1Nanophotonic Research Centre, Institute of Microscale Optoelectronics & State Key Laboratory of Radio Frequency Heterogeneous Integration, Shenzhen University, Shenzhen 518060, China
Optical topological quasiparticles with nontrivial topological textures, such as skyrmions and meron lattices, have attracted considerable attention due to their potential applications in high-dimensional optical data storage and communications. Most previous studies of optical topological quasiparticles have focused on the formation of topological structures in isotropic media, whereas in our work, we perform a comprehensive investigation into the formation, topological stability, and phase transitions of optical meron lattices at the metal/uniaxial crystal interface. Our theoretical studies show that by rotating the optical axis orientation of the uniaxial crystal, meron lattices constructed by electric-field vector undergo phase transitions from a topologically nontrivial to a topologically trivial state, whereas the skyrmion number of the spin meron lattices remains robust against such rotations. The findings offer new insights into the topological stability and phase transitions of topological quasiparticles under light–matter interactions and hold promise for applications in optical data storage, information encryption, and communications.
【AIGC One Sentence Reading】:This study explores formation, stability, and phase transitions of photonic meron lattices at the metal/uniaxial crystal interface. Rotating the crystal's optical axis causes phase changes in electric-field meron lattices, while spin meron lattices remain stable, with potential for data storage and communications.
【AIGC Short Abstract】:Optical topological quasiparticles like meron lattices are promising for high-dimensional optical data storage and communications. Unlike prior isotropic media studies, we explore the formation, topological stability, and phase transitions of photonic meron lattices at the metal/uniaxial crystal interface. Rotating the crystal's optical axis causes phase transitions in electric-field-vector-constructed meron lattices, while spin meron lattices remain stable, offering insights for applications.
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1. INTRODUCTION
Skyrmions are topologically protected quasiparticles characterized by three-dimensional (3D) topologically nontrivial spin textures into a two-dimensional (2D) plane via stereographic projection. The concept was originally proposed by nuclear physicist Tony Skyrme in the 1960s as soliton solutions in nonlinear field theory [1]. Since then, skyrmions and other quasiparticles have been widely predicted in various physical systems, including Bose–Einstein condensates [2], liquid crystals [3], superfluid [4], magnetic materials [5], and twistronics [6]. Particularly, magnetic skyrmions, owing to their topological stability and nanoscale feature size, are considered promising candidates for next-generation data storage [5]. Recently, skyrmionic structures have been introduced into optics [7–11], where topological skyrmionic textures are constructed by various degrees-of-freedom of electromagnetic (EM) fields, including the spin angular momentum (SAM) [8,10,12–23] and the electric-field vector [7,9,24–26] in confined fields, the Poynting vectors [27,28] and the Stokes vectors [29–40] in propagating fields, and the pseudo-spin vectors in nonlinear photonic crystals [41]. Similar to topological quasiparticles in magnetic materials [42–44], optical skyrmions can form either as isolated quasiparticles [11,28–39] or in lattice configurations [7,9–12,14–18]. For instance, in surface plasmon polaritons (SPPs) with continuous rotational symmetry, the spin-orbit coupling (SOC) of light leads to the formation of skyrmion-like spin quasiparticles [8], whereas in discrete rotational symmetries, spin skyrmion or meron lattices emerge, with their topologies constrained by both the rotational symmetry and the conservative property of total angular momentum (TAM) [13,20,21,45–48]. Optical quasiparticles show great potential for applications in optical communications [49,50] and topological quantum communications [51], and the concept has also been extended to other physical systems, such as water waves [52,53] and acoustic waves [54].
Previously, most research on topological quasiparticles in the optical near field has primarily focused on the construction of various novel types of optical topological textures at the metal/isotropic media interface, and the topological stability of the resulting textures remains unexplored. In particular, the evolution of optical topological lattices in anisotropic media has yet to be investigated. The anisotropy related to the lattice symmetry of crystals or artificial meta-atoms is widely present in modern nanophotonics, such as liquid crystal devices for topological storage and logic devices [55], and metamaterials and metasurfaces for chiral bound states in the continuum [56,57], and thus the investigation of the evolution of optical topological lattices in anisotropic media is critical for the future exploitation of applications.
