Two- and three-photon absorption of the ferrocene derivative containing fluorene based on the quantum impedance Lorentz oscillator

Xiaofeng Wang; Meng Liu; Yu Yu; Yulei Wang; Yong Zhang; Yuanqin Xia; Peide Zhao

doi:10.3788/IRLA20230410

Infrared and Laser Engineering, Volume. 52, Issue 12, 20230410(2023)

Two- and three-photon absorption of the ferrocene derivative containing fluorene based on the quantum impedance Lorentz oscillator

Xiaofeng Wang¹, Meng Liu¹, Yu Yu^2,3, Yulei Wang^2,3, Yong Zhang^1,3, Yuanqin Xia^2,3、*, and Peide Zhao^1,3、*

Author Affiliations

¹School of Science, Hebei University of Technology, Tianjin 300401, China

²Center of Advanced Laser Technology, Hebei University of Technology, Tianjin 300401, China

³Hebei Key Laboratory of Advanced Laser Technology and Equipment, Tianjin 300401, China

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Fig. 1. Interaction diagram between photon and the outermost electron of a hydrogen-like atom

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Fig. 2. Numerical simulation of single-, two-, and three-photon absorption of R=NO₂-fluorene-containing ferrocene derivative based on QILO. (a) Molecular structure; (b) Fitting diagram of linear absorption spectrum based on QILO; (c) Molecular 2PA cross section based on QILO (blue line); (d) Molecular three-photon-absorption cross section based on QILO

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Fig. 3. Influence between 2PA and 3PA of R=NO₂-fluorene-containing ferrocene derivative based on the QILO. (a) Molecular 2PA cross-section; (b) The imaginary part of the third-order electropolarization; (c) Molecular 3PA cross-section; (d) The imaginary part of the fifth-order electropolarization

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Table 1. Theoretical and experimental results of 2PA and 3PA cross sections of R=NO₂-fluorene-containing ferrocene derivative based on QILO model

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Table 1. Theoretical and experimental results of 2PA and 3PA cross sections of R=NO₂-fluorene-containing ferrocene derivative based on QILO model

Method	$\begin{array}{l}{\sigma }_{2} /\times1{0}^{-20}\;{ {\rm{cm} } }^{4}\cdot{ {\rm{GW} } }^{-1}\end{array}$	$\begin{array}{l}{\sigma }_{3}/\times1{0}^{-25}\;{ {\rm{cm} } }^{6}\cdot{ {\rm{GW} } }^{-2}\end{array}$
Method	793 nm	1260 nm	1314 nm
Experiment	0.40	3.00	2.45
Theory	0.49	2.01	1.00

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Xiaofeng Wang, Meng Liu, Yu Yu, Yulei Wang, Yong Zhang, Yuanqin Xia, Peide Zhao. Two- and three-photon absorption of the ferrocene derivative containing fluorene based on the quantum impedance Lorentz oscillator[J]. Infrared and Laser Engineering, 2023, 52(12): 20230410

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Paper Information

Category:

Received: Jul. 5, 2023

Accepted: --

Published Online: Feb. 23, 2024

The Author Email: Xia Yuanqin (xiayq@hebut.edu.cn)

DOI:10.3788/IRLA20230410

Topics

laser devices and laser physics

Lasers and Laser Optics

Laser physics

laser manufacturing

Instrumentation, Measurement and Metrology

Table 1. Theoretical and experimental results of 2PA and 3PA cross sections of R=NO2-fluorene-containing ferrocene derivative based on QILO model

Table 1. Theoretical and experimental results of 2PA and 3PA cross sections of R=NO2-fluorene-containing ferrocene derivative based on QILO model

Table 1. Theoretical and experimental results of 2PA and 3PA cross sections of R=NO₂-fluorene-containing ferrocene derivative based on QILO model

Table 1. Theoretical and experimental results of 2PA and 3PA cross sections of R=NO₂-fluorene-containing ferrocene derivative based on QILO model