Chinese Journal of Lasers, Volume. 50, Issue 24, 2402101(2023)

Femtosecond Time‑Resolved Electronic States in Femtosecond Laser Multipulse Ablation

Qianhao Wang1,2, Hualong Zhao1、*, Xiaojun Yang1, Wenlong Wen1, and Yi Li1,2
Author Affiliations
  • 1Photonic Manufacturing System and Application Research Center, Xi’an Institute of Optics and Precision Mechanics, Chinese Academy of Sciences, Xi’an 710119, Shaanxi, China
  • 2University of Chinese Academy of Sciences, Beijing 100049, China
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    Figures & Tables(17)
    Pump-probe shadow imaging device
    Air plasma at the material surface
    Propagation of Gaussian beam when the focus is 100 μm inside the material
    Effects of the microstructure formed by the first 219 pulses irradiating the material on propagation and ionization of subsequent individual pulses when the focus is on the quartz surface. (a) 20×, NA=0.4; (b) 40×, NA=0.6
    Propagation of the 220th pulse when the focusing condition is 20× and the focal point is at the quartz surface
    Propagation of the 220th pulse when the focusing condition is 20× and the focal point is 100 μm inside the quartz
    Color number density distribution of free electrons. (a) Focal point is at the quartz surface; (b) focal point is 100 μm inside the quartz
    Time distribution of maximum electron number density when the focusing condition is 20×. (a) Focal point is at the quartz surface; (b) focal point is 100 μm inside the quartz
    Shaded diagrams of the propagation process of the 220th pulse when focusing condition is 40× and the focal point is at the quartz surface
    Shaded diagrams of the propagation process of the 220th pulse when focusing condition is 40× and the focal point is 100 μm inside the quartz
    Variation of maximum electron number density with time when the focusing condition is 40×. (a) Focal point is at the quartz surface; (b) focal point is 100 μm inside the quartz
    Propagation and ionization of the pulse when the focus is different locations (20× focus). (a) Propagation and ionization images of the pulse at 498 fs; (b) crater morphology formed by the first 220 pulses
    Propagation and ionization of the pulse when the focus is different locations (40× focus). (a) Propagation and ionization images of the pulse at 498 fs; (b) crater morphology formed by the first 220 pulses
    Common process problems and transient ionization images in processing V-shaped microstructures. (a) Microcracking problem in processing sapphire V-shaped structures; (b) induced streak problem in processing SiO2
    Common process problems and transient ionization images in processing inverted trapezoidal microstructures. (a) Cracking problem in processing diamond inverted trapezoidal structures; (b) fragmentation problem in processing SiC inverted trapezoidal structures
    • Table 1. Power density on material surface under different conditions

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      Table 1. Power density on material surface under different conditions

      Focusing conditionFocusing positionPower density /(W·cm-3
      20×,NA=0.4Surface(0 μm)2.3×1015
      20×,NA=0.4+100 μm2×1012
      40×,NA=0.6Surface(0 μm)5.1×1015
      40×,NA=0.6+100 μm9.04×1011
    • Table 2. Comparison of relaxation time of maximum electron number density under different focusing conditions

      View table

      Table 2. Comparison of relaxation time of maximum electron number density under different focusing conditions

      Focusing conditionFocusing positionFWHM /fs

      Pulse

      width /fs

      20×,NA=0.4Surface125290
      20×,NA=0.4100 μm250290
      40×,NA=0.6Surface200290
      40×,NA=0.6100 μm125290
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    Qianhao Wang, Hualong Zhao, Xiaojun Yang, Wenlong Wen, Yi Li. Femtosecond Time‑Resolved Electronic States in Femtosecond Laser Multipulse Ablation[J]. Chinese Journal of Lasers, 2023, 50(24): 2402101

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    Paper Information

    Category: Laser Forming Manufacturing

    Received: May. 16, 2023

    Accepted: Aug. 1, 2023

    Published Online: Dec. 7, 2023

    The Author Email: Zhao Hualong (281731466@qq.com)

    DOI:10.3788/CJL230834

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