Chinese Optics Letters, Volume. 17, Issue 3, 032601(2019)

Enhanced nonlinearity for filamentation in gold-nanoparticle-doped water

Shuai Yuan1, Lirong Wang1, Fengjiang Liu2, Fengquan Zhou1, Min Li1, Hui Xu1, Yuan Nie1, Junyi Nan2, and Heping Zeng1,2、*
Author Affiliations
  • 1Shanghai Key Laboratory of Modern Optical System, Engineering Research Center of Optical Instrument and System, Ministry of Education, School of Optical-Electrical and Computer Engineering, University of Shanghai for Science and Technology, Shanghai 200093, China
  • 2State Key Laboratory of Precision Spectroscopy, East China Normal University, Shanghai 200062, China
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    Figures & Tables(5)
    Schematic diagram of the experimental setup. The laser pulses were focused by a fused silica lens F1 (f=21 cm) into pure water and doped water. Filament in the cuvette was imaged by a CCD camera with ND and bandpass filters in front. The output emission was collected and directed to a fiber-coupled spectrometer. VA, variable attenuator; CCD, charge-coupled device.
    Top views of light channel (top row) and the corresponding longitudinal white light intensity distribution in gold-nanoparticle-doped water (bottom row) with input pulse energy of (a), (b) 5.49 μJ and (c), (d) 9.86 μJ and in pure water with pulse energy of (e), (f) 9.72 μJ.
    Starting position of multifilaments as a function of P/Pcr (input power divided by critical power) in gold-nanoparticle-doped water. Solid squares, experimental results; red line, simulations. We take Pcr=0.5 MW for the critical power of self-focusing in doped water by considering the results in Table 1.
    Spectra obtained for the propagation of the laser pulse in gold-nanoparticle-doped water (green and dark yellow solid curves) as compared with those in pure water (pink and red solid curves) under (a) low and (b) high average input energy. The spectra are normalized to the intensity of the signal at 800 nm.
    • Table 1. Measured Critical Power (Pcr) and Nonlinear Refractive Index (n2) in Gold-nanoparticle-doped Water and Pure Water Under Different Input Pulse Energy

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      Table 1. Measured Critical Power (Pcr) and Nonlinear Refractive Index (n2) in Gold-nanoparticle-doped Water and Pure Water Under Different Input Pulse Energy

       Pulse Energy (μJ)Critical Power Pcr (MW)Nonlinear Refractive Index n2(cm2/W)
      Doped water5.490.4815.0×1016
      Doped water9.860.5313.6×1016
      Pure water9.722.353.04×1016
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    Shuai Yuan, Lirong Wang, Fengjiang Liu, Fengquan Zhou, Min Li, Hui Xu, Yuan Nie, Junyi Nan, Heping Zeng. Enhanced nonlinearity for filamentation in gold-nanoparticle-doped water[J]. Chinese Optics Letters, 2019, 17(3): 032601

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    Paper Information

    Category: Physical Optics

    Received: Oct. 17, 2018

    Accepted: Dec. 7, 2018

    Posted: Dec. 13, 2018

    Published Online: Mar. 8, 2019

    The Author Email: Heping Zeng (hpzeng@phy.ecnu.edu.cn)

    DOI:10.3788/COL201917.032601

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