Acta Optica Sinica, Volume. 45, Issue 2, 0200002(2025)

Key Technologies and Applications of Ultrasensitive and Rapid Quartz-Enhanced Photoacoustic Sensing (Invited)

Lei Dong1,2、*, Wenfei Han1,2, Hongpeng Wu1,2, Weiguang Ma1,2, Lei Zhang1,2, Wangbao Yin1,2, and Suotang Jia1,2
Author Affiliations
  • 1State Key Laboratory of Quantum Optics and Quantum Optics Devices, Institute of Laser Spectroscopy, Shanxi University, Taiyuan 030006, Shanxi , China
  • 2Collaborative Innovation Center of Extreme Optics, Shanxi University, Taiyuan 030006, Shanxi , China
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    Figures & Tables(15)
    QTF assembled with acoustic micro-resonator[37]
    Resonance diagrams of sound wave in segmented resonator[37]. (a) Acoustic intensity distribution when segmented resonator is strongly coupled and approximated as single tube; (b) acoustic intensity distribution when segmented resonator is no acoustic coupling; (c) acoustic intensity distribution when acoustic coupling occurs between QTF and segmented resonator
    Gain of signal-to-noise ratio (SNR) of micro-resonator with respect to bare QTF[37] (length, inner diameter, and outer diameter of micro-resonator are 4.4 mm, 0.6 mm, and 0.9 mm, with 50 µm gap between tube facet and QTF surface)
    Variations of signal amplitude, quality factor, and signal-to-noise ratio of QEPAS system with distance yt between top of acoustic micro-resonator and top of QTF[45]. (a) Detected signal amplitude of QEPAS system; (b) quality factor of QEPAS system; (c) signal-to-noise ratio of QEPAS system
    Schematic of QEPAS system based on double-tube acoustic micro-resonator[46]
    On-beam single-tube acoustic micro-resonator[48]. (a) Assembly of on-beam single-tube acoustic micro-resonator; (b)‒(d) geometric parameters of on-beam single-tube acoustic micro-resonator
    Photograph of custom-made tuning fork[60]
    Illustrations of QTF arm deformations under different vibration modes[71]. (a) Fundamental flexural mode; (b) first overtone flexural mode; (c) combined fundamental and first overtone flexural modes
    Simultaneous dual gas (C2H2 and H2O) measurements using QEPAS sensor based on combined vibration motion of QTF[71]
    Simultaneous dual gas continuous monitoring of H2O (fundamental channel) and CH4 (1st overtone channel)[73]
    Setup of simultaneous dual gas measurement using double-tube resonators[74]
    Continuous measurement results of volume fraction of atmospheric CH4 near Hou Village Landfill in Taiyuan, China on October 11, 2018[73]
    Seven-day CO volume fraction at Shanxi University, China[63]. (a) Measured data by CO sensor based on grooved QTF; (b) corresponding data available from nearby station of the Department of Ecology and Environment of Shanxi Province
    • Table 1. Performance comparison of different QEPAS phonometer configurations

      View table

      Table 1. Performance comparison of different QEPAS phonometer configurations

      ConfigurationChannelInner diameter /mmOuter diameter /mmLength /mmResonance frequency /HzQCalculated response time /msMeaured response time /ms
      Double AmR #1Top0.600.904.4328415945.85.0
      Bottom0.600.904.4
      Double AmR #2Top0.841.244.032747189018.418.1
      Bottom0.841.244.0
      Single AmR #10.600.94.432742410940.042.3
      Single AmR #20.841.244.032758216021.020.1
      Bare QTF3275213466130.9136.3
    • Table 2. Detection limits of BF-QEPAS sensor bsased on three different kinds of semiconductor lasers

      View table

      Table 2. Detection limits of BF-QEPAS sensor bsased on three different kinds of semiconductor lasers

      Laser typeFrequency /cm-1Gas typeTechniquePressure /TorrIntegration time /msft /Hzf0 /HzQt/Q0NEC /10-6

      NNEA /

      (cm-1·W·Hz-1/2

      DFB-DL7306.75H2OQEPAS760300.0--0.4101.50×10-8
      BF-QEPAS0.13276032760184818460.0592.45×10-9
      DFB-QCL2190.02COQEPAS700300.0--0.0112.40×10-8
      BF-QEPAS3.03275532755185118460.0102.30×10-8
      DFB-ICL2778.64CH4QEPAS700300.0--55.5701.81×10-8
      BF-QEPAS3.032757327571817182340.7501.30×10-8
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    Lei Dong, Wenfei Han, Hongpeng Wu, Weiguang Ma, Lei Zhang, Wangbao Yin, Suotang Jia. Key Technologies and Applications of Ultrasensitive and Rapid Quartz-Enhanced Photoacoustic Sensing (Invited)[J]. Acta Optica Sinica, 2025, 45(2): 0200002

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    Paper Information

    Category: Reviews

    Received: Jul. 5, 2024

    Accepted: Aug. 15, 2024

    Published Online: Jan. 22, 2025

    The Author Email: Lei Dong (donglei@sxu.edu.cn)

    DOI:10.3788/AOS241259

    CSTR:32393.14.AOS241259

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