Recently, the concepts of parity–time (PT) symmetry and band topology have inspired many novel ideas for light manipulation in their respective directions. Here we propose and demonstrate a perfect light absorber with a PT phase transition via coupled topological interface states (TISs), which combines the two concepts in a one-dimensional photonic crystal heterostructure. By fine tuning the coupling between TISs, the PT phase transition is revealed by the evolution of absorption spectra in both ideal and non-ideal PT symmetry cases. Especially, in the ideal case, a perfect light absorber at an exceptional point with unidirectional invisibility is numerically obtained. In the non-ideal case, a perfect light absorber in a broken phase is experimentally realized, which verifies the possibility of tailoring non-Hermiticity by engineering the coupling. Our work paves the way for novel effects and functional devices from the exceptional point of coupled TISs, such as a unidirectional light absorber and exceptional-point sensor.
1. INTRODUCTION
Topological interface states (TISs) in photonic heterostructures composed of two 1D photonic crystals (PCs) with different bulk band topologies have attracted researchers’ considerable interest [1–6]. It has been shown that a quantized number called the Zak phase assigned to every band can be defined for PCs with inversion symmetry, and the Zak phases between two bands can be exchanged with a topological transition [7,8]. It is worth mentioning that the topological transition in PCs can also be revealed with the transition between two effective single negative media [9,10] in the bandgap. In practice, different band topologies can be related to the sign of the reflection phase for the gap [11–14]. TIS can greatly enhance light–matter interaction including enhancement of nonreciprocal radiation [15,16], as its smaller mode volume leads to an increased Purcell factor [17]. For instance, strongly coupled TISs have been theoretically investigated to achieve multi-band perfect absorption [18,19] and strong Rabi splitting [20]. Very recently, TISs have been used to explore high-order topological properties with synthetic dimensions [21].
On the other hand, since Bender et al. [22] proposed a class of non-Hermitian Hamiltonians whose real spectra can be ensured by parity–time (PT) symmetry [23], PT-symmetric systems have been widely investigated in photonics [24], acoustics [25], circuits [26], and atom physics [27]. After the early observations of PT phase transitions in the field of optics [28,29], a variety of intriguing phenomena in optical PT-symmetric systems were exploited, including loss-induced revival of lasing [30], unidirectional propagation [31] and invisibility [32,33], negative refraction [34], coherent perfect absorption (CPA) [35,36], etc. The phase transition takes place at the so-called “exceptional point” (EP) [37], where not only eigenvalues merge with each other, but also their corresponding eigenvectors become completely parallel.
In recent years, many novel applications of PT-symmetric photonic structures have been proposed [38,39], such as a single mode laser [40,41] and a integrated orbital angular momentum microlaser [42]. Particularly, the advantages of the non-Hermitian degeneration (coalescence of both eigenvalues and eigenstates) at EP in detecting and sensing have attracted much attention [43–45], including single nanoparticle detection [46], microelectromechanical systems (MEMS)-based implantable wireless sensing [47,48], and weak nonlinearity sensing [49]. Very recently, based on an optical system of coupled whispering gallery mode microcavities, optical CPA at EP has been demonstrated [50].
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The combination of topology and non-Hermitian physics leads to many novel phenomena, including the non-Hermitian skin effect [51], recovery of topological zero mode [52], interplay with nonlinearity [53], etc. Recently, a flip-of-state phenomenon related to the topology of EP in a non-Hermitian system has been widely discussed [54,55]. Researchers have also investigated EP in topological systems such as a Kitaev chain [56] and quasiperiodic Aubry–Andre–Harper model [57]. Novel sensors [58] and new concepts of topological wireless power transfer [59,60] involving coupled topological states [61] have been proposed based on these findings. Given that topological states can greatly enhance light–matter interactions, the introduction of TISs into a PT-symmetric system working around EP is a straightforward approach to improve the performance of non-Hermitian photonic structures.
Nevertheless, there is a lack of experimental demonstration of perfect absorption at EP in topological photonic systems where the coupling strength between TISs is comparable to the dissipation.
