Spectroscopy and Spectral Analysis, Volume. 42, Issue 4, 1036(2022)

Observation of Variations of Ambient CO2 Using Portable FTIR Spectrometer

Ling-ling ZHA1,*... Wei WANG2,2; *;, Yu XIE1,1;, Chang-gong SHAN2,2;, Xiang-yu ZENG2,2;, You-wen SUN2,2;, Hao YIN2,2; and Qi-hou HU2,2; |Show fewer author(s)
Author Affiliations
  • 11. Department of Automation, Hefei University, Hefei 230061, China
  • 22. Key Laboratory of Environmental Optics and Technology, Anhui Institute of Optics and Fine Mechanics, Hefei Institute of Material Sciences, Chinese Academy of Sciences, Hefei 230031, China
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    Figures & Tables(12)
    (a) Observing site (Science Island in the western suburb of Hefei); (b) Observing site (Environmental monitoring center of Shanghai); (c) FTIR spectrometer
    Amplitude modulation efficiency and phrase error of the spectrometer
    Typical spectral fitting and residuals of CO2 in two spectral windows near (a) 6 220 cm-1, (b) 6 339.5 cm-1
    Time series of retrieved Xair
    The time series of XCO2 observed in HefeiThe light blue circles represent individual measurements; the red circles represent daily average XCO2; the dark blue lines with blue triangles represent monthly average XCO2
    XCO2 observed by portable FTIR and high-resolution FTIR spectrometer in 2017
    Daily average of XCO2 measured by portable FTIR spectrometer plotted against the corresponding values of the high-resolution FTIR spectrometerThe line shows the best fit to the ratio of the two values
    XCO2 observed by GOSAT and portable FTIR spectrometerBlue circles are GOSAT data and orange triangle are FTIR data
    Scatter plot of XCO2 observed by GOSAT and portable FTIR spectrometer
    The time series of XCO2 observed in Hefei and ShanghaiThe black and red circles indicate the data observed in Hefei and Shanghai, respectively
    • Table 1. ME and PE values

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      Table 1. ME and PE values

      Distance/cmME/无量纲PE/rad
      3000.990.002
      4000.990.003
      5000.970.003
      6000.970.003
      Mean0.980.003
      Standard deviation0.013.02×10-4
    • Table 2. Spectral windows for retrieval of CO2 column

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      Table 2. Spectral windows for retrieval of CO2 column

      GasCenter of
      spectral
      Windows/cm-1
      Width
      /cm-1
      Interfering
      gases
      CO26 220.080.0H2O, HDO, CH4
      CO26 339.585.0H2O, HDO
      O27 885.0240.0H2O, HF, CO2
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    Ling-ling ZHA, Wei WANG, Yu XIE, Chang-gong SHAN, Xiang-yu ZENG, You-wen SUN, Hao YIN, Qi-hou HU. Observation of Variations of Ambient CO2 Using Portable FTIR Spectrometer[J]. Spectroscopy and Spectral Analysis, 2022, 42(4): 1036

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    Paper Information

    Category: Research Articles

    Received: Mar. 31, 2021

    Accepted: --

    Published Online: Jul. 25, 2023

    The Author Email: ZHA Ling-ling (llzha96@163.com)

    DOI:10.3964/j.issn.1000-0593(2022)04-1036-08

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