Lithium niobate (LN) has rich physical effects, such as electro-optic, nonlinear, photorefractive, piezoelectric, pyroelectric, and wide transparent window (0.35 to
Advanced Photonics, Volume. 5, Issue 3, 034002(2023)
Advances in lithium niobate thin-film lasers and amplifiers: a review
Lithium niobate (LN) thin film has received much attention as an integrated photonic platform, due to its rich and great photoelectric characteristics, based on which various functional photonic devices, such as electro-optic modulators and nonlinear wavelength converters, have been demonstrated with impressive performance. As an important part of the integrated photonic system, the long-awaited laser and amplifier on the LN thin-film platform have made a series of breakthroughs and important progress recently. In this review paper, the research progress of lasers and amplifiers realized on lithium niobate thin film platforms is reviewed comprehensively. Specifically, the research progress on optically pumped lasers and amplifiers based on rare-earth ions doping of LN thin films is introduced. Some important parameters and existing limitations of the current development are discussed. In addition, the implementation scheme and research progress of electrically pumped lasers and amplifiers on LN thin-film platforms are summarized. The advantages and disadvantages of optically and electrically pumped LN thin film light sources are analyzed. Finally, the applications of LN thin film lasers and amplifiers and other on-chip functional devices are envisaged.
1 Introduction
Lithium niobate (LN) has rich physical effects, such as electro-optic, nonlinear, photorefractive, piezoelectric, pyroelectric, and wide transparent window (0.35 to
On the other hand, active optical devices, such as lasers and amplifiers, on the LNOI platform have also been expected for a long time as an essential part of integrated photonics. Due to the inherent indirect bandgap structure, it is difficult for LN to achieve electroluminescence. A simple and feasible scheme is to dope rare-earth ions (REIs) into LN as a gain medium to realize light sources and amplifiers under an optical pump. In addition, lasers and amplifiers for LNOI integrated photonics can also be realized by hybrid integration of the commercial semiconductor lasers or amplifiers or heterogeneous integration of the III-V gain materials with an electrical pumping scheme.
This paper reviews the recent research on lasers and amplifiers developed on the LNOI platform. Figure 1 shows the research road map for the LNOI light sources and amplifiers, which is also the overall idea of this paper. In Sec. 2, the research processes of lasers and amplifiers based on REI doping LN are introduced. Specifically, the common methods of REI doping in LN crystals and the study of spectral characteristics of doped crystals are discussed first. Subsequently, the important parameters for characterizing microlasers are discussed. Then, the research works of multimode microdisk lasers, multimode microring lasers, single-mode lasers, and amplifiers on the REI-doped LN thin film are presented. At the same time, the challenges of laser and amplifier performance and the potential improvement scheme for the REI-doped LNOI lasers and amplifiers are discussed. In Sec. 3, the electrically pumped III-V lasers and amplifiers on LNOI platform, as well as the applications of the laser transmitter and tunable Pockels laser confirmed by deploying the electro-optical effect of LN are introduced. Then, the advantages and challenges of the LNOI III-V lasers are analyzed with a comparison with REIs-doped lasers. In Sec. 4, the application prospects of LNOI-based lasers and amplifiers are explored, combined with other LNOI functional devices, such as sensing, broadband optical communication, and frequency converter. Finally, in Sec. 5, the contents of the whole review are briefly summarized. At the same time, future research and development of LNOI-based lasers and amplifiers are envisaged.
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Figure 1.Research field overview of LNOI light sources and amplifiers, which can be roughly classified into three parts: the optical-pump REI-doped devices and electrical-pump III/V devices and their applications. Some schematic sources: M-M (multi-mode) laser, reprinted from Ref. 27; S-M (single-mode) laser, reprinted from Ref. 28; amplifier, reprinted from Ref. 29; Hybrid laser, reprinted from Ref. 30, © 2021 Optica; hetero laser, reprinted from Ref. 31, © 2021 Optica; printing laser, reprinted from Ref. 32, © 2021 Optica; transmitter, reprinted from Ref. 33, © 2021 Optica; tunable laser, reprinted from Ref. 34 under a CC-BY license.
2 Optically Pumped Lasers and Amplifiers
The indirect bandgap structure of LN crystal makes it challenging to realize electrically pumped luminescence. Nevertheless, photoluminescence based on REI doping is a simple and effective method that is widely favored by researchers. For example, various REI-doped waveguide lasers and amplifiers based on bulk LN crystal have been confirmed successfully.35
2.1 Rare-Earth Ion Doping and Spectroscopic Analysis
Roughly, there are three main ways to dope REIs into LN crystal. The first one is to add REI oxide for doping when growing LN crystal by the Czochralski method and obtain LN single crystal with uniform ion concentration,39,40 as shown in Figs. 2(a) and 2(d). The second method is thermal diffusion, mainly through vacuum deposition of the REI layer, and then selective doping through high-temperature diffusion,37 as shown in Fig. 2(b). In thermal diffusion doping, the diffusion depth of REIs has the characteristics of from complementary error function (erfc)-like to semi-Gaussian shape distribution [Fig. 2(e)].41 Due to the low diffusion rate of REIs, the diffusion temperature must be close to the Curie temperature of LN, which is generally as high as 1100°C and requires a diffusion time of up to 150 h. The diffusion time depends on the crystal phase of the LN substrate. The third method is to dope LN crystals with REIs by ion implantation,42 as shown in Fig. 2(c). At room temperature, ions are accelerated to million electron volt energy by Van der Graaff accelerator or transistor accelerator and implanted into the LN crystal. The ion concentration displays a nearly Gaussian distribution [Fig. 2(f)] and high-temperature annealing above 1000°C is needed to eliminate the defects caused by implantation and restore the quality of single-crystal LN.
Figure 2.Methods for REI doping into LN crystal and the corresponding concentration-depth distribution. (a) and (d) Crystal growth doping; (b) and (e) thermal diffusing doping; and (c) and (f) ion implantation doping.