In this paper, we propose and investigate a perfect light absorber (so called one-channel CPA [62]) with two coupled TISs. We calculate spectral responses for these TISs using coupled mode theory (CMT), which are consistent with numerical simulations obtained from the transfer matrix method (TMM). By carefully adjusting the scattering losses of TISs, a passive but ideal PT-symmetric system is achieved from the perspective of an effective Hamiltonian [36,63]. With a decrease in coupling between two TISs, the two perfect absorption peaks are preserved at the beginning but gradually get close to each other, until they merge at EP. After that, the absorption peak begins to decline. These featured spectral responses reveal the PT phase transition near EP. Also, unidirectional invisibility at EP is numerically obtained. Results in the non-ideal case are similar, except that the absorption peaks of coupled TISs in the PT-symmetric phase are not perfect, and the maximum value of absorption in the broken phase changes non-monotonically as coupling decreases. In particular, perfect light absorption can be observed with critical coupling in the PT-broken phase. We experimentally demonstrate such a perfect light absorber in the non-ideal case, which verifies the possibility of tailoring non-Hermiticity by engineering the coupling. Our work paves the way for novel effects and functional devices from EP of coupled TISs, such as a unidirectional light absorber and EP sensor.
2. EFFECTIVE HAMILTONIAN WITH PT SYMMETRY IN COUPLED TISs
The proposed PC structure with coupled TISs under normal incidence is shown in Fig. 1(a), which comprises , , and a silver layer . Layers and are titanium dioxide with a refractive index of , and are silicon dioxide with a refractive index of , and and are period numbers of and unit cells, respectively. The thicknesses of layers are designed to be , , , , and , respectively. The lengths of two unit cells are and . The band structures of () PC (whose unit cell is ) and () PC (whose unit cell is ) with corresponding Zak phases are illustrated in Figs. 1(b) and 1(c), respectively. One can see that two PCs in the first gaps have different topological orders. According to “bulk-interface correspondence” [8], TIS 1 at the interface between two PCs must emerge within the overlapping gap-frequency region (500–550 THz). Reflectance dips in Fig. 1(d) indicate that TIS 1 exists in . It is notable that the resonance frequency of TIS is slightly affected by the period number when is small, and it becomes independent of when is sufficiently large (). Similarly, for the TIS in , the frequency becomes independent of when is sufficiently large ().
Figure 1.(a) Schematic of sandwich structure with two coupled TISs. (b) Band structure of PC. Red stripe represents the first bandgap with positive reflection phase. The Zak phase of each band is displayed next to it, and the sum of Zak phases below the first gap is shown in parentheses. (c) Band structure of PC. Yellow stripe represents the first bandgap with negative reflection phase. (d) Reflectance for TIS 1 in . The blue solid, red dotted, black dashed, and green solid lines represent , 9, 7, and 6, respectively. (e) Reflectance for TIS 2 in . (f) Reflectance for coupled TISs in . The blue solid, red dotted, and black dashed lines represent , 13, and 15, respectively.
TIS also exists at the interface between metal and PC, also known as Tamm plasma polaritons, as long as the reflection phases and satisfy [2,11,64–67]. As indicated by the reflection dip in Fig. 1(e), TIS 2 emerges at the interface between the silver layer with negative reflection phase and with positive reflection phase in the first bandgap. Here, a Lorentz–Drude model is used for the dielectric constant of silver in TMM calculation [68], and TIS 1 and TIS 2 are engineered to have nearly the same resonance frequency of (corresponding vacuum wavelength is about 577 nm). The electric field distributions of two TISs are shown in Figs. 2(a) and 2(b), which clearly illustrate the strong localization of TISs.
Figure 2.Distribution of normalized electric field amplitude for different topological states. The yellow, red, gray, and white shaded areas represent the photonic crystal , , silver, and air background, respectively. (a) TIS 1 in . (b) TIS 2 in . (c), (d) Super-modes with (c) lower and (d) higher energy in with strong coupling. (e) Merged TISs in with critical coupling. (f) Merged TISs in with weak coupling. The red dashed lines represent the interfaces between different PCs and metal.
