Acta Optica Sinica, Volume. 39, Issue 8, 0801001(2019)

Measuring Vertical Profile and Vertical Column Density of SO2 in Troposphere by Multi-Axis Differential Optical Absorption Spectroscopy

Fusheng Mou, Jing Luo*, Suwen Li**, Wei Shan, Minhong Wei, and Xude Wang
Author Affiliations
  • School of Physics and Electronic Information, Huaibei Normal University, Huaibei, Anhui 235000, China
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    Figures & Tables(9)
    Retrieval results under elevation of 2° on December 28th, 2013. (a) Retrieval result of SO2; (b) retrieval error at different wavelengths
    Retrieval results of O4 and SO2 under elevation of 3° on December 28th, 2013. (a) Differential optical depth of O4; (b) differential optical depth of SO2; (c) retrieval residual of O4; (d) retrieval residual of SO2
    Retrieval results of VCD of tropospheric SO2. (a) AOD retrieved by MAX-DOAS; (b) measured aerosol profiles and typical aerosol profiles are used as input to obtain VCD of tropospheric SO2
    Retrieval example of SO2 vertical profiles. (a) Priori profile and retrieved profile; (b) comparison between measured result and simulated result
    Temporal series profiles of SO2 vertical column concentration based on MAX-DOAS retrieval
    Correlation analysis on retrieval and measured values of SO2 differential slant column density
    Temporal series profiles of SO2 volume fractions during December 27-31, 2013
    Comparison of SO2 concentration (0-100 m) measured by MAX-DOAS and point instrument results. (a) Hourly mean values; (b) daily mean values
    • Table 1. Settings used for O4 and SO2 retrievals

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      Table 1. Settings used for O4 and SO2 retrievals

      ParameterData sourceFitting interval
      337-370 nm (O4)307-330 nm (SO2)
      NO2Vandaele, et al.(1998) 220 K, 294 K[21]IncludedIncluded(only 294 K)
      SO2Bogumil, et al.(2003) 293 K[22]Included
      O3Bogumil, et al.(2003) 223 K, 243 K[22]IncludedIncluded
      O4Hermans, et al.(2003) 296 K[23]Included
      HCHOMeller and Moortgat (2000) 298 K[24]Included
      RingChance and Spurr(1997)[25]IncludedIncluded
      Polynomial degree55
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    Fusheng Mou, Jing Luo, Suwen Li, Wei Shan, Minhong Wei, Xude Wang. Measuring Vertical Profile and Vertical Column Density of SO2 in Troposphere by Multi-Axis Differential Optical Absorption Spectroscopy[J]. Acta Optica Sinica, 2019, 39(8): 0801001

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    Paper Information

    Category: Atmospheric Optics and Oceanic Optics

    Received: Feb. 13, 2019

    Accepted: Apr. 8, 2019

    Published Online: Aug. 7, 2019

    The Author Email: Luo Jing (ljmfs0926@163.com), Li Suwen (swli@chnu.edu.cn)

    DOI:10.3788/AOS201939.0801001

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