In recent years, artificially engineered metasurfaces, which can effectively manipulate the polarization, amplitude, and phase of electromagnetic waves on the two-dimensional (2D) scale, have attracted more and more attention^[1–3]. Compared with conventional optical devices dependent on phase accumulation, metasurfaces can obtain abrupt phase change within subwavelength thickness by appropriately changing specific parameters, thereby generating various functions^[4,5]. Specifically, metasurfaces can generate spatial phase discontinuities over the entire 2π range of a specific frequency, which have manifested that they can be utilized in a flat wave plate^[6,7], hologram imaging^[8–10], beam deflectors^[11,12], achromatic focusing lenses^[13,14], spin-orbital angular momentum manipulation^[15–18], and other fields.

Pancharatnam–Berry (PB) phase, also called geometric phase, has been proposed to achieve phase-wavefront manipulation of circularly polarized (CP) waves^[19,20]. However, the output waves of PB phase metasurfaces under orthogonal CP waves have inherent correlation. To break this restriction, spin-decoupled metasurfaces combining PB phase with dynamic phase were designed to independently manipulate the output waves under left-handed CP (LCP) and right-handed CP (RCP) incidences^{[12,18,21,22]}. Spin-decoupled metasurfaces have many applications in holography^[21], focusing^[18], and polarization multiplexing^[22].

It is worth noting that the above-mentioned metasurfaces all have the properties of a half-wave plate, so the wavefront phase manipulation is only achieved for cross-polarized waves. Once the metasurface no longer has the properties of a half-wave plate, the outgoing wave will exist with LCP and RCP components under CP incidence, meaning that it makes sense to independently manipulate cross and co-polarization. Recently, phase-modulated metasurfaces, which can realize the independent manipulation of co- and cross-polarized output waves under CP incidence, have been reported^[23–25]. In this paper, a metasurface composed of meta-atoms with a phase difference of 2π/3 between linear orthogonal polarizations is introduced to generate LCP and RCP waves with different amplitudes under CP wave incidence so as to be superimposed into a specific elliptically polarized (EP) wave (see Fig. 1). As shown in Fig. 1(b), the metasurface composed of meta-atoms with a phase difference of 2π/3 and a phase difference of π/3 according to certain rules can generate focused linearly polarized (LP) (CP) exit waves under CP (LP) incidence. The demonstration of specific polarization conversion and multiplexing achieved at the all-silicon metasurfaces opens new ways to polarize metasurfaces with full potentials and can be hopefully further extended to other frequency regimes.

Here, we demonstrate the feasibility of the concept through the derivation of the Jones matrix: J(θ)=[cosθ−sinθsinθcosθ][|txx|eiφxx00|tyy|eiφyy][cosθsinθ−sinθcosθ],(1)where θ is the angle at which the meta-atom rotates counterclockwise around the +z direction, which originates from the rotation matrix [cosθsinθ−sinθcosθ], φxx,φyy,|txx|, and |tyy| represent corresponding phase delays and amplitudes along the x and y axis under x and y LP incidences. It is supposed that |txx|=|tyy| and the phase difference along x and y axes Δφ is equal to φxx−φyy. Besides, the summation of propagation phase is expressed as ∑φ=φxx+φyy.

For input with the RCP state as |R〉=[1i], the exit field can be described as^[25]$$\begin{gathered} J(θ)·|R〉=sin(12Δφ)·ei(12∑φ−π2+2θ)|L〉 \\ +cos(12Δφ)·ei12∑φ|R〉. \end{gathered}$$(2)

Similarly, for the incident LCP wave (|L〉=[1−i]), the electric field of the transmitted wave generated is $$\begin{gathered} J(θ)·|L〉=sin(12Δφ)·ei(12∑φ−π2−2θ)|R〉 \\ +cos(12Δφ)·ei12∑φ|L〉. \end{gathered}$$(3)

Surprisingly, Eqs. (2) and (3) indicate that the transmitted waves both exist with LCP and RCP components under LCP or RCP incidence. Moreover, under CP incidence, the amplitudes of the co- and cross-polarized components of the transmitted wave are cos(Δφ/2) and sin(Δφ/2), respectively.