Now we discuss coupled TISs in the sandwich structure . As shown in Fig. 1(f), two dips in reflectance can be observed when , which indicates that the coupling of TISs leads to formation of two super-modes with different energies. Field distributions of the super-modes are shown in Figs. 2(c) and 2(d), where strong confinement of fields can be found near two interfaces. With the increase in period number , the two super-modes gradually approach and merge at the critical coupling strength. To better show how affects the coupling strength, the reflectance spectra for critical coupling (, red dotted line) and weak coupling (, black dashed line) are also given in Fig. 1(f). It is found that the reflection minimum increases with for greater than 13. The corresponding field distributions at resonance frequencies are shown in Figs. 2(e) and 2(f), respectively. It is seen that for greater than 13, the field amplitude of TIS 2 decreases quickly with , while for less than 13, there is very little change in the field amplitude of TIS 2. These spectral responses, as well as field distributions, are closely related to the PT phase transition at critical coupling (EP), which will be discussed in detail in the next section.
Spectral responses of the aforementioned structures can be well explained by CMT, and a PT-symmetric system can be achieved based on the analysis of CMT. Here, a TIS can be regarded as resonance mode , and the dynamic equation for a single resonance mode with single-port excitation based on the Lorentz model can be written as [69] where , , and are the resonance frequency, intrinsic loss, and amplitude of the input wave at port 1, respectively. () denotes scattering loss, which is determined by the coupling between TIS and input port 1 (output port 2). The reflection coefficient at port 1 is
The dynamic equations for coupled TISs in a sandwich structure (, ) can be described by CMT as follows [70]: where denotes the coupling rate between TISs and ; () denotes the coupling rate between TIS 1 (TIS 2) and port 1 (port 2). () denotes intrinsic loss. and denote resonance frequencies of TIS 1 and TIS 2, respectively. Here, for the chosen parameters, we have . From the equations above, the reflection coefficient can be written as
Considering the zero-reflection case , we obtain an eigenvalue equation from Eqs. (3) and (4) as where
The eigenvalues of are
It can be concluded that represents the effective Hamiltonian of the sandwich structure, in which can be regarded as an effective gain. The Hamiltonian becomes ideal PT symmetric when satisfying [61].
3. PERFECT LIGHT ABSORBER VIA COUPLED TISs WITH IDEAL PT SYMMETRY
Now we focus on the design of a PT-symmetric photonic structure with coupled TISs to realize perfect absorption. First, the model parameters in the effective Hamiltonian , which can be engineered by altering period numbers and , are extracted from fitting the spectral response with CMT. For the selected sandwich structure , the coupling rate between port 1 and TIS 1 (denoted as ) and intrinsic loss of TIS 2 (denoted as ) can be obtained independently from the resonance spectra of structures and . As shown in Figs. 3(a) and 3(b), within the interested frequency region, TMM-based calculation for the reflectance spectra of two TIS resonances in and can be well fitted using the Lorentz model in Eq. (2). Here, () denotes the coupling rate between TIS 1 and port 1 (port 2) in . () denotes the coupling rate between TIS 2 and port 1 (port 2) in . () denotes intrinsic loss of TIS 1 (TIS 2). Hence the model parameters for are derived as follows: , (), , (thickness of the silver layer is , which is thick enough to ensure TIS 2 is isolated from port 2), , . Specific methods to obtain these model parameters are given in Appendix A. It is obvious that the ideal PT symmetry condition () is almost satisfied in this design (). Further, by fitting the reflectance of the sandwich structure for different period numbers (), the relation between and is obtained as .
Figure 3.(a) Reflectance spectra of TIS 1 in calculated by TMM (blue solid line) and Lorentz model (red hexagonal points). (b) Same as in (a), but for TIS 2 in .
Then the eigenvalue spectra of the effective Hamiltonian versus can be calculated from Eq. (8) and are shown in Fig. 4(a) with red solid (real part) and black dashed (imaginary part) lines. The eigenvalues are a pair of conjugated complex numbers with weak coupling (), while with strong coupling (), the eigenvalues are two real numbers, which means that this ideal PT-symmetric non-Hermitian system has pseudo-Hermiticity in the PT-unbroken phase [71]. The case with is found to be very close to the phase transition EP (), at which two eigenvalues coalesce.