The above three doping methods are relatively mature technologies after a long time of development and are expected to realize industrialization. But they also have their advantages and disadvantages. For example, compared to diffusion and ion implantation doping, crystal growth doping can obtain a high doping concentration and more uniform ion distribution and thus has a promising future in realizing high power and low transmission loss lasers and amplifiers. In contrast, for thermal diffusion and ion implantation, the maximum concentration of doped erbium ions is
In recent years, referring to the incorporation of REIs into LN bulk crystal, many research groups have carried out research on REI-doped LNOI integrated photonics.45,46 For example, Dutta et al. first prepared 300-nm-thick thin-film LN from 0.1% thulium-doped X-cut LN bulk by the smart-cut process, and then prepared the grating coupling structure and single-mode waveguide by EBL-dry etching process, as shown in Fig. 3(a).47 To explore the optical properties of thulium ions in the thin-film waveguide, the absorption, emission spectra, and fluorescence lifetime were measured at a 3.6 K low temperature. Compared to a thulium doped-bulk crystal, the thulium ions in smart-cut thin film displayed virtually identical optical properties, which indicates that the smart-cut process can preserve the optical properties of REIs in thin films well. Notably, the preparation of the REI-doped LNOI is compatible with wafer-scale integration, paving the way to achieve on-chip active photonics systems and applications. Furthermore, an atomic frequency comb memory was realized in thulium-doped LNOI waveguides by the same doping and fabrication process, and the storage spectrum bandwidth and optical storage time were up to 100 MHz and 250 ns, respectively.53
Figure 3.(a) Schematic of the thulium-doped LNOI waveguide with grating couplers. Reprinted with permission from Ref. 47, © 2020 American Chemical Society. (b) SEM image and concentration distribution of erbium ions implanted in LNOI structure. Reprinted from Ref. 48, with the permission of AIP Publishing. (c) Schematic cross-sectional diagram and SRIM simulation distribution of ytterbium ions implanted in LNOI structure. Reprinted from Ref. 49, with the permission of AIP Publishing. (d) Schematic diagram of ytterbium ions implanted in LNOI tunable microcavities. Reprinted from Ref. 50, © 2022 Optica. (e) Optical micrograph of the LNOI device and schematic cross-sectional drawing after bonding with
Recently, Wang et al. explored the optical coherence of the erbium-doped smart-cut LN thin film prepared from bulk erbium-doped LN. Experimentally,
In addition, Wang et al. also carried out research on ion implantation doping based on a prepared LNOI microcavity. First, a microring coupled with a waveguide was fabricated by the
At the same time, Xia et al. directly doped ytterbium ions into an X-cut LN thin film with a thickness of 470 nm by ion implantation.50 After post-annealing at a slightly higher temperature of 650°C, no apparent film damage was observed. Then, ytterbium-doped microcavities with a radius of
In addition, Yang et al. hybrid integrated the erbium-doped yttrium orthosilicate with a concentration of 50 ppm (parts per million) to LNOI microring by flip-chip bonding, as shown in Fig. 3(e).51 The fluorescence lifetime of erbium ions was measured as 11.5 ms, consistent with the bulk material result of 11.4 ms. At the same time, the resonance broadening phenomenon caused by ion-cavity coupling was also observed, and the coupling intensity factor was assessed to be 0.36. Moreover, the erbium ions-implanted LN crystal directly integrated on a silicon photonic chip was reported by Jiang et al., as shown in Fig. 3(f). The optical properties of erbium ions in the integrated structure were investigated, and a modification of the photoluminescent emission was observed.52
Affected by the differential thermal expansion rates of the layers in the LNOI wafer, the tolerable annealing temperature (
2.2 Whispering Gallery Microcavity Lasers Based on REI-Doped LNOI
The three elements of a laser are the pump source, the gain medium, and the resonator. The gain medium and pump wavelength are determined by selecting the type of REI. The resonant cavity of a traditional laser is mainly composed of two or more mirrors. Compared with traditional resonators, whispering gallery mode (WGM) microcavities with circular structures can confine light by “continuous total internal reflection” for a long time within an ultrasmall mode volume, leading to strong light–matter interactions. Benefiting from the high quality factor (
2.2.1 Important parameters for characterizing microlasers
Before introducing the research progress of microlasers based on REI-doped LNOI, we discuss some important parameters for characterizing microlaser performance.
Lasing threshold
The lasing threshold refers to the pump power when the gain provided by the gain medium is just equal to the loss of the laser cavity. The pump threshold power (
Conversion efficiency and maximum laser output power
The conversion efficiency of a laser refers to the rate of change of the generated signal power relative to the pump power at the working stage above the lasing threshold, which reflects the conversion efficiency from the pump to signal during the laser operation. At the same time, it is obvious that the maximum laser output power refers to the maximum power that can be obtained when the laser is working, which can reflect the available power level of the laser for subsequent work. For optimizing these two parameters, laser signal extraction should also be optimized. That is to say, high pump efficiency and signal extraction efficiency should be guaranteed simultaneously. However, because the pump and signal are in different bands, the coupling state between a tapered fiber or straight waveguide and a resonator is inconsistent. Generally, the maximum output power of the laser is observed when the pump light is in an overcoupled regime in the experiment. To realize high conversion efficiency and low threshold, it is often necessary to design a broadband coupling to meet the requirements of efficient pump and signal extraction.68 In addition, different from optimizing the laser threshold, a large resonator size or cavity length is required to improve the gain accumulation to obtain an intense laser output.
Laser linewidth
Laser linewidth usually refers to the full width at half-height of the signal mode in the laser spectrum, which is an important parameter reflecting the coherence and noise of the laser. According to the Haken–Lax–Scully formula, the linewidth of the emitted laser operating above the threshold can be expressed as69
2.2.2 Multimode microdisk and microring lasers
Wang et al. reported an erbium-doped LNOI laser based on a
Figure 4.(a) The emitted laser signal at the 1560-nm band under the 976 nm laser pump. Inset: the accompanied green-up conversion fluorescence. Reprinted from Ref. 70, © 2021 Optica. (b) The observed signal wavelength drift process with different pump powers for the 974 nm pump. Reprinted from Ref. 27. (c) The dependence of the dominant mode signal power on the pump power. Reprinted from Ref. 71. (d) The collected spectra at different pump power. (e) The observed SHG and SFG at the 969 nm laser pump. Inset, the captured photograph of the microdisk at the visible (left) and IR (right) regions. (d) and (e) Reprinted from Ref. 72, © 2021 Optica. (f) The dependence of signal power (squares) and linewidth (circles) of the dominating lasing mode on the increasing pump power. Reprinted from Ref. 73, © 2022 Optica.