In this study, we systematically investigated the formation, topological stability, and phase transitions of optical meron lattices at the metal/uniaxial crystal interface. We derived the explicit expressions for the electric and magnetic fields, as well as the SAM, of surface plane waves at the metal/uniaxial crystal interface. By arranging these surface plane waves in rotational symmetry and considering the conservation of TAM, we constructed electric-field meron lattices and spin meron lattices, respectively. More importantly, our theoretical results demonstrate that varying the optical axis (OA) orientation of the uniaxial crystal can induce phase transitions in the electric-field meron lattice, from a topologically nontrivial to a topologically trivial state. In contrast, the skyrmion number of the spin meron lattice remains stable against such rotations, demonstrating its topological stability. This difference arises because in the instance of the electric-field meron lattices, the surface waves are no longer pure transverse magnetic (TM) SPP modes at the metal/uniaxial crystal interface, whereas for the spin meron lattices, the decomposition of TAM into orbital and spin components in an anisotropic medium is similar to that in an isotropic medium. The results provide a novel mechanism to achieve the topological stability and phase transitions of topological quasiparticles in optical systems and open new avenues for advanced spin-optics and topological photonics applications.
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2. THEORY
A. EM Field at Metal/Uniaxial Crystal Interface
The optical system as illustrated in Fig. 1(a) consists of a semi-infinite uniaxial crystal occupying the region and an isotropic metal in the region . The and axes lie in the interface between the two media (), while the axis is perpendicular to the interface. Silver is selected as the isotropic metal material with its dielectric constant set to at a wavelength of [58]; the imaginary part is neglected for simplicity. Without loss of generality, we first assume that the principal axes of the uniaxial crystal are aligned along the , , and directions of the Cartesian coordinate system. The principal dielectric constants and refractive indices of the crystal are denoted as and , respectively. In this case, the permittivity tensor of the uniaxial crystal can be expressed as a diagonal matrix comprising the principal elements: , where is the permittivity in vacuum. The anisotropic medium is chosen as the negative uniaxial crystal material calcite () [59], with the ordinary refractive indices and the extraordinary refractive index .
Figure 1.(a) Schematic diagram of surface waves at the metal/uniaxial crystal interface. As shown, the OA of the uniaxial crystal lies in the plane and forms an angle with the axis. (b) Variation of the normalized propagation constant of the surface waves with respect to the OA orientation angle .
To derive the expressions of electric and magnetic fields of the hybrid surface waves and the propagation constants, we consider the case where the hybrid surface plane waves propagate along the direction and rotate the OA orientation angle , which is defined by the intersection angle between the OA and the axis. In this instance, the corresponding permittivity tensor can be obtained by the rotational operator as (see Appendix A for details) where , , and . It can be observed that, when the OA is rotated, the horizontal components and the nondiagonal terms determined by the , and of the permittivity tensor are changed correspondingly, which results in the variations of the propagation constants.
The metal/uniaxial crystal waveguide can support the hybrid SPP modes that include both TM and transverse electric (TE) polarization components [60,61]. As indicated above, we assume that the surface plane wave propagates along the axis and decays exponentially in the direction: and , where and are the transverse (propagation constant) and longitudinal (attenuation coefficient) wave vector components. Based on Eq. (B7) in Appendix B, we obtain that the propagation constant in the hybrid surface mode is determined by where there are , with and . Here, represents the angular frequency of the EM field, and denotes the permeability. By applying the boundary conditions, the attenuation coefficient and the propagation constant can be obtained. As shown in Fig. 1(b), the normalized parameter reaches its maximum at and , and attains its minimum at , where denotes the wavenumber in vacuum. Subsequently, the distributions of the electric and magnetic fields via the OA orientation can be derived (see Appendix B for details).
B. Formation of Optical Topological Lattices in C4 Rotational Symmetry
Optical topological lattices can be constructed by the superimposition of multiple surface plane waves. However, it is worth noting that the fundamental mechanisms for generating the optical lattices are the rotational symmetry and the conservative property of TAM in optical systems [13,20,21]. By superimposing multiple surface plane waves, it is possible to approach the solutions of Maxwell’s equations under discrete rotational symmetries. Therein, optical topological lattices with strictly rotational and translational symmetries can be formed in , and rotational symmetries, whereas other polygonal symmetries, such as five-fold rotational symmetry, give rise to optical quasi-crystals, moiré lattices, and mixing skyrmions and merons topologies [45–48]. In systems with continuous rotational symmetry, the isolated skyrmions can be formed [8]. In rotational symmetry, the out-of-plane electric-field component of the hybrid surface wave can be derived by the Hertz potential, expressed as [62] where is a constant, , and represents the quantum number of TAM.
In the real optical systems for generating optical topological lattices, it is more convenient to fix the uniaxial crystal and rotate the excited surface waves. Although Eq. (2) considers the solution of the propagation constant when the surface wave propagates along the axis direction and the OA of the uniaxial crystal is rotated, it can be transformed to the solution of the real optical systems by a rotation matrix along the axis flexibly. Consequently, can be reformulated as where , and plays a key role in tuning the optical topological texture. It can be observed from Eq. (4) that even in the presence of an anisotropic uniaxial crystal, the distributions of EM fields still exhibit periodicity with respect to the quantum number of TAM.