Figure 4.(a) Eigenvalue spectra of effective PT-symmetric system [] versus coupling rate (period number ) between two TISs. Blue circles represent absorption peaks with varied period numbers . (b) Reflectance and normalized electric field distribution of system for forward (F)/backward (B) propagation with . Red/blue line stands for forward/backward propagation. The layers at two ends are air layers.
TMM-based calculation for the absorption spectra of with different as well as the corresponding well-fitted CMT results is given in Fig. 5. According to analysis in Section 2, the frequencies of perfect absorption peaks can be regarded as real eigenvalues of the effective Hamiltonian . Hence, the PT phase transition in Fig. 4(a) can be demonstrated clearly in these absorption spectra. In Fig. 5(a), two perfect absorption peaks indicating a PT-symmetric phase can be found in a relatively strong coupling regime (). With the decrease in coupling rate, the frequencies of absorption peaks gradually get close to each other, which can be seen in Figs. 5(b) and 5(c) for the cases of , 11. They merge in the vicinity of in the case of , indicating the existence of EP. In the cases of , 14, the peak value of the absorption peak gradually decreases as increases, as shown in Figs. 5(e) and 5(f). In these cases, the system gets into the PT-broken phase. With the imaginary part of the eigenvalue increasing, the reflectance caused by mode-mismatch also increases, so the absorption drops accordingly. The frequencies of these absorption peaks from TMM with varying are illustrated in Fig. 4(a) with blue circles, which further indicates the PT phase transition.
Figure 5.Calculated absorption spectra of with different period numbers by using TMM (blue solid line) and CMT (red hexagonal points).
It is worth noting that perfect absorption peaks in Figs. 5(a)–5(d) all satisfy the condition , ( represents reflectance, subscript left stands for left incidence, and right stands for right incidence), which resembles unidirectional invisibility discovered in modulated PT-symmetric waveguides [31]. Here, unidirectional invisibility in structure is visualized in Fig. 4(b). Light incident from the left side can go through the structure without reflection at , while light incident from the right side is totally reflected. The resulted asymmetric field distributions for left and right incidences are given in the bottom panel of Fig. 4(b). The reflectance is not precisely zero because the case of deviates a little bit from exact EP (), which can be seen in Fig. 4(a).
4. LIGHT ABSORBER VIA COUPLED TISs WITH NON-IDEAL PT SYMMETRY
The number of layers involved in the aforementioned structure is too large, so it is difficult to fabricate the structure with high accuracy. For such a multilayer film prepared by electron beam evaporation, the thicker the total structure becomes, the more likely fabrication error will be introduced, which will eventually lead to the failure of the experiment. To solve the problem, we substitute the PC for a coated silver layer so that total thickness of the sample can be greatly reduced. Here, the reflection phase of coated silver layer is negative, so TIS 1 can still be achieved according to the existence condition of TIS .
But now there is another problem: loss and effective gain are not exactly balanced in the proposed new structure. Fortunately, the PT phase transition can still be observed in a system with unbalanced loss and gain [72]. So finally, we design a non-ideal PT-symmetric (also called gauged PT) structure that is possible to achieve in the experiment.
The considered non-ideal PT-symmetric structure, namely, , which support two TISs at both ends of , is shown in Fig. 6(a). The thicknesses of dielectric layers are designed to be , , , and (here, we adjust the thickness of layer a bit to further reduce total thickness). The thicknesses of silver layers adjacent to the left/right boundaries of PC are and , respectively. Also, one unit cell of acts as a coating layer to protect silver from air. Similar to the previous design, the two TISs are first investigated in the separated structures, i.e., and , as given in Figs. 6(b) and 6(c), respectively. The corresponding field enhancements are verified in Figs. 6(d) and 6(e). It must be pointed out that there is no interface state on the interface between silver and [this interface is denoted by the yellow dashed line in Fig. 6(d)], as and are topologically indistinguishable in the interested gap-frequency region. A little asymmetry for the line shape in Fig. 6(b) may result from dispersion of the thin silver layer. Nevertheless, the Lorentz model is sufficient enough for us to acquire the scattering loss and intrinsic loss of the resonance. For these new samples, using the same method in the ideal PT symmetry case, we have , (), and the other fitted parameters are: , , , , as shown in Figs. 6(b) and 6(c). In addition, the dependence of coupling rate on period number () is .
