Infrared and Laser Engineering, Volume. 50, Issue 2, 20200342(2021)

Nonlinear optics and ultrafast dynamics characteristics of CdTe/CdS quantum dots with different core sizes and shell thickness

Qing Chang1, Hengyu Tan2,3, and Tianming Meng3
Author Affiliations
  • 1College of Media Engineering, Communication University of Zhejiang, Hangzhou 310018, China
  • 2Beijing Institute of Metrology, Beijing 100029, China
  • 3College of Electronic Engineering, Heilongjiang University, Harbin 150080, China
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    Figures & Tables(14)
    Absorption spectra of the CdTe/CdS quantum dots
    Open/closed aperture Z-scan normalized transmittance curves of water-soluble CdTe/CdS, S1-S2 quantum dots
    Open/closed aperture Z-scan normalized transmittance curves of water-soluble CdTe/CdS, S3-S4 quantum dots
    Open/closed aperture Z-scan normalized transmittance curves of water-soluble CdTe/CdS, S5-S6 quantum dots
    Transient absorption spectra of water-soluble CdTe/ CdS, S1-S2 quantum dots
    Transient absorption spectra of water-soluble CdTe/ CdS, S3-S4 quantum dots
    Transient absorption spectra of water-soluble CdTe/ CdS, S5-S6 quantum dots
    Ultrafast kinetic curves of water-soluble CdTe/CdS, S1-S2 quantum dots
    Ultrafast kinetic curves of water-soluble CdTe/CdS, S3-S4 quantum dots
    Ultrafast kinetic curves of water-soluble CdTe/CdS, S5-S6 quantum dots
    Transient absorption spectrum of the solvent water
    • Table 1. Six kinds of the CdTe/CdS core-shell quantum dots

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      Table 1. Six kinds of the CdTe/CdS core-shell quantum dots

      Sample numberQuantum dotsSize /nmCore colorCladding time
      S1CdTe/CdS-13.2Orange30 min
      S2CdTe/CdS-23.3orange1 h
      S3CdTe/CdS-33.0Yellow30 min
      S4CdTe/CdS-43.1Yellow1 h
      S5CdTe/CdS-52.6Green30 min
      S6CdTe/CdS-62.7Green1 h
    • Table 2. Nonlinear optical parameters obtained from Z-scan measurement data for CdTe/CdS quantum dots

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      Table 2. Nonlinear optical parameters obtained from Z-scan measurement data for CdTe/CdS quantum dots

      Sample nameCore colorShellSize/nmβ/10-13 m·W-1n2/10−12esu χ3/10−14esu
      S1OrangeCdS-30 min3.24.391.423.85
      S2OrangeCdS-1 h3.35.011.494.12
      S3YellowCdS-30 min3.05.071.383.90
      S4YellowCdS-1 h3.15.291.854.92
      S5GreenCdS-30 min2.65.231.183.58
      S6GreenCdS-1 h2.76.421.734.92
    • Table 3. CdTe/CdS quantum dots fitting parameters

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      Table 3. CdTe/CdS quantum dots fitting parameters

      Sample nameSizeτ-rise/ps τ1/ps τ2/ps
      S13.20.341.0617.81
      S23.30.331.9818.43
      S33.00.351.1313.79
      S43.10.592.1338.24
      S52.60.311.7412.77
      S62.70.321.7916.78
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    Qing Chang, Hengyu Tan, Tianming Meng. Nonlinear optics and ultrafast dynamics characteristics of CdTe/CdS quantum dots with different core sizes and shell thickness[J]. Infrared and Laser Engineering, 2021, 50(2): 20200342

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    Paper Information

    Category: Lasers and laser optics

    Received: Oct. 6, 2020

    Accepted: --

    Published Online: Mar. 22, 2021

    The Author Email:

    DOI:10.3788/IRLA20200342

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