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Laser & Optoelectronics Progress, Volume. 61, Issue 5, 0530001(2024)

Terahertz Spectral Anharmonicity of ANPZ Under Heating

Chai Xie1, Yongwei Duan1, Quancheng Liu1、*, Hu Deng1,2, Qi Zhang3, Zhixiang Wu1, Wenqing Wei1,2, and Liping Shang1,2、**
Author Affiliations
  • 1School of Information Engineering, Southwest University of Science and Technology, Mianyang 621010, Sichuan , China
  • 2Tianfu Institute of Research and Innovation, Southwest University of Science and Technology, Chengdu 610299, Sichuan , China
  • 3Institute of Chemical Materials, Chinese Academy of Engineering Physics, Mianyang 621900, Sichuan , China
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    AbstractGet PDF(in Chinese)
    Figures&Tables (8)
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    References (17)
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    Figures & Tables(8)
    The unit cell of ANPZ

    Fig. 1. The unit cell of ANPZ

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    Terahertz absorption spectra of ANPZ under heating

    Fig. 2. Terahertz absorption spectra of ANPZ under heating

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    Comparison of experimental and theoretical calculated spectra of ANPZ

    Fig. 3. Comparison of experimental and theoretical calculated spectra of ANPZ

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    Vibration displacement vectors at 1.16 THz and 1.91 THz (arrow represents vector)

    Fig. 4. Vibration displacement vectors at 1.16 THz and 1.91 THz (arrow represents vector)

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    Decomposition of intramolecular and intermolecular vibration of two modes

    Fig. 5. Decomposition of intramolecular and intermolecular vibration of two modes

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    Calculation of the intramolecular vibrational contribution of each atom of two modes

    Fig. 6. Calculation of the intramolecular vibrational contribution of each atom of two modes

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    Hydrogen bond network of ANPZ (dotted line indicates hydrogen bond)

    Fig. 7. Hydrogen bond network of ANPZ (dotted line indicates hydrogen bond)

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    Anisotropic displacements of atoms over a temperature range of 23‒260 °C

    Fig. 8. Anisotropic displacements of atoms over a temperature range of 23‒260 °C

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    Chai Xie, Yongwei Duan, Quancheng Liu, Hu Deng, Qi Zhang, Zhixiang Wu, Wenqing Wei, Liping Shang. Terahertz Spectral Anharmonicity of ANPZ Under Heating[J]. Laser & Optoelectronics Progress, 2024, 61(5): 0530001

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    Paper Information

    Category: Spectroscopy

    Received: Mar. 13, 2023

    Accepted: Apr. 7, 2023

    Published Online: Mar. 5, 2024

    The Author Email: Quancheng Liu (Liuquancheng@swust.edu.cn), Liping Shang (shangliping@swust.edu.cn)

    DOI:10.3788/LOP230848

    CSTR:32186.14.LOP230848

    Topics

    laser devices and laser physics
    Lasers and Laser Optics
    Laser physics
    laser manufacturing
    Instrumentation, Measurement and Metrology