Subsequently, Liu et al. fabricated a
Except for the 1550-nm band, the microlaser operating at other wavelength bands has many unique applications. For example, due to the negligible water absorption at the 1060-nm band, the ytterbium ion emission can be applied for biosensing. In addition, compared with an erbium ion, ytterbium ion has a simple energy level structure and higher absorption cross section at the 980-nm band, which has substantial potential to improve the output power and conversion efficiency of microlasers. Zhou et al. first reported a microdisk laser based on an ytterbium-doped LNOI chip.72 With the continuous laser pump at 984 nm, the lasing signals at the 1030- and 1060-nm bands were observed in the increasing pump power range, as shown in Fig. 4(d). A threshold of
Subsequently, Luo et al. also reported 1060-nm band microdisk lasers with a high conversion efficiency.73 Based on an ytterbium-doped LNOI wafer with a doping concentration of 1.5%, the microdisk cavities were fabricated in a batch using
The research works of REI-doped LNOI laser described above are based on microdisk cavities. The microdisk cavity is mainly pumped and monitored by a fiber taper, which has the limitations of unstable coupling and inconvenient further integration with other on-chip functional devices. Microring cavities coupled with an on-chip waveguide can overcome these limitations. Furthermore, microring cavities usually have a smaller mode volume than a microdisk cavity with the same radius, which means that the light field power density in the cavity is more significant under the same pump power, leading to a lower laser threshold.
Luo et al. prepared a microring cavity coupled with a waveguide using the
Figure 5.(a) Collected power of signal mode under different pump powers. Inset: the captured green up-conversion fluorescence. Reprinted from Ref. 77, © 2021 Optica. (b) The detected emission spectra at different pump power. Inset: schematic of the bonding process for the microring and waveguide structures. (c) The recorded signal spectrum at 1533 nm for the varying electric voltage between
At the same time, Yin et al. fabricated a Z-cut erbium-doped LNOI microring cavity with 1% doping concentration and an undoped LNOI waveguide by the PLACE technique, respectively. Then, the LNOI microring was vertically coupled with the waveguide structure, as shown in the inset of Fig. 5(b).78 With a 980-nm laser pump, a broadband lasing signal in the 1550-nm band was observed with different pump power. A lasing threshold of 3 mW was deduced by fitting the signal power data. The wavelength tuning of the mode around 1533 nm was electrically tuned in a range of 0.2 nm with an EO coefficient of
In addition, an integrated ytterbium-doped LNOI microring laser working at 1060-nm band was recently demonstrated by Luo et al.79 Similar to the reported erbium-doped microring laser,77 the microring was fabricated using the
2.2.3 Single-mode lasers
Due to the broadband gain property of REIs, the REI-doped LNOI microcavity lasers introduced above generally operate in a multimode state, which is subject to false signals, random fluctuations, and instabilities and thus limits its application scenarios. Therefore, single-mode lasers featuring monochromaticity, high stability, and controllable output wavelength have attracted much attention due to their great potential for practical applications, such as optical communication and optical sensing. At present, there are four main ways to realize a single-mode laser. (1) Decreasing the size of the cavity to enlarge the free spectral range (FSR) and ensure only one resonant mode in the gain band range. (2) Designing narrowband distributed Bragg reflector (DBR) or distributed feedback (DFB) structures in the resonance cavity to achieve mode selection. (3) Cascading two or more cavities to realize mode selection by the Vernier effect. The specific mechanism is that the subcavities with different FSR (size) are coupled together. In such a system, the “supermode” is formed in the coupled cavities at the resonance overlapping location, while other normal modes resonate in only one cavity and dissipate in another cavity, resulting in greater losses. Therefore, the supermode with enlarged FSR and higher
First, Gao et al. fabricated coupled microdisks, also referred to as photonic molecule, based on erbium-doped LNOI with 1% doping concentration using the PLACE technique.80 The coupled microdisks with a diameter of 29.8 and
Figure 6.(a) Single-mode lasing spectra at different pump power. Inset: SEM image of the fabricated coupled microdisks. Reprinted from Ref. 80, © 2021 Optica. (b) Single-mode lasing signal with a high SMSR in coupled microrings at a pump power of about
Subsequently, to effectively improve the integration and scalability of REI-doped LNOI single-mode lasers, Zhang et al. designed a microring photonic molecule with radii of 85 and
Soon afterward, to reduce the requirement of tunability of pump light, Liu et al. demonstrated an erbium-doped LNOI single-mode laser based on a photonic molecule with a microdisk and a microring, as shown in the inset of Fig. 6(c).81 In this device, a single-mode laser emission with an SMSR of 31.4 dB in the range of 1520 to 1570 nm was observed with a 974-nm LD light source pump. Figure 6(c) displays the collected single-mode laser power as a function of pump power. The threshold and slope efficiency were deduced as 1.31 mW and
During the same period, Xiao et al. designed a single-frequency erbium-doped LNOI laser based on a coupling structure composed of a short microring cavity with a diameter of
Actually, controlling mode loss is also a popular way to achieve single-mode lasing due to the compact device size. For example, Li et al. demonstrated a single-mode laser based on a single microring resonator by regulating the mode loss.83 The microring resonator with a pulley waveguide was fabricated on a Z-cut 1% doped erbium-doped LNOI wafer using the
Figure 7.(a) Simulated mode profile for the four supported modes. (b) Collected single-mode laser emission spectra. Inset: the pump spectra after passing through the microring. (a) and (b) Reprinted from Ref. 83 under a CC-BY license. (c) Observed single-mode laser with a 37 dB SMSR. Inset: a captured image of the excited polygon modes for lasing signal, upconversion fluorescence, and pump, respectively. (d) Single-mode lasing wavelength at different applied voltages. (c) and (d) Reprinted from Ref. 84 under a CC-BY license. (e) Recorded signal spectra in the range of 1500–1600 nm with increasing pump power. Inset: the observed green upconversion fluorescence of the pumped microring. Reprinted from Ref. 85, © 2022 Optica. (f) Observed single-frequency lasing spectrum at 1544.658 nm with a pump power of 18 mW. Inset: the electrode configuration schematic of the tunable microdisk laser. Reprinted from Ref. 86.