The topological property of the skyrmionic texture can be characterized by the skyrmion number, which is defined as follows [5]:
Here, denotes the normalized unit vector, and the skyrmion number quantifies how many times the vectors wrap around a unit sphere. Specifically, corresponds to skyrmions, in which the entire unit sphere is covered once, whereas corresponds to merons, in which only a hemisphere is covered [43,44].
3. RESULTS
A. Electric-field Meron Lattices and Topological Phase Transitions
In this section, we first analyze the case and the propagating directions of surface waves align with the principal axes (i.e., ). In this instance, the four surface plane waves form the standing wave fields along the and directions. The standing wave fields interfere at the metal/uniaxial crystal interface, thereby generating the electric-field meron topological lattice. Figure 2(a) shows the real part of the out-of-plane electric-field component , which exhibits a symmetry. The corresponding 3D electric-field vector structure is shown in Fig. 2(b). Within each unit cell, the electric-field vector varies from a central “up” or “down” state to an edge flat state, which manifests as a Néel-type meron texture with alternating polarity. According to Eq. (5) and , we use the breadth-first search (BFS) algorithm [63] to identify the boundaries where , and calculated the skyrmion number within the unit cell marked by a black square to be . The skyrmion number can approach 0.5 by increasing the number of sample points further.
Figure 2.Electric-field meron lattice with symmetry for . (a) Distribution of the normalized real part of the out-of-plane electric-field component at . Black square markers indicate the boundaries of the unit cell located at the central region of the lattice. (b) 3D vector diagram of the electric-field meron lattice corresponding to (a). (c) Variation of the skyrmion number within the unit cell at the center of the lattice via . The grid size in simulation is 0.633 μm and the number of sample points is 1001.
To evaluate the stability of the electric-field meron lattices with respect to the OA orientation of the uniaxial crystal, we rotate the four surface plane waves and compute the skyrmion number of the central unit cell under varying , as illustrated in Fig. 2(c). The skyrmion number is found to oscillate as the varies from 0° to 180°, and it reaches 0.5 only at discrete angles: , 45°, 90°, 135°, and 180°. The results reveal that the topological properties of the optical lattices can be tuned from topologically nontrivial states to topologically trivial states by varying the orientation angle .
Under rotational symmetry, the lattices remain invariant upon a 90° rotation. Accordingly, three orientation angles , 45°, and 70° are selected for analysis. Figures 3(a)–3(c) show the distributions of , where the black arrows represent the directions of the in-plane electric-field vectors. The symmetry of lattices is further confirmed by the Fourier transform of , shown in the insets of Figs. 3(a)–3(c). The electric-field meron lattices in Figs. 3(a) and 3(b) exhibit a Néel-type topology at and a twisted-type topology at , respectively. However, at , the calculated skyrmion number is 0.365, and the electric-field vectors exhibit a discontinuous distribution, indicating a nontopological lattice, as shown in Fig. 3(c). The mechanism underlying the phase transitions in the electric-field meron lattice can be understood through the propagation constant diagram in Fig. 1(b). Similar to the case of TM SPP modes at the metal/isotropic media interface, the surface waves at the metal/uniaxial crystal interface remain a pure TM SPP mode at , 90°, and 180°, which supports the formation of the electric-field meron lattices. However, at other orientation angles, the surface waves evolve into hybrid SPP modes, leading to the observed topological phase transitions. Notably, at and 135°, the off-diagonal components of the dielectric tensor of the uniaxial crystal reach their maximum values, resulting in strong coupling between TE and TM SPP modes. This strong coupling leads to the propagation constant reaching a peak and gives rise to the twisted-type topological lattice. Figures 3(d)–3(f) represent the corresponding topological textures of electric-field vectors encoded in the HSL color space: saturation is maximal, lightness encodes the component, and hue corresponds to . These visualizations reveal that the electric-field lattice becomes structurally unstable as varies, revealing that the OA orientation governs the topological phase transitions of the electric-field meron lattices.
Figure 3.Electric-field topological textures at , 45°, and 70°. (a)–(c) Distributions of (background) with the orientations of the in-plane electric-field vectors (black arrows), and the insets show the corresponding Fourier space patterns. (d)–(f) Topological textures for , 45°, and 70°, respectively. A consistent mapping scheme is used throughout the paper to visualize the topological textures.
