Journal of Inorganic Materials, Volume. 37, Issue 1, 72(2022)

4-Chlorobenzylamine-based 2D/3D Perovskite Solar Cells

Xinyue YANG*... Qingshun DONG, Weidong ZHAO and Yantao SHI |Show fewer author(s)
Author Affiliations
  • State Key Laboratory of Fine Chemicals, Department of Chemistry, School of Chemical Engineering, Dalian University of Technology, Dalian 116024, China
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    Figures & Tables(13)
    Water contact angle measurements of (a) 3D and (b) 2D/3D perovskite films
    (a) XRD patterns of 3D and 2D/3D perovskite films, and (b) XRD pattern of 2D perovskite film
    Tauc plots of the perovskite films, the optical bandgap is 1.62 eV
    GIWAXS patterns of (a, c) 3D and (b, d) 2D/3D perovskite films with incident angles of (a, b) 0.1° and (c, d)1°
    Top-view SEM images of (a) 3D and (b) 2D/3D perovskite films, cross-sectional SEM images of (c) 3D-PSCs and (d) 2D/3D-PSCs
    Statistics of the PCE for PSCs, processed by 4-CBAI treatment with various concentrations of 0, 0.5, 1.0, and 1.5 mg·mL-1
    (a) UV-Vis absorption, PL spectra and (b) TRPL decay curves of 3D and 2D/3D perovskite films
    J-V curve of flexible PSCs based on 2D/3D perovskite
    Stabilized PCE and photocurrent density curves at the maximum power point for the flexible PSCs based on 2D/3D perovskite
    (a) Schematic diagram of 2D/3D-PSCs structure, (b) J-V curves (reverse and forward scans), (c) EQE spectra with the corresponding integrated current densities, and (d) stabilized PCE curves at the maximum power point for 3D-PSCs and 2D/3D-PSCs
    (a) Thermal stability of 3D-PSCs and 2D/3D-PSCs under 85 ℃ in air (relative humidity: 40%-70%), and (b) light stability of 3D-PSCs and 2D/3D-PSCs under continuous 1 sun illumination in N2
    • Table 1. TRPL fitting results of 3D and 2D/3D perovskite films

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      Table 1. TRPL fitting results of 3D and 2D/3D perovskite films

      Sampleτ1/ns A1τ2/ns A2τave/ns
      3D2.550.7117.260.3013.49
      2D/3D4.750.5324.860.4321.02
    • Table 2. Detailed photovoltaic parameters of 3D-PSCs and 2D/3D-PSCs

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      Table 2. Detailed photovoltaic parameters of 3D-PSCs and 2D/3D-PSCs

      SampleScan methodVOC/V JSC/(mA·cm-2) FF/% PCE/%
      3DReverse1.1123.1772.7418.70
      Forward1.0823.1871.8518.06
      2D/3DReverse1.1723.4576.3920.88
      Forward1.1623.4475.0720.41
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    Xinyue YANG, Qingshun DONG, Weidong ZHAO, Yantao SHI. 4-Chlorobenzylamine-based 2D/3D Perovskite Solar Cells[J]. Journal of Inorganic Materials, 2022, 37(1): 72

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    Paper Information

    Category: EDITORIAL

    Received: Mar. 25, 2021

    Accepted: --

    Published Online: Sep. 23, 2022

    The Author Email: YANG Xinyue (yangxinyue@mail.dlut.edu.cn)

    DOI:10.15541/jim20210199

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