A section of graphene film is transferred on the tapered fiber and the light interacts with graphene by the evanescent field so as to generate the mode-locked pulse. When the pump power is transferred to the threshold of 230 mW, the self-staring mode-locked pulse can be realized. Fixing the pump power at 300 mW, soliton bundles with controlled 2-6 sub-pulses are generated by adjusting the polarization controller. Fixing the pump power at 450 mW, different order harmonic mode-locked pulses can be achieved by adjusting the polarization controller. The highest order of harmonic mode-locked pulse is 117, and the corresponding pulse repetition frequency is 2.412 GHz.