity[53]; (e) dispersion relation of exciton-polaritons[53]; (f) structure of the nanobeam cavity and the electric field distribution of cavity mode M1[54]; (g) magneto PL spectra recorded at a low excitation power and the intensity of exciton-photon coupling given by the relationship between the linewidth and the detuning[54]
    Interactions of exciton-phonon. (a) Temperature-dependent cavity-coupled PL spectra of monolayer WSe2, from top to bottom is 320, 240, 160 K, and 80 K, respectively[62]; (b) calculated vibrational modes of the nanobeam cavity[63]; (c) TN dependence of gX0,2LA in cavities[63]; (d) schematic diagram of the exciton-phonon-phonon coupling[63]
    Interactions of exciton-magnon. (a) Relationship between the relative spin alignment and the exciton resonance energy in CrSBr[69]; (b) reflectance and transient reflectance spectra of CrSBr[67]; (c) schematic diagrams of the bright (B) and dark (D) modes[69]; (d) magnon dispersion of CrSBr obtained by Fourier transform of the ultrafast spectral data[69]; (e) calculated exciton resonance energy shift during the precession of the optical and acoustic magnon modes[69]
    Electric field control of 2D materials. (a) Optical image of WSe2 device[72]; (b) schematic diagram of a monolayer WSe2 device[72]; (c) PL spectrum of monolayer WSe2[72]; (d) schematic diagram of a bilayer MoS2 device encapsulated in hBN[73]; (e) schematic diagram of the coexistence of IXs and phonons[73]; (f) schematic diagram of the variation in emission energies of IX1 and IX2 from the PL spectrum of bilayer MoS2 with electric field, illustration is schematic diagram of IXs configurations in real space[73]; (g) schematic diagram of the first-order derivative for Raman intensity with respect to phonon frequency[73]
    Magnetic field control of 2D materials. (a) Reflection spectrum of monolayer WS2 at 0 T and 4 K, along with the normalized reflection spectra of A and B excitons under σ+ polarized light[74]; (b) variation in the magneto-optical Kerr rotation angle with magnetic field for CrI3 with different layer numbers, illustration is structural diagram of CrI3 and its Ising-type spin orientation[65]; (c) schematic diagram of the CrSBr crystal and its magnetic structure[75]; (d) PL spectra of bilayer CrSBr with the magnetic field direction along the b-axis[75]; (e) PL spectra of bilayer CrSBr with the magnetic field direction along the c-axis[75]
    Optimization and regulation of micro-nano photonic cavities. (a) Resonant spectra of microcavities with various shifts of air rods at defects and their SEM pictures, illustration is the resonant spectrum of the microcavity measured over a wide wavelength range with 0.15a shift[76]; (b) variation in estimated Q/V values with shift of air rods[76]; (c) schematic diagram of monolayer WSe2 integrated with L3-type photonic crystal[77]; (d) schematic diagram of bilayer MoS2/WSe2 heterobilayers integrated with photonic crystal[78]
    Schematic diagrams of multi-cavity coupling. (a) Theoretical curves of the energies and Q values of the split fundamental modes of parallel L3 cavities coupled along different directions[81]; (b) schematic diagram of the homoatomic PMs[82]; (c) schematic diagram of the heteroatomic PMs[82]; (d) bare frequency, frequency-dependent coupling strength, and eigenfrequency of the PMs when homoatomic PMs is coupled[82]; (e) bare frequency,eigenfrequency at the diabolical point between weak and strong coupling, and eigenfrequency of the PMs when heteroatomic PMs is coupled[82]
    • Table 1. Bandgaps of several typical 2D materials

      View table

      Table 1. Bandgaps of several typical 2D materials

      Type of 2D materialBandgap-bulk /eVBandgap-monolayer /eVBandgap-monolayer /nm
      Graphene~0~0(Terahertz & microwave)
      TiS31.01.21033 (infrared)
      2H-MoS21.31.8689 (visible)
      hBN4.06.0207 (ultraviolet)
    Tools

    Get Citation

    Copy Citation Text

    Yuhang Li, Xiulai Xu, Chenjiang Qian. 2D Material-Micro/Nano-Photonic Cavity Coupling Quantum Systems and Their Control in Multiple Degrees of Freedom (Invited)[J]. Laser & Optoelectronics Progress, 2025, 62(11): 1127005

    Download Citation

    EndNote(RIS)BibTexPlain Text
    Save article for my favorites
    Paper Information

    Category: Quantum Optics

    Received: Feb. 27, 2025

    Accepted: Apr. 7, 2025

    Published Online: May. 26, 2025

    The Author Email: Xiulai Xu (xlxu@pku.edu.cn), Chenjiang Qian (chenjiang.qian@iphy.ac.cn)

    DOI:10.3788/LOP250712

    CSTR:32186.14.LOP250712

    Topics