Acta Optica Sinica, Volume. 45, Issue 10, 1019001(2025)

Spatial Self-Phase Modulation and Nonlinear Optical Devices Based on PDMS/WS2

Qifan Li1, Zexin Cui2, Lihua Tong1, Mengting Jiang1, Guangyuan Cui1, Churui Guo1, and Xiaodan Xu1、*
Author Affiliations
  • 1Hebei Key Laboratory of Microstructural Material Physics, School of Science, Yanshan University, Qinhuangdao 066004, Shandong , China
  • 2School of Physics, Beijing Institute of Technology, Beijing 100081, China
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    Figures & Tables(6)
    Sample preparation and physical property characterization. (a) Preparation process of PDMS/WS2; (b) absorption spectra of PDMS/WS2 and PDMS; (c) Raman spectrum of WS2 crystal powder
    SSPM effect of PDMS/WS2. (a) Optical path diagram of SSPM experiment for PDMS/WS2; (b) diffraction ring patterns of PDMS/WS2 under different incident intensities and wavelengths; (c) variation of the number of diffraction rings of PDMS/WS2 with the incident intensity; (d) SSPM effect of PDMS at different wavelengths
    Stability analysis of PDMS/WS2 diffraction rings. (a) Comparison of diffraction ring for PDMS/WS2 and NMP/WS2; (b) variation of diffraction ring of PDMS/WS2 and NMP/WS2 over time; (c) relative variation of nonlinear refractive index of PDMS/WS2 and NMP/WS2 with light intensity; (d) diffraction ring patterns of PDMS/WS2 under the condition of wavelength of 473 nm and a light intensity of 16.28 W/cm²; (e) intensity value extracted along the dashed X-axis in Fig. 3(d); (f) intensity value extracted along the dashed Y-axis in Fig. 3(d)
    All-optical switch based on PDMS/WS2. (a) Schematic diagram of the experimental setup for the all-optical switch; (b) diffraction patterns of PDMS/WS2 as the pump light intensity increases; (c) linear relationship between the number of diffraction rings and total light intensity under 473 nm controlling 532 nm; (d) linear relationship between the number of diffraction rings and total light intensity under 532 nm controlling 473 nm
    All-optical diode based on PDMS/WS2. (a) Forward-biased of the all-optical diode; (b) backward-biased of the all-optical diode; (c) variation of the diffraction rings of SSPM based on PDMS for forward and backward configurations with light intensity; (d) relationship between the number of diffraction rings and light intensity for forward-biased and backward-biased conditions
    • Table 1. Nonlinear optical parameters of PDMS/WS2 under different wavelengths

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      Table 1. Nonlinear optical parameters of PDMS/WS2 under different wavelengths

      λ /nmdN/dI /(cm2/W)n2 /(cm2/W)χtotal(3) /e.s.u.χmonolayer(3) /e.s.u.
      4050.766210.946×10-55.512×10-32.849×10-9
      4730.622610.443×10-55.259×10-32.718×10-9
      5320.47268.916×10-54.490×10-32.321×10-9
      7210.15043.845×10-51.936×10-31.001×10-9
      9140.10693.465×10-51.745×10-39.019×10-10
      10640.07452.811×10-51.416×10-37.318×10-10
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    Qifan Li, Zexin Cui, Lihua Tong, Mengting Jiang, Guangyuan Cui, Churui Guo, Xiaodan Xu. Spatial Self-Phase Modulation and Nonlinear Optical Devices Based on PDMS/WS2[J]. Acta Optica Sinica, 2025, 45(10): 1019001

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    Paper Information

    Category: Nonlinear Optics

    Received: Dec. 26, 2024

    Accepted: Mar. 4, 2025

    Published Online: May. 19, 2025

    The Author Email: Xiaodan Xu (xxd@ysu.edu.cn)

    DOI:10.3788/AOS241942

    CSTR:32393.14.AOS241942

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