Once it is guaranteed that the rotation angle θ is equal throughout to π/4, then Eqs. (2) and (3) can be respectively simplified as J(θ)·|R〉=[sin(12Δφ)·|L〉+cos(12Δφ)·|R〉]·ei12∑φ,(4)J(θ)·|L〉=[−sin(12Δφ)·|R〉+cos(12Δφ)·|L〉]·ei12∑φ.(5)

It can be readily seen from Eqs. (4) and (5) that by adjusting the phase difference Δφ, the desired EP exit wave can be obtained under the CP illumination.

In order to verify the feasibility of the above concept, we apply the anisotropic all-silicon meta-atoms A [permittivity ε=11.9, see Fig. 2(a)] with the phase difference Δφ=2π/3 as the basic elements for the metasurface construction. The thickness of the substrate is h2=300μm with a period of P=150μm. By rotating the silicon pillar with height h1=200μm, width W, and length L, the rotation angle is 45° to the y axis, and then the final structure is formed. CST MICROWAVE STUDIO (2019) is exploited to simulate the transmission phase shifts and amplitudes of meta-atoms A. The simulated phase shift and amplitude of the exit wave under x–LP illumination at 0.95 THz are shown in Figs. 2(b) and 2(c) (here, the angle between the rectangular silicon pillar and the x axis is 0°). Figures 2(d) and 2(e) depict the corresponding phase shift and amplitude under y–LP incidence. It is worth noting that a phase variation of 2π can be generated regardless of whether the incident wave is x LP or y LP, which is crucial for metasurfaces design. After a quite careful selection, six types of meta-atoms A [see Fig. 2(a) for specific parameters] are utilized for metasurface design. Figure 2(f) presents phase delays φxx and φyy of transmission waves under x–LP or y–LP incidence; meanwhile, the corresponding amplitudes of the cross and co-components under CP incidence are shown in Fig. 2(g). Obviously, the phase variation of 2π is well covered by meta-atoms A. It can be seen from Fig. 2(g) that the amplitudes of cross and co-polarizations of the meta-atoms A are consistent with the expected concepts, which can be exploited to construct a metasurface that can generate ellipsoidal polarization under LP or CP incidence. By this time, according to Eq. (4), it can be found that when the RCP wave is incident, the transmitted wave can be expressed as [3+1(1−3)i]. In addition, the exit EP wave can be described as [1−3−(3+1)i] under LCP incidence. After theoretical calculations, we can also conclude that the generated EP wave can be described as [1−3i]([3i]) under x–LP (y–LP) incidence.

Next, we design a metasurface composed of the meta-atoms A [see Fig. 2(a)] that meet a specific phase distribution, which can generate focused EP waves under LP or CP incidences, to demonstrate the hypothesis. To realize the beam focusing, the phase distribution of the meta-atoms A needs to meet the following conditions: φ=12∑φ=−2πλ(f2+r2−f),(6)where λ is the incident wavelength corresponding to 0.95 THz, f=4.8mm stands for focal length, and r represents the distance from any point on the metasurface to the center of its circle.

The results of polarization conversion and focusing generated by the metasurface under the incidence of different polarized waves are obtained through simulation, as shown in Fig. 3. To more intuitively verify that the metasurface can generate specific EP waves under different polarized waves, the simulated results of its orthogonally polarized waves are also displayed here. It is noted that the intensity of the EP wave ([3+1(1−3)i]) is concentrated in a certain place in space, while the intensity of its orthogonally polarized wave ([3−1(3+1)i]) is negligible [see Fig. 3(a)]. Figures 2(b)–2(d) show the simulated results under LCP, x–LP, and y–LP incidences, which are consistent with the results obtained by the above calculations. Furthermore, comparing the simulation results of LCP and RCP incidence, it is not difficult to find that under the incidence of orthogonal CP waves, the EP waves generated by the metasurface are also orthogonal, similar to the case under the orthogonal LP incidences. In short, through setting a specific phase difference Δφ, the expected EP waves can be generated under the incidence of different polarized waves.

