Chinese Journal of Lasers, Volume. 17, Issue 12, 1803(2005)
Compensation for effect of third-order nonlinearity on second harmonic generation of ultrashort pulses
The effect of third-order nonlinearity on the second harmonic generation of ultrashort pulses in KDP crystal is analyzed theoretically.It is found that the influence of third-order nonlinearity on conversion efficiency becomes dominant when the incident intensity is above 100 GW/cm~2.A novel approach in which an initial phase-mismatch is introduced to compensate for third-order nonlinearity effect is proposed.The calculated results show that for a 50 fs pulse and a 250 GW/cm~2 input intensity,the conversion efficiency is increased by a factor of 1.1 at the condition of 0.9 mrad initial phase-mismatching angle.At the same time,the fluence modulation of the fundamental and second harmonic pulses due to third-order nonlinearity is suppressed effectively and the temporal profiles are improved.
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HAN Wei, ZHENG Wan-guo, ZHU Qi-hua. Compensation for effect of third-order nonlinearity on second harmonic generation of ultrashort pulses[J]. Chinese Journal of Lasers, 2005, 17(12): 1803
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Received: Jun. 1, 2005
Accepted: --
Published Online: Jan. 25, 2021
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CSTR:32186.14.