Further, Lin et al. realized a single-frequency ultranarrow linewidth laser on a single microdisk, taking advantage of the polygon modes with high-quality factors and sparse mode distribution.84 The microdisk with a diameter of
In addition, Liang et al. also demonstrated a single-frequency microlaser based on an erbium-doped LNOI microring with the shape of quarter Bezier curves.85 The signal spectra in the wavelength range of 1500 to 1600 nm with a single-frequency lasing were recorded with the increasing pump power of a 976-nm laser, as shown in Fig. 7(e). The reason for realizing single-frequency lasing was probably mode-dependent loss and gain competition by comparing the transmission spectrum of the microring and the amplified spontaneous emission (ASE) spectrum in the waveguide. For a similar mechanism, Zhu et al. observed a single-frequency lasing with an SMSR of 29.12 dB based on an electro-optically tunable erbium-doped LNOI microdisk, as shown in Fig. 7(f).86 In addition, the wavelength of lasing mode was realized through continuous tuning in a 45 pm range by applying the electric voltage from
With the continuous attention and efforts of researchers, microdisks, microrings, and microdisk-microring coupling lasers have been realized based on the REI-doped LNOI platform, and the working state of the laser has also been improved from multimode to single mode. Table 1 summarizes the main performance parameters of the REI-doped LNOI microlasers reported so far. Based on the current research results, we discuss the main limitations and potential solutions for the development of REI-doped LNOI lasers.
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Low output power (μW-level) and conversion efficiency
At present, the conversion efficiency and output power of the reported lasers are still at a relatively low level of microwatts in either multimode or single-mode operation, which hinders the further integration of the laser with other functional devices. We believe that there are several ideas to improve the output power of lasers. (i) Increase the scale of the resonator. The reported works are based on WGM microcavities with a micrometer-scale radius, which limits the optical gain of the laser within such a small gain volume. Therefore, expanding the scale of the gain resonator is a promising method to improve the laser output power. For example, a high laser output power based on large-sized microdisk cavities87 and long waveguides with Sagnac loop reflectors88 has been reported recently. Compared with previous work of REI-doped LNOI microlasers, the output power has been improved by an order of magnitude. It should be noted that increasing the cavity length will naturally bring about the impact of multimode resonance, which poses a challenge to the single-mode operation of the laser. The mode screening mechanism for realizing single-mode operation described above needs to be considered in laser design. At the same time, the optimization of coupling between the bus waveguide (or tapered fiber) and resonant cavity for both pump and signal bands, such as introducing the bending waveguide coupling design68 to ensure effective pumping and effective extraction of signal light, can also effectively improve the output power and conversion efficiency of the laser. In addition, the waveguide integrated with the Bragg grating resonance structure can effectively increase the cavity length and ensure single-mode operation. The DBR or DFB laser with high output power has been confirmed on the silicon-based integrated photonics platform,89
Optical pumping scheme
Due to the selection of REIs as the gain medium, the working mechanism of optical pumping for the lasers is necessary, which imposes limitations on using lasers for out-of-laboratory applications, such as gas detection and biosensing. A practical solution is to integrate a commercial semiconductor laser as the pump source for the LNOI laser. For example, the electrically pumped laser and REI-doped chip can be hybrid integrated by the flip-chip technology, which is expected to effectively improve the portability of the laser. Zhou et al. reported the pioneering work demonstrating the electrically pumped REI-doped LNOI laser for the first time by butt-coupling a laser diode chip with an erbium-doped LN gain chip.96 In addition, the electrically pumped REI-doped LN lasers can also be realized by heterogeneously integrating III-V materials on REI-doped LN chips to construct the pump laser.97 It should be mentioned that compared with the electric pump laser realized by direct hybrid integration or heterogeneous integration, REIs have a long excited-state lifetime, resulting in REI-doped LNOI lasers with low signal noise and narrow linewidth, which has advantages for developing applications, such as optical coherent communication and quantum optics.
Wafer global doping
As mentioned in the previous introduction, the LN thin film cannot tolerate the high temperature conditions required by thermal diffusion or ion implantation to achieve high-concentration doping. Therefore, the method of incorporating REIs into LN thin film for the currently reported REI-doped microlasers is mainly doping in the growth process of bulk LN before ion slicing. However, one of the side effects of this doping method is that REIs are distributed on the entire LN thin-film wafer, which brings additional absorption loss and refractive index changes to the passive device integrated on the same chip, degenerating the device’s performance. There are several ways to realize local doping. (i) Before the LN thin film is formed by ion slicing, bulk LN wafers can be doped locally with REIs by thermal diffusion or ion implantation. Rüter et al. prepared a neodymium-doped LN thin film by thermal diffusion doping before ion slicing, which confirmed the possibility of local doping by this method.57 At the same time, it should be noted that incorporating REIs by thermal diffusion or ion implantation may pose a challenge to the sliced thin film quality. For example, Xu et al. reported that the thermal diffusion doping process increases the roughness and causes a slight deformation at the diffusion surface of the erbium-doped LN wafer.61 An additional CMP step before the ion slicing process is expected to improve this diffusion surface quality. (ii) Integrated REIs-doped LN thin film with undoped LN thin film by butt-coupling to construct active-passive LN thin-film devices. For example, Zhou et al. reported the work of tiling erbium-doped LN film and undoped LN film with ultraviolet curing adhesive and then prepared the monolithically integrated amplifier using a single continuous photolithography process based on the active-passive chip.98 The limitation of this method is that due to the integration of two different chips, the thickness may vary, resulting in an additional loss at the optical interface of active and passive chips. At the same time, the scalability and stability of large-scale integration for this method have certain limitations due to splicing the two independent chips. (iii) Hybrid REI material on LN thin film. Another promising scheme for localized incorporation of REIs is to deposit materials locally with REI gain media on LN thin film. For example, REI-doped
