ObjectivePhotodetectors, as multifunctional devices and critical components of photoelectric detection technology, play a pivotal role in converting optical signals into electrical signals within photoelectric systems. Their applications span diverse fields, including infrared detection and night-vision equipment in defense technology, visible-light detection in consumer cameras, and optical communication satellites, demonstrating significant practical value and broad prospects. However, the growing demand for miniaturized, broadband, and polarization-sensitive photodetectors poses new challenges, particularly in developing multifunctional devices capable of room-temperature operation, wide-spectrum response, and polarized-light detection. Sb
2Te
3, an emerging topological insulator material, offers novel opportunities to address these challenges due to its unique optical and electronic properties. Meanwhile, ReS
2 exhibits anisotropic optoelectronic behavior and a stable bandgap, making it promising for polarization-sensitive photodetection. By leveraging these two materials, a multifunctional photodetector was developed, exhibiting room-temperature operation, broadband response, and polarization-sensitive characteristics.
MethodsThe heterojunction device was fabricated through a dry transfer process, comprising three key steps: mechanical exfoliation, material transfer, and metal electrode preparation. The Sb
2Te
3/ReS
2 heterostructure-based optoelectronic device was obtained. Raman spectroscopy, Atomic Force Microscopy (AFM), a low-temperature probe station, a semiconductor analyzer, and lasers with various single wavelengths were utilized to characterize the microscopic morphology and optoelectronic properties of the device.
Results and DiscussionsAFM and Raman spectroscopy confirmed the formation of a high-quality heterointerface, with ReS
2 and Sb
2Te
3 layer thicknesses of 20 nm and 50 nm, respectively. Transfer curves tests of individual materials revealed P-type (Sb
2Te
3) and N-type (ReS
2) behavior, indicating efficient charge separation at the heterojunction. The device exhibited a c broad spectral response from 400 nm to
1550 nm with low dark current. Under 532 nm laser illumination, the responsivity reached 0.27 A/W, with a specific detectivity (
D*) of 5.1×10
9 Jones(1 Jones = 1
$\mathrm{cm} \cdot \sqrt{\mathrm{Hz}} / \mathrm{W} $) and an external quantum efficiency (EQE) of 61.6%. Rise/fall times were 8/10 ms for 650 nm illumination and 27/27 ms for
1550 nm illumination. Stability tests under 10 Hz pulsed 532 nm laser cycling for 220 seconds showed no performance degradation. Polarization-sensitive measurements yielded a dichroic ratio of 1.3 at 650 nm.
ConclusionsThe Sb
2Te
3/ReS
2 van der Waals heterostructure demonstrates exceptional room-temperature photodetection performance across visible to near-infrared wavelengths, coupled with polarization sensitivity. This work highlights the potential of integrating topological insulators with anisotropic 2D materials for multifunctional optoelectronic devices, offering a promising pathway toward advanced broadband and polarization-resolved sensing technologies.