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Journal of Inorganic Materials, Volume. 36, Issue 10, 1053(2021)

Fe-Co-K/ZrO2 Catalytic Performance of CO2 Hydrogenation to Light Olefins

Qiang LIU... Jie DING*, Guojing JI, Juanmin HU, Hao GU and Qin ZHONG* |Show fewer author(s)
Author Affiliations
  • School Chemistry and Chemical Engineering, Nanjing University of Science and Technology, Nanjing 210094, China
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    Figures & Tables(13)
    CO2 conversion (a) and light olefins selectivity (b) of CO2 hydrogenation by x-FCK/ZrO2 at different temperatures and catalytic production distribution of x-FCK/ZrO2 at 300 ℃(c) Colorful images are available on website
    1. CO2 conversion (a) and light olefins selectivity (b) of CO2 hydrogenation by x-FCK/ZrO2 at different temperatures and catalytic production distribution of x-FCK/ZrO2 at 300 ℃(c) Colorful images are available on website

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    Stability experiments of 0-FCK/ZrO2 and 0.3-FCK/ZrO2
    2. Stability experiments of 0-FCK/ZrO2 and 0.3-FCK/ZrO2

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    TEM images of 0-FCK/ZrO2 (a,b) and 0.3-FCK/ ZrO2 (c,d)
    3. TEM images of 0-FCK/ZrO2 (a,b) and 0.3-FCK/ ZrO2 (c,d)

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    XRD patterns of the calcined (a) and reduced (b) catalysts
    4. XRD patterns of the calcined (a) and reduced (b) catalysts

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    H2-TPR spectra of catalysts with different K contents
    5. H2-TPR spectra of catalysts with different K contents

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    CO2-TPD spectra of the catalysts with different K contents
    6. CO2-TPD spectra of the catalysts with different K contents

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    XPS spectra of Fe2p over 0-FCK/ZrO2 and 0.3-FCK/ZrO2
    7. XPS spectra of Fe2p over 0-FCK/ZrO2 and 0.3-FCK/ZrO2

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    In-situ DRIFTS of 0-FCK/ZrO2 (a) and 0.3-FCK/ZrO2 (b) with pure CO2 introduced, and in-situ DRIFTS of 0-FCK/ZrO2 (c) and 0.3-FCK/ZrO2 (d) with CO2 and H2 introduced
    8. In-situ DRIFTS of 0-FCK/ZrO2 (a) and 0.3-FCK/ZrO2 (b) with pure CO2 introduced, and in-situ DRIFTS of 0-FCK/ZrO2 (c) and 0.3-FCK/ZrO2 (d) with CO2 and H2 introduced

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    Mass spectra for the 0.3-FCK/ZrO2 of reactive production
    S1. Mass spectra for the 0.3-FCK/ZrO2 of reactive production

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    SEM-EDS analyses of 0-FCK/ZrO2 (a-c) and 0.3-FCK/ZrO2 (d-g)
    S2. SEM-EDS analyses of 0-FCK/ZrO2 (a-c) and 0.3-FCK/ZrO2 (d-g)

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    XPS spectra of Co2p over 0-FCK/ZrO2 (a) and 0.3-FCK/ZrO2 (b)
    S3. XPS spectra of Co2p over 0-FCK/ZrO2 (a) and 0.3-FCK/ZrO2 (b)

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    XRD patterns of the catalysts after reaction for 85 h
    S4. XRD patterns of the catalysts after reaction for 85 h

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    H2-TPD spectra for x-FCK/ZrO2
    S5. H2-TPD spectra for x-FCK/ZrO2

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    Qiang LIU, Jie DING, Guojing JI, Juanmin HU, Hao GU, Qin ZHONG. Fe-Co-K/ZrO2 Catalytic Performance of CO2 Hydrogenation to Light Olefins [J]. Journal of Inorganic Materials, 2021, 36(10): 1053

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    Paper Information

    Category: RESEARCH ARTICLE

    Received: Jan. 25, 2021

    Accepted: --

    Published Online: Nov. 26, 2021

    The Author Email: DING Jie (tonlyjding@njust.edu.cn), ZHONG Qin (zq304@njust.edu.cn)

    DOI:10.15541/jim20210044

    Topics

    laser devices and laser physics
    Lasers and Laser Optics
    Laser physics
    laser manufacturing
    Instrumentation, Measurement and Metrology