We consider introducing another kind of meta-atoms (called meta-atoms B) to form a new metasurface together with the meta-atoms A, realizing the mutual polarization conversion between linear polarization and circular polarization. For RCP incidence, the meta-atoms B with the phase difference Δφ1=π−Δφ will bring about an EP wave that can be described as $$\begin{gathered} J(θ)·|R〉=[sin(12Δφ1)·|L〉+cos(12Δφ1)·|R〉]·ei12∑φ1 \\ =[cos(12Δφ)·|L〉+sin(12Δφ)·|R〉]·ei12∑φ1, \end{gathered}$$(7)where ∑φ1 is the summation of propagation phase along the x and y directions. Once ∑φ and ∑φ1 in Eqs. (4) and (7) remain equal, the superposition of the two meta-atoms with phase differences of Δφ and Δφ1 can generate x–LP waves under RCP incidence. Besides, under LCP illumination, EP waves generated by the meta-atom with the phase difference Δφ1 are J(θ)·|L〉=[−cos(12Δφ)·|R〉+sin(12Δφ)·|L〉]·ei12∑φ1.(8)

Obviously, the above scheme can also generate y−LP waves under the incidence of LCP waves. After further derivation, it can be found that this polarization multiplexing method can effectively achieve the polarization conversion between linear polarization and circular polarization.

With the proposed scheme, the six meta-atoms B with a phase difference of π/3 are carefully selected, with parameters shown in Fig. 4. Comparing Fig. 2(f) with Fig. 4(a), it can be seen that the difference between the phase delay φxx of the meta-atom A and the phase delay φxx′ of the meta-atom B is π/6. Substituting the phase difference Δφ1=π/3 into Eqs. (7) and (8), we can get the following conclusion: when RCP, LCP, x−LP and y−LP waves are incident on the meta-atom B, the polarized waves generated are [3+1(3−1)i], [3−1(−3−1)i], [3−i], and [13i], respectively.

Then, we introduce the way of spatial interleaving to arrange the meta-atoms A and B, so as to construct a metasurface with the function of polarization multiplexing. For the meta-atoms A, the phase distribution satisfies Eq. (6), and the frequency of incident wave and focal length are 0.95 THz and 4.8 mm, respectively. Similarly, considering a focused polarized wave generated by meta-atoms B with a specific phase arrangement, the corresponding phase distribution is φ1=12∑φ1=−2πλ[f12+(x−x1)2+(y−y1)2−f1]+π6,(9)where x1=−75μm, y1=75μm, f1=4.8mm, and (x1,y1,f1) represents the focal point of the transmitted wave. Meanwhile, to obtain the polarization multiplexing metasurface [see Fig. 4(b)] we designed, the meta-atoms B, whose phase distribution satisfies Eq. (9) by 75 µm along the positive x direction and 75 µm along the negative y direction, are translated. It is worth noting that the use of such a spatial interleaving method needs to ensure that there is no overlap between the meta-atoms A and B. Figures 4(c) and 4(d), respectively, show the intensity distribution of the two EP components on the xz plane under RCP incidence, implying that the outgoing wave generated by the metasurface will be focused on a certain point. In order to further describe the characteristics of the outgoing wave, Fig. 4(e) depicts the intensity profile of the corresponding outgoing wave on the focal plane. It can be seen that the EP waves generated by the meta-atoms A and B are superimposed on the focal plane to generate x−LP waves.

Next, we discuss the transmission results of the metasurface under LCP, x−LP, and y−LP incidences. Figure 5(a) exhibits the intensity distributions of the expected polarization and corresponding orthogonal polarization on the focal plane when the incident wave is LCP. The simulated results indicate that the metasurface composed of meta-atoms A and B can generate focused y−LP waves under LCP incidence. Figures 5(b) and 5(c) illustrate the simulated results of CP waves under x−LP and y−LP waves, respectively. In this part, the proposed metasurface with polarization multiplexing can generate CP (LP) waves under LP (CP) incidences, proving the feasibility of such design.

We present an all-silicon metasurface composed of meta-atoms A with the phase difference of 2π/3 along the x and y directions to generate specific EP waves under different polarized waves. For instance, when an RCP wave is incident, the metasurface will generate LCP and RCP waves with the same phase but different amplitudes, and then they are superimposed to engender EP waves. Furthermore, we introduce meta-atoms B with a phase difference of π/3 and meta-atoms A to construct a metasurface that can realize bidirectional polarization conversion between linear polarization and circular polarization. The simulated results are in good agreement with the deduced results, verifying the good performance of our design concepts. We envisage that such an approach may spur a new wave of photonics devices and can effectively extend the polarization multiplexing metasurfaces to a broader range.