Journal of Inorganic Materials, Volume. 39, Issue 6, 634(2024)

Research Progress of High Thermal Conductivity Silicon Nitride Ceramics Prepared by Non-oxide Sintering Additives

Weiming WANG1... Weide WANG1,2,*, Yi SU1, Qingsong MA1, Dongxu YAO3 and Yuping ZENG3,* |Show fewer author(s)
Author Affiliations
  • 11. Science and Technology on Advanced Ceramic Fibers and Composites Laboratory, College of Aerospace Science and Engineering, National University of Defense Technology, Changsha 410073, China
  • 22. College of Advanced Interdisciplinary Studies, National University of Defense Technology, Changsha 410073, China
  • 33. Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai 200050, China
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    Figures & Tables(19)
    Schematic of typical packaging of power semiconductor device[1]
    Schematic of the liquid phase sintering mechanism for Si3N4 ceramics[10]
    Effects of volume fraction of glassy phase, grain- boundary film thickness(δ), and grain size on the thermal conductivity of β-Si3N4[13]
    Effect of lattice oxygen content on the thermal conductivity of Si3N4 ceramics[17]
    Displacement-temperature curves of Si3N4 ceramics with MgF2 or MgO as sintering additives[19]
    XRD patterns of Si3N4 samples prepared with different LiF contents[20]
    Depolymerization mechanism of F atom in silicate melts[22]
    SEM morphologies of the polished surfaces of Si3N4 ceramics after gas pressure sintering (GPS) with different additives added[24]
    Typical HRTEM images of Si3N4 ceramics added with Y2O3 (a) and Y2Si4N6C (b) as additives[31]
    Curves of relative displacement of the as-pressed specimens with temperature variation[32]
    Densification mechanism of Si3N4 ceramics with ZrSi2-MgO additive[36]
    Shrinkage curves of the Si3N4 ceramics[10]
    Schematic illustration of Si3N4-Y2O3-SiO2 phase at 1900 ℃[10]
    STEM-EDS characterizations of Si3N4 ceramics with the addition of ZrO2 and ZrH2[47]
    SEM images on the fracture surfaces of nitrided samples (a, b) and post-sintered samples (c, d) without (a, c) and with (b, d) graphite powder bed addition[57]
    TEM images of PDA-coated powder and schematic of Si3N4-C core-shell structure[59-60]
    (a) Shrinkage behaviors and densification mechanism of Si3N4 ceramics during sintering, and (b) relationship between β phase ratio and relative density[62]
    Evolution of microstructure and diameter of Si3N4 ceramics[10]
    • Table 1. Properties of ceramic substrate materials[2]

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      Table 1. Properties of ceramic substrate materials[2]

      MaterialThermal conductivity/(W·m-1·K-1) Fracture toughness/(MPa·m1/2) Bending strength/MPa
      Al2O318-243.5-4.0300-400
      AlN150-2703.0-3.5220-310
      ZTA284.5650
      Si3N480-1776.5-7.5600-800
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    Weiming WANG, Weide WANG, Yi SU, Qingsong MA, Dongxu YAO, Yuping ZENG. Research Progress of High Thermal Conductivity Silicon Nitride Ceramics Prepared by Non-oxide Sintering Additives[J]. Journal of Inorganic Materials, 2024, 39(6): 634

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    Paper Information

    Category:

    Received: Nov. 14, 2023

    Accepted: --

    Published Online: Jul. 31, 2024

    The Author Email: WANG Weide (nudtwwd@163.com), ZENG Yuping (yuping-zeng@mail.sic.ac.cn)

    DOI:10.15541/jim20230530

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