Some other aspects still need to be explored. The locking of the pump mode and the encapsulation of the coupling region deserve to be explored in the experiment to obtain high output power and stable operation of the laser during high-power pumping. Moreover, the wavelength tunability of the reported single-mode lasers is also limited. The thermo-optic effect of LN crystal can be utilized to achieve broadband wavelength tuning by integrating microheaters on the coupled resonators.105 Furthermore, combined with the outstanding electro-optical properties of LN, the REI-doped LNOI laser provides a promising platform for fundamental physics research, such as PT-symmetry breaking with natural advantages.106,107
2.3 Amplifiers Based on REI-Doped LNOI
In addition to lasers, amplifiers can provide gain for on-chip signals and therefore have fairly broad-based demand in on-chip optical communication, nonlinear frequency conversion, and other applications. High-gain waveguide amplifiers based on silicon nitride and integrated silicon platforms have been proven to be successful.108,109 However, due to the weak optical confinement as well as nonuniform distribution of REIs in titanium-diffused channel waveguide, the gain performance of waveguide amplifiers based on bulk LN is generally low (
Zhou et al. demonstrated the first waveguide amplifier on a Z-cut 600 nm-thick erbium-doped LNOI chip with 1% doping concentration.111 The 3.6-cm-long waveguide amplifier with a spiral design to reduce the overall device size was fabricated by the PLACE process. The signal gain at 1530 nm under different pump power was measured with a fixed on-chip signal power of 19.64 nW by a bi-directional pumping scheme. Then, considering the propagation loss calibration, the internal net gain for this signal wavelength was obtained by the equation
Figure 8.(a) The obtained internal net gain at 1530 nm with increasing pump. Inset: observed green upconversion fluorescence under the 980 nm laser pump. (b) The measured signal gain at different wavelengths. Inset: spontaneous spectrum measured in erbium-doped LN waveguide. Inset: detected spontaneous spectrum measured in erbium-doped LN waveguide. (a) and (b) Reprinted from Ref. 111. (c) Measured signal spectra as a function of increasing pump powers measured at 1531.6 nm. Reprinted from Ref. 112, © 2021 Optica. (d) Dependence of internal net gain at 1531.5 nm on the signal power. Inset: observed green upconversion fluorescence in the compact waveguide. Reprinted from Ref. 113. (e) The measured net gain for
At the same time, Chen et al. fabricated a compact 5-mm-long waveguide amplifier using the
Subsequently, Luo et al. reported on-chip erbium-doped LNOI waveguide amplifiers based on a similar simplified fabrication process without Cr film deposition and CMP steps.113 The amplifiers consist of a compact straight waveguide with a length of 5 mm. The doping concentration of erbium ions is 0.1%, which is much lower than that in previous reports. Under the 974.3-nm laser pump, the net internal gain at 1531.5 nm with a fixed signal power of 5 nW was investigated by increasing the pump power. A maximum net internal gain of 5.5 dB was obtained at a higher pump power of
To enhance the integration density of devices, Yan et al. also fabricated a 1% erbium-doped LNOI waveguide amplifier with a spiral design using the
In addition, inspired by the design of double-cladding fiber, Liang et al. fabricated
Also, the influencing factors, such as pump wavelength, pump mode, and waveguide length for the performance of the amplifier were carefully investigated by Cai et al. based on an erbium-doped LNOI waveguide amplifier with a concentration of
Figure 9.(a) The measured signal enhancement and internal net gain at different signal input power at 1531.6 nm. (b) The noise figure power and (c) the pump power conversion efficiency for different signal input power at 1531.6 nm. (d) The comparison of signal enhancement between 980 nm and 1484 nm pumps. Inset: modes distribution at 980 nm, 1484 nm, and 1530 nm. (e) The comparison of signal enhancement for different waveguide lengths. Inset: the simulation internal net gain at 1531.6 nm as a function of waveguide lengths. (f) The signal enhancement for different pumping schemes at 1531.6 nm. (a)–(f) Reprinted with permission from Ref. 117, © 2022 IEEE.
As can be seen from the above introduction, amplifiers with straight and spiral oxide cladding waveguide structures have been successfully verified based on REI-doped LNOI platforms. The pumping wavelength and pumping scheme of amplifiers are also explored. Table 2 summarizes the key parameters of REI-doped LNOI waveguide amplifiers reported so far. However, there are still several problems that need to be resolved in the development of amplifiers, as discussed below.
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2.3.1 High output power
Although a maximum net gain factor of 20 dB was realized based on a 10-cm-long waveguide. The high gain of the amplifier is obtained at the low input signal power (
2.3.2 L-band amplification
At present, the erbium-doped LNOI waveguide amplifiers confirmed work in the C-band (1530 to 1565 nm), and there is no research report on L-band (1565 to 1625 nm) LNOI amplifiers. However, it is very important to expand the bandwidth of on-chip communication. Because the emission cross section of erbium ion in LN at the L-band is much lower than the C-band, it is necessary to accumulate the gain with a longer waveguide length than the C-band amplifier to achieve the L-band amplification. Referring to the research of L-band erbium-doped fiber amplifier (EDFA),123 there are some methods to improve the L-band gain of the erbium-doped LNOI waveguide amplifier. (i) Since the signal to be amplified is in the L-band, the ASE in the C-band can also be used for pumping to improve the gain. For example, a C-band high-reflectivity grating structure can be introduced at the input end of the erbium-doped waveguide to recycle the unused backward ASE. (ii) An auxiliary pump light working at 1550 to 1560 nm can be introduced to enhance the L-band gain.
2.3.3 Gain flattening amplification
Another problem that needs attention is the gain flatness of the erbium-doped LNOI amplifier, which is particularly important in optical communications based on on-chip wavelength division multiplexing. Because the gain of an erbium ion is not flat in the broadband range, many studies have been done based on the erbium-doped fiber amplifier system to obtain the flat gain. The basic idea is to introduce a filter so that the changing trend of transmission loss relative to wavelength is consistent with that of the gain relative to wavelength and thus obtain broadband and flat gain. For example, Mach–Zehnder filter,124 acousto-optic filter,125 and long-period fiber grating126 have been used in EDFA to achieve wide flat-band gain. In addition, a dual-core fiber design was demonstrated to obtain an ultrawide-band gain-flattened EDFA by regulating the coupling between parallel transmission fibers.127 With the excellent photoelectric and acousto-optic properties of LN and the mature micro-nano processing technology of LNOI, the design experience based on the EDFA system can be conveniently transferred to the LNOI platform and hopefully achieve better gain flatness.