Then, we consider the formation of topological lattices for the quantum number of TAM . It is worth noting that, at the metal/isotropic media interface, the topological lattice formed at is similar to that of , as the propagation constants of all OA orientation angles are the same. However, at the metal/anisotropic media interface, the situation is different. At , an electric-field meron lattice is formed, with its 3D vector distribution depicted in Fig. 4(a). It can be found that the topological lattice formed at differs from that of . This difference arises from the distinct quantum number in phase terms of Eq. (4): for and for . Furthermore, we calculate the skyrmion number of the marked unit cell via [Fig. 4(b)]. A significant transition occurs near , where the skyrmion number undergoes a sharp gradient. This sharp variation demonstrates strong sensitivity to the OA orientation, which is potentially applied in the optical sensing with ultrahigh sensitivity. Figures 4(c) and 4(d) illustrate the distributions of and their corresponding topological textures for , 45°, and 90°, respectively. The calculated skyrmion numbers are , 0, and 0.490, respectively. Notably, comparing Fig. 4(c3) with Fig. 4(c1), a reversal of the electric-field vector directions is observed within the marked unit cell at . This reversal originates from the difference in electric-field vector orientation induced by in phase term of Eq. (4), and explains why the skyrmion number becomes positive in the range of approximately 45°–135°, as illustrated in Fig. 4(b). It can be observed that it even caused the annihilation of topological lattice due to the appearance of an imaginary unit in the electric-field component when at . It should be emphasized that for , when the OA orientation angle is not an integer multiple of 0° or 45°, the skyrmion number calculated from is not strictly accurate. In such cases, the electric-field components are not in phase, and due to the presence of temporal components, the field oscillates at different time points. As a result, the electric-field structure varies with time, making it impossible to form a strictly defined skyrmion. However, since only the real part of an electric-field component can be measured experimentally, we use to calculate the skyrmion number here.
Figure 4.Electric-field meron lattice with symmetry for . (a) 3D electric-field vector diagram of the meron electric-field lattice at . (b) Variation of the skyrmion number within the unit cell at the center of the lattice via . (c) and (d) Distributions of and the corresponding topological textures at , 45°, and 90°, respectively. The grid size in simulation is 0.8862 μm, and the number of sample points is 1001.
Finally, we consider the case of nonzero quantum number of TAM. In evanescent vortex fields, the formation of spin lattices induced by SOC has already been reported [20,21]. As for the surface plane wave at the metal/uniaxial crystal, the time-average Poynting vector is given by , where the asterisk denotes the complex conjugate, whereas the kinetic momentum of light associated with the time-average Poynting vector is . Then, the TAM is with the position vector, and it can be re-expressed by the sum of SAM and orbital angular momentum (OAM) through vector calculation with identities based on Eq. (B2) in Appendix B as [64]
The first term in the right-hand side of Eq. (6) is the OAM density, and the second term is the SAM density.
We perform a comparative analysis of the cases with the quantum numbers of TAM and . Under rotational symmetric field, the SOC present in the hybrid surface waves field leads to the formation of spin meron lattices by the unit vectors of SAM as .
In both cases, Figs. 5(a) and 5(b) depict the normalized out-of-plane SAM distributions at , which exhibit symmetry. The corresponding 3D spin orientation distributions show the formation of spin meron lattices, as shown in Figs. 5(c) and 5(d). Within each unit cell, the local spin orientations gradually transition from a central “up” or “down” state to an edge flat state (). The calculated skyrmion numbers within the black-framed regions are and , respectively. To evaluate the stability of these lattices, we calculate the skyrmion number of the central unit cell under different , as shown in Fig. 5(e). It can be observed that regardless of changes, the skyrmion numbers remain nearly constant at approximately in both cases. This remarkable stability indicates that the topological spin lattice exhibits robustness to varying .
Figure 5.Spin meron lattices in rotational symmetry for and 3. At , (a) and (b) present the normalized out-of-plane SAM distributions for and 3, respectively. (c) and (d) show the corresponding 3D vector diagrams of the spin meron lattices. (e) Variation of the skyrmion number within the unit cell at the center of the lattices via , for (blue curve) and (orange curve). The grid size in simulation is 0.633 μm, and the number of sample points is 1001.
To further explore the topological characteristics of spin lattices for and , we chose , 45°, and 70°, as the instance of . The first row of Figs. 6(a) and 6(b) presents distributions, with black arrows indicating the directions of the normalized in-plane SAM. The insets show the Fourier transforms of to observe the symmetry of lattices. The second row illustrates the calculated phase distributions of , where black arrows represent the energy flow of the hybrid surface waves, exhibiting alternating circulations. Specifically, each vortex center of the Poynting vector corresponds to a phase singularity of . The third row visualizes the spin vector orientations, clearly displaying the evolution of topological spin textures. At and 45°, each unit cell exhibits a Néel-type meron texture, whereas at , a twisted-type meron texture emerges. Despite these changes in spin texture, the skyrmion number remains unchanged, reflecting its topological protection. This demonstrates both the invariance of the skyrmion number and the robustness of spin meron lattice textures against changes in .
