Chinese Journal of Liquid Crystals and Displays, Volume. 40, Issue 8, 1115(2025)

Siloxane-side-chain-induced vertical phase separation in polymer blends for stretchable organic transistors

Runfang JIANG and Longzhen QIU*
Author Affiliations
  • Anhui Industrial Innovation Research Institute of Advanced Optoelectronic Materials and Systems, Anhui Province Key Laboratory of Measuring Theory and Precision Instrument, School of Instrument Science and Optoelectronic Engineering, Hefei University of Technology, Hefei 230009, China
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    Conventional conjugated polymers face the critical challenge of achieving simultaneous optimization of electrical and mechanical properties. This study focuses on siloxane-side-chain-functionalized diketopyrrolopyrrole (DPP)-based conjugated polymer (DPP-4Si) blended with hydrogenated styrene-butadiene block copolymer (SEBS). Through precise control of film preparation and microphase separation structures, we developed high-performance elastic semiconductor films with a maximum mobility of 1.08 cm2·V-1·s-1. Fully stretchable transistors fabricated using the optimal blend ratio demonstrated remarkable electromechanical stability, maintaining over 72% current retention even under 100% tensile strain, showcasing exceptional stretchability.

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    Runfang JIANG, Longzhen QIU. Siloxane-side-chain-induced vertical phase separation in polymer blends for stretchable organic transistors[J]. Chinese Journal of Liquid Crystals and Displays, 2025, 40(8): 1115

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    Paper Information

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    Received: Jun. 4, 2025

    Accepted: --

    Published Online: Sep. 25, 2025

    The Author Email: Longzhen QIU (lzhqiu@hfut.edu.cn)

    DOI:10.37188/CJLCD.2025-0112

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