2.3.4 Some other limitations
The reported amplifiers mainly operate in the communication band. There is less research on amplifiers in other bands, which can be effectively expanded by doping with different REIs, such as neodymium and thulium.128 In addition, the problems of optical pumping and local doping of REIs also exist, which can be referred to in the previous discussion on REI-doped microlasers.
3 Electrically Pumped III-V Lasers and Amplifiers on LNOI Platform
In addition to REI doping, introducing III-V material as a gain medium is another common method to realize an integrated light source and amplifier. Because the laser and amplifier based on III-V material can work through direct electric pumping, it has the advantages of high gain efficiency and portability. It thus has become the mainstream route to develop integrated photonics gain devices. At present, the way to integrate an electric pump light source based on III-V gain materials with an LNOI platform can be roughly divided into hybrid integration, heterogeneous integration, and microtransfer printing, as described below.129
Hybrid integration is one of the most mature integration technologies that assembles several fully processed chips, such as III-V semiconductor devices and passive integrated photonics devices, into a single multifunctional device at the last packaging stage. Moreover, it can test and optimize discrete devices before integration to ensure the yield of integrated device products. Based on the current commercial mature small size III-V gain chip with high power and efficiency (such as support from Freedom Photonics LLC), namely, electrically pumped laser or semiconductor optical amplifier chip, there are mainly inter-chip hybrid integration and flip-chip hybrid integration methods used to realize an integrated active device. (i) Inter-chip hybrid integration. The active chip is assembled adjacent to the passive integrated external cavity chip and introduces gain through butt coupling. For example, Fig. 10(a) shows that the off-chip reflective semiconductor optical amplifier and the low-loss silicon nitride micro-ring external cavity chip are placed next to each other to realize the electrically pumped compact narrow linewidth integrated laser.135 To improve the optical coupling efficiency of the gain chip and the external cavity chip, the optical waveguides of the two chips should be aligned. A spot-size converter design is usually introduced in the optical interface of the passive chip. (ii) Flip-chip hybrid integration. The active chip is assembled on a solder bumps recess at the passive chip by the pick-and-place method. A schematic diagram of a hybrid silicon photonic flip-chip laser is shown in Fig. 10(b), and vertical alignment accuracy of
Figure 10.The integrated schemes for electrically-pumped integrated photonics gain devices. (a) Schematic diagram of a typical inter-chip hybrid integrated laser. Reprinted from Ref. 135, © 2017 Optica. (b) Schematic diagram of a flip-chip hybrid integrated laser. Reprinted from Ref. 136, © 2017 Optica. (c) Left, illustration of heterogenous integration for wafer bonding. Reprinted from Ref. 134 under a CC-BY license. Right, schematic diagram of a heterogenous integration narrow-linewidth
Heterogeneous integration is an integration technology that bonds III-V thin film wafer or dies to the top of a processed base wafer at the intermediate stage, as shown in the left panel of Fig. 10(c).134 Then the unprocessed III-V material is fabricated to the III-V gain devices, such as laser or amplifier arrays, by the lithography-etching process with a wafer-level scale. Due to the III-V devices being defined by the lithography process, an ultrahigh alignment accuracy for the light source and the passive device is realized by the adiabatic coupling at the interfaces between different layer waveguide structures to ensure an effective coupling. The right part of Fig. 10(c) shows the schematic diagram of a narrow-linewidth
Microtransfer printing is another popular technique that can pretest III-V devices before integration and enables a large-scale parallel integration, which elegantly combines the advantage of flip-chip hybrid integration and heterogeneous integration techniques. As shown in the left panel of Fig. 10(d), different from the wafer bonding technique, the laser or amplifier devices are prefabricated on the native III-V wafer before transfer to the processed wafer. In the microtransfer printing process, a polydimethylsiloxane (PDMS) stamp is used to pick up the prefabricated active devices (referred to as coupons) with an underneath release layer and transfer them to the passive devices with a single or arrays form.129 The alignment between the coupons and the passive device is realized by the digital pattern recognition based on the markers defined on the III-V wafer and base wafer in the prefabricated process. At present, an alignment accuracy of
Compared to wafer bonding techniques, microtransfer printing technology can achieve high-yield integration and does not need to adjust the back-end process flow due to the parallel processing of III-V devices and passive devices and the short transfer cycle. In addition, microtransfer printing techniques can reuse the expensive III-V native substrate, which reduces the cost to a certain extent. On the other hand, the wafer bonding approach has a high alignment accuracy and thus provides great advantages in optical coupling efficiency between active devices and passive devices and scalability. A more comprehensive introduction and discussion of the three basic integration approaches can be found in recent reviews.129,132 Based on the integration schemes of the above primary III-V gain devices, the electrically pumped III-V lasers and amplifiers based on the LNOI platform have also been developed, as presented in this section.
3.1 Hybrid Integration III-V Lasers
Han et al. first integrated an electrically pumped III-V laser with a passive LNOI chip.30 To realize broadband tuning and single-mode lasing, the LNOI chip incorporates a Vernier filter consisting of two cascaded microring resonators and a distributed Bragg reflector with a Gaussian apodization profile, as shown in Fig. 11(a). The hybrid laser has a threshold current of 100 mA corresponding to a threshold current density of
Figure 11.(a) Schematic of the tunable hybrid LNOI/III-V laser composed of an InP-based optical gain chip and an LNOI passive chip. (b) Recorded spectra of coarse wavelength tuning process. (a) and (b) Reprinted from Ref. 30, © 2021 Optica. (c) Schematic of the butt coupling of the electrically pumped hybrid laser. (d) Optical power inside the LNOI waveguide laser and voltage versus the laser driving current. Inset, the recorded lasing spectrum with the single-mode operation. (c) and (d) Reprinted from Ref. 33, © 2021 Optica. (e) Schematic illustration of lithium niobate integrated on Damascene platform (top) and self-injection locking principle (bottom) with laser wavelength tuning achieved by applying a voltage signal. Reprinted from Ref. 140 under a CC-BY license. (f) Single-sided power spectral density of frequency noise of the hybrid LNOI laser upon self-injection locking to racetrack resonator (red) and in free-running regime (green). Reprinted from Ref. 141. (g) The structure schematic of the hybrid integrated III-V/LNOI external cavity laser. (h) Laser frequency modulation rate as a function of modulation speed. (i) Observed dual-wavelength lasing spectra. (g)–(i) Reprinted from Ref. 34 under a CC-BY license.