Figure 6.Spin meron lattices textures at , 45°, and 70°. The first row shows distributions, with black arrows representing the orientations of the normalized in-plane SAM vectors, and the insets show the corresponding Fourier space patterns. The second row presents the phase distributions (background) of for hybrid surface waves, with black arrows representing the directions of the normalized Poynting vectors. The vortex center of the Poynting vector corresponds to a phase singularity. The third row shows the corresponding topological spin textures for , 45°, and 70°. The left panel (a) corresponds to the case of , while the right panel (b) shows the results for . The scale bar represents .
The origin of this topological stability can be attributed to two key factors. First, as shown in Eq. (6), the decomposition of TAM into orbital and spin components in an anisotropic medium is similar to that in an isotropic medium. Second, the results illustrated in Fig. 6 indicate that within a uniaxial crystal, the directions of spin and energy flow density are locked with each other to maintain the stability of the skyrmion number of topological textures. According to the spin-momentum equation [62], the surface integral of SAM over the transverse plane can be converted into a line integral of the kinetic momentum . As the integration region extends to infinity, approaches zero, so the surface integral of is also zero. Consequently, SAM must simultaneously exhibit positive and negative values in a continuous distribution. This ensures the existence of regions where spin vector orientation transitions from positive to zero and from negative to zero, thus maintaining the topological stability of the spin meron lattice.
4. CONCLUSION
In conclusion, we have demonstrated the formation of optical meron lattices at the metal/uniaxial crystal interface. Specifically, electric-field meron lattices are formed when the TAM quantum numbers are and , while spin meron lattices emerge for and , and the topological lattices exhibit periodicity () with respect to the quantum number of TAM. Notably, the skyrmion number of the spin meron lattices is invariant for various values of , indicating its topological stability. This invariance can be attributed to the fact that the decomposition of TAM into orbital and spin components in an anisotropic medium is similar to that in an isotropic medium. Furthermore, based on the spin-momentum relations, the SAM exhibits a continuous distribution containing both positive and negative values, thereby ensuring the topological stability of the spin meron lattice. In contrast, as the orientation angle is tuned, the surface waves are no longer pure TM SPP modes at the metal/uniaxial crystal interface, leading to topological phase transitions in the electric-field meron lattices. These results provide novel physical insights into the topological stability and phase transitions of topological quasiparticles in optical systems, and offer an avenue for exploring applications in advanced spin-optics and topological photonics.
APPENDIX A: PERMITTIVITY TENSOR
When the uniaxial crystal is rotated around the axis by an angle , its permittivity tensor can be obtained via a coordinate transformation, where represents the rotation operator and is the permittivity tensor with the principal axes of the uniaxial crystal aligned along the , and axes of the Cartesian coordinates. By calculating Eq. (A1), Eq. (1) can be derived.
APPENDIX B: HYBRID MODES AT METAL/UNIAXIAL CRYSTAL INTERFACE
First, for systems containing anisotropic materials, Maxwell’s equations can be written as where and . Under the condition with no free charges and the time-harmonic monochromatic EM field, the equations can be re-expressed as where , represents electric conductivity. By applying the curl operation to both sides of Faraday’s law and Ampere’s law, the wave equations for the electric and magnetic fields can be derived as follows:
For a hybrid SPP mode (), we can obtain that the electric and magnetic fields at metal/uniaxial crystal interface are where . If we assume that the hybrid surface plane wave is along the direction [ and ], which means that only survives in the transverse wave vector, and the transverse wave vector component is derived from the terms of the electric and the magnetic Gauss’ law,
They can be rewritten as
Therefore, the propagation constant (take the positive value) can be calculated as follows:
In the metal half-space, the EM fields can be expressed as ()
The propagation constant can be re-expressed as in the metal material and the electric and magnetic fields can be given by
In the uniaxial crystal half-space, there are
And in metal materials, there are
By utilizing the continuity of the transverse field at the boundary plane, we can obtain
After simplification, the expression can be rewritten in the form of a linear matrix by setting and ,
The nontrivial solutions of matrix [Eq. (B13)] requests,
From Eqs. (B14) and (B7), one can obtain the propagation constant and evanescent wave vector and the distributions of electric and magnetic fields for any OA orientation angle .