Chinese Optics Letters, Volume. 20, Issue 10, 100010(2022)

Large bandgap oscillations in two-dimensional Dion–Jacobson phase perovskites caused by coherent longitudinal acoustic phonons [Invited]

Fengke Sun, Boning Wu*, and Shengye Jin**
Author Affiliations
  • Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, China
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    Figures & Tables(4)
    Cross-sectional SEM images of the (DMAPA)PbI4 films.
    (a) Scheme of TA experiments; (b) 2D contour plot of TA spectra; (c) ΔA spectra at selected time delays; (d) dependence of oscillation period and amplitude on film thickness; (e) dependence of oscillation period and amplitude on pump photon energy; (f) elucidating the origin of TA bandgap oscillation.
    (a) Scheme of front-face TR experiments; (b) 2D contour plot of TR spectra; (c) time-dependent ΔR/R at selected wavelengths; (d) dependence of oscillation period on wavelength of probe light; (e) elucidating the origin of oscillation observed in TR experiments.
    (a) Scheme of BTR experiments; (b) 2D contour plot of BTR spectra; (c) time-dependent ΔR/R at selected wavelengths; (d) time when the CLAP arrives at air–perovskite interfaces for films of different thicknesses; (e) elucidating the origin of oscillation, and the CLAP arrival time observed in BTR experiments.
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    Fengke Sun, Boning Wu, Shengye Jin. Large bandgap oscillations in two-dimensional Dion–Jacobson phase perovskites caused by coherent longitudinal acoustic phonons [Invited][J]. Chinese Optics Letters, 2022, 20(10): 100010

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    Paper Information

    Special Issue: ULTRAFAST OPTICS: FUNDAMENTALS AND APPLICATIONS

    Received: Aug. 19, 2022

    Accepted: Sep. 8, 2022

    Published Online: Oct. 13, 2022

    The Author Email: Boning Wu (boning@dicp.ac.cn), Shengye Jin (sjin@dicp.ac.cn)

    DOI:10.3788/COL202220.100010

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