Additionally, Shams-Ansari et al. developed a fully integrated high-power laser on a passive LNOI chip by flip-chip bonding a DFB laser.33 The LNOI chip was fabricated on an X-cut 600 nm thick LNOI chip by the
In addition, Kippenberg’s group reported a heterogenous
Recently, Li et al. demonstrated an electrically pumped Pockels laser through a hybrid integrated III-V RSOA with an LNOI external cavity structure.34 As shown in Fig. 11(g), the LNOI chip was designed as a Vernier mirror structure consisting of two racetrack resonators. To enrich the functionality of laser and expand its application scenarios, a microheater, electro-optic modulator, phase shifter, as well as a PPLN wavelength converter were incorporated into the LNOI external cavity chip. At the same time, the racetracks and bus waveguides were designed to support only quasi-TE mode to use the significant Pockels effect of LN. The lasing mode at 1581.12 nm with a threshold current of 80 mA was observed in experiments. The on-chip power was measured as
3.2 Heterogeneous Integration and Microtransfer Printing III-V Lasers and Amplifiers
Besides hybrid integration, de Beeck et al. reported a novel strategy for the microtransfer printing of III/V gain materials on a thin-film LN platform.32 First, the rib waveguides were fabricated starting from a 500-nm X-cut LN thin film with a sapphire substrate by the
Figure 12.(a) Top: schematic drawing of the different cross-sections for the heterogeneous integration platform. Bottom: schematic diagram of the designed ring laser and single-mode tunable laser. (b) Measured gain bandwidth of the III/V-on-LN amplifier. (c) Obtained LI curves of the ring laser at different temperatures. (d) Recorded spectra of the fine wavelength tuning of the single-mode laser. (a)–(d) Reprinted from Ref. 32, © 2021 Optica. (e) Optical microscopy image and SEM image of the cross-section of the heterogeneously integrated III-V-on-LN device. (f) Detected electroluminescence spectrum of the heterogeneously integrated III-V-on-LN broadband light sources. (e) and (f) Reprinted from Ref. 144, © 2022 Optica.
Experimentally, the gain performance of the III/V-on-LN amplifier was characterized first under different bias currents with a fixed input power of
More recently, Zhang et al. demonstrated a heterogeneous integration of III-V active device on LNOI waveguide by adhesive bonding, as shown in Fig. 12(e).144 An electroluminescence spectrum with a 3-dB bandwidth of 40 nm centered at 1600 nm was observed, as shown in Fig. 12(f). Moreover, due to selecting the InP-based III-V material, the active devices can also function as a photodetector. A peak responsivity of
The electrically pumped lasers and amplifiers have the characteristics of portability, which is more conducive to the application out of the laboratory and can eliminate the influence of doping on non-gain area devices, which is a beneficial supplement to the optically pumped LNOI light sources. Table 3 summarizes the main parameters of LNOI electrically pumped lasers reported so far. Hybrid integration, heterogeneous integration, and microtransfer printing have their advantages and limitations. For example, with the help of commercial mature semiconductor single-frequency lasers or amplifiers and the fabricated low-loss LNOI devices, as well as the introduction of end-coupler design and fine adjustment and alignment before final packaging, hybrid integrated electrically pumped lasers can obtain narrow linewidth and high output power. The disadvantage is that hybrid integration requires high-precision alignment tools and can only integrate a single device at a time, which increases the cost of integrated devices to some extent and is therefore more suitable for initial prototype exploration. On the other hand, the heterogeneous integration and microtransfer printing technology can realize wafer-scale preparation and effectively lead to high throughput. However, due to the complexity of the preparation process, the whole process is still in the research and development stage. Inconsistent thermal diffusivity and unmatched refractive index of different film layers result in a low yield of products, especially for heterogeneous integrated products. In addition, the microtransfer-printing process is complex and requires high alignment accuracy (
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As can be seen from the above introduction, various lasers and amplifiers based on the LNOI platform have been demonstrated by doping REIs or integrating III-V gain materials. Nevertheless, the two gain introduction schemes have their advantages and disadvantages. Specifically, compared with III-V gain media, REI-doped materials have a long excited-state lifetime and less refractive index change, resulting in relatively higher temperature stability, lower noise figure, and narrower laser linewidth for the REI-doped laser and amplifier. For example, 4 Hz of the fundamental linewidth of lasers based on erbium-doped silica microtoroid cavity has been demonstrated.148 Therefore, lasers and amplifiers based on REI-doped LNOI are more suitable for on-chip coherent communication, quantum optics, and other related applications. Another advantage of the REIs-doped LNOI lasers and amplifiers is that the fabrication process is simple and compatible with the CMOS process, which promises to be scalable, low-cost, and amenable to mass production. But the output power for the REI-doped LNOI lasers and amplifiers is still at a low level (
4 Application Prospects of LNOI-Based Lasers and Amplifiers
Based on the realization of the long-awaited active light source, a series of promising applications are expected to be carried out based on the platform of REI-doped LN film. This section discusses the application fields of combining on-chip light sources with other LNOI functional devices, including sensors, electro-optic modulators, frequency converters, and microcavity combs.
4.1 Sensing Based on LNOI Light Sources
WGM microcavity has a high
4.2 Broadband Optical Communication
The optical transmitter is an essential building block in optical communication applications, and its critical component is the modulator module. Electro-optic modulators based on LNOI have been developed and shown noticeable advantages in driving voltage, bandwidth, linearity, and excitation ratio. However, due to the inherent luminescence difficulties of LN materials, the lack of an on-chip integrated light source, especially the electrically pumped high-power light source, is considered the main obstacle for applying the LNOI modulator to the optical transmitter. With the development of LN thin-film lasers, electrically pumped high-power lasers have become possible, effectively overcoming this limitation. In the future, an LN thin-film optical transmitter with low power consumption and high performance is expected to play an important role in data centers. In addition, to further increase the capacity of optical communication, the broadband tunable laser sources realized on the LNOI platform were expected to combine with the on-chip electro-optical modulator and wavelength division multiplexer153 for the construction of a multichannel wavelength division multiplexer emitter, which is helpful to achieve ultrabroadband optical fiber communication and reduce the communication costs.
4.3 Frequency Converter Based on LNOI Active Light Source
It can be seen from Tables 1 and 3 that the reported lasers are mainly concentrated in the 1550- and 1060-nm bands. In addition, a single type of REI or semiconductor gain medium has a limited gain bandwidth (
4.4 Chip-Based Microcombs
Optical frequency combs have attracted wide attention due to their application in optical clocks, metrology, and spectroscopy. Especially in recent years, the optical comb generated in the WGM microresonators, referred to as microcombs, has the excellent characteristics of low power consumption, high repetition rate, and on-chip integration compatibility, which endows the optical frequency comb with a new generation mechanism and application range. The LN has excellent third-order nonlinear and electro-optical effects. The soliton microcomb19 and broadband electro-optic frequency comb based on the LN platform have been confirmed, which shows the feasibility of the LN thin-film platform to generate an optical microcomb. In addition, based on the unique electro-optic effect of LN, the generation and modulation of an optical microcomb can be realized simultaneously on a monolithic chip, which can expand the application field of microcombs, such as programmable pulse shaping and coherent microwaves processing.156,157 With the development of LN thin-film laser sources, the combination of laser and high-quality Kerr microcavity is a promising way to realize the miniaturization and integration of the microcomb system, which can enhance the portability of the microcomb and expand its application scenarios, such as parallel coherent lidar. Some research routes can refer to the development of a silicon nitride-based integrated optical microcomb. For example, electrically pumped soliton frequency combs are generated by hybrid integrating semiconductor amplifiers or lasers with passive silicon nitride chips.158
5 Conclusion
In this review, the current research progress on lasers and amplifiers based on LN thin-film platforms was reviewed comprehensively. Specifically, in the section on optical pumping laser and amplifier realized by REI doping, several mainstream ways of introducing REIs into LN were introduced, and their advantages and disadvantages were discussed. Then the fluorescence spectrum research of REIs based on the LNOI platform was introduced. Then, vital parameters of the WGMs microlasers, such as threshold and conversion efficiency, were analyzed. On this basis, the research progress on microdisks, microrings, and single-mode lasers on the REI-doped LNOI platform is introduced. At the same time, the research on the REI-doped LNOI amplifiers was also reviewed. The limitations and improvement measures of the current optically pumped lasers and amplifiers were also discussed. On the other hand, in the section on LNOI electrically pumped III-V lasers and amplifiers, several mainstream mechanisms of introducing III-V gain materials into the current integrated photonics platform, namely, hybrid integration, heterogeneous integration, and microtransfer printing, were introduced in detail. The research progress on LNOI electrically pumped III-V lasers and amplifiers was reviewed. On this basis, the restrictions and improvement schemes for the current realization of electrically pumped lasers and amplifiers were explored in depth. Then the advantages and disadvantages of the two routes to realizing LNOI lasers and amplifiers were also discussed. Finally, the application scenarios based on the combination of an LNOI-based light source and other excellent device-based LN thin-film platforms, such as sensing, frequency conversion, and on-chip optical communication, were envisioned.
In addition to the rapid development of various photoelectric devices of LN thin-film platforms, the realization of on-chip light sources will undoubtedly make the LN thin-film platform achieve a high degree of integration. At the same time, detectors based on Si,165 black phosphorus,166,167 and superconducting nanowires168,169 have been proven on the LNOI platform, demonstrating the feasibility of integrated photodetectors. Furthermore, the experience of heterogeneously integrated III-V photodetectors based on Si-based photonics can also be transferred into the LN thin-film platform and is expected to achieve high detector bandwidth.170
Figure 13.Schematic diagram of integrated optical chips based on LN thin film. SOA, semiconductor optical amplifier; RDFA, rare-earth-doped waveguide amplifier; PD, photodetector; and SHG, second-harmonic generation.
Qiang Luo received his BS degree from Shangqiu Normal University in 2017. Currently, he is a PhD student at TEDA Institute of Applied Physics, Nankai University. His research interests include microlasers and amplifiers based on lithium niobate thin-film platforms.
Fang Bo received his BS (also BE) and PhD degrees from Nankai University in 2002 and 2007, respectively. Currently, he is working as a professor at Nankai University. From 2013 to 2014, he was working as a visiting scholar at Washington University in St. Louis. His research interests include micro-/nano-optics, quantum optics, and nonlinear optics, in particular, fabrication and nonlinear effects of on-chip lithium niobate resonators.
Yongfa Kong received his BS and MS degrees from Nankai University and PhD degree from the School of Material Science and Engineering of Tianjin University. Currently, he is working as a professor of physics at Nankai University in China. He has worked at the School of Physics of Nankai University since 1999 following postdoctoral appointments at the Photonics Center of Nankai University. His research interests are diverse and cover the physics and devices of nonlinear optical and photonic materials.
Guoquan Zhang received his bachelor’s degree in 1993, the master’s degree in 1995 in condensed matter physics, and the PhD in condensed matter physics from Nankai University, Tianjin, China. Currently, he is working as a professor at Nankai University. His research interests include nonlinear optics and quantum optics.
Jingjun Xu received his BS degree in solid-state physics and PhD in condensed matter physics from Nankai University in 1988 and 1993, respectively. Currently, he is working as a professor at the School of Physics at Nankai University. He is the founding director of the Ministry of Education Key Laboratory of Weak-Light Nonlinear Photonics. His research interests include nonlinear photonic materials and physics and their application in information technology.
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Qiang Luo, Fang Bo, Yongfa Kong, Guoquan Zhang, Jingjun Xu, "Advances in lithium niobate thin-film lasers and amplifiers: a review," Adv. Photon. 5, 034002 (2023)
Category: Reviews
Received: Dec. 10, 2022
Accepted: Apr. 26, 2023
Published Online: Jun. 2, 2023
The Author Email: Bo Fang (bofang@nankai.edu.cn)