Figure 6.(a) Schematic of PC heterostructure . (b), (c) Calculated absorption spectra of (b) TIS 1 in and (c) TIS 2 in , using TMM (blue solid line) and Lorentz model (red hexagonal points). (d), (e) Corresponding distribution of normalized electric field amplitude. The yellow (red) dashed line represents the interface between silver layers and ().
Although the ideal PT symmetry condition is not satisfied for , we will show that a PT phase transition and one-channel CPA can still be demonstrated in the following. The eigenvalues calculated by CMT together with absorption peaks extracted from TMM are shown in Fig. 7(a). The system is found to be working in the vicinity of a real eigenvalue when , leading to nearly perfect absorption at . This eigenvalue can be seen as one-cannel CPA in the PT symmetry broken phase, as shown in Fig. 7(a). It should be pointed out that in Fig. 7(a), EP is reached between and with a non-zero imaginary part []. Absorption spectra calculated by TMM and CMT are also given in Fig. 7(c). Two absorption peaks (671.9, 698.5 THz) with peak values less than one (about 0.90) are observed when the system is in the unbroken phase before EP (). In the case of , only one (nearly perfect) absorption peak of 0.99 can be found at , indicating one-channel CPA. It should be pointed out that perfect absorption with broken PT symmetry is also achieved in a metasurface system [73]. With the increase in period number , absorption decreases from 0.99 to 0.80 at , while the frequency of the peak remains unchanged. Such merging in absorption peaks illustrates the PT phase transition in the non-ideal case. Particularly, the system can have a real eigenvalue at the critical coupling of (approximately ) in the PT broken phase. It means proper coupling may result in pseudo-Hermiticity of a non-ideal PT-symmetric system.
Figure 7.(a) Eigenvalue spectra of non-ideal PT symmetric system [] versus different coupling rates (period number ). Blue circles represent absorption peaks of the system with varied period numbers calculated by TMM. Green star represents the case where the Hamiltonian of the system has a real eigenvalue (one-channel CPA is achieved). (b) SEM image of one sample of . (c) Absorption spectra calculated from TMM (solid lines) and CMT (hexagonal dots). (d) Measured absorption spectra.
Finally, we fabricate the structures discussed above and conduct the experiment. The sample is evaporated on the substrate BK7 with a refractive index of 1.51 by electron beam evaporation. The Nova NanoSEM 450 scanning electron microscopy image of the case of as an example is shown in Fig. 7(b). The reflectance as well as transmittance is measured using a Perkin Elmer LAMBDA 1050 WB ultraviolet-visible-near-infrared spectrophotometer, and the absorption spectra are calculated through the relation , shown in Fig. 7(d).
As shown in Fig. 7(d), the evolution of the absorption spectrum unique to non-ideal PT symmetry is measured in experiments. First, under strong coupling, two absorption peaks (660.8, 684.9 THz) are observed in the case of (bule line). In the case of (red line), which is approximately under critical coupling, only one nearly perfect absorption peak of 0.98 appears at . It is very consistent with the simulated resonance frequency (). As the period number increases further, the measured peak absorption drops from 0.98 to 0.90 at (yellow line), while the frequency of the peak remains unchanged at . The measured absorption spectrum is reasonably consistent with the calculation in Fig. 7(c). Small deviation (less than 2%) of the resonance frequency in the case of is mainly caused by errors in refractive index discrepancies between the experimental materials and simulated values and layer thickness monitoring errors during the deposition process. Nevertheless, the PT phase transition and perfect light absorber are clearly demonstrated in experiments.
5. CONCLUSION
In conclusion, we propose an optical PT-symmetric scheme to realize a perfect light absorber based on the coupling of TISs in PCs. The PT phase transition is achieved in both ideal and non-ideal PT symmetry cases. In the ideal PT symmetry case, one-channel CPA with unidirectional invisibility at EP is numerically obtained. In the non-ideal case, one-channel CPA in the broken phase is observed experimentally. Our work demonstrates the possibility of manipulating non-Hermiticity of a PT system by tuning the coupling rate of TISs. The results facilitate the design of EP-based functional devices, such as unidirectional light absorbers, EP sensors, and nonlinear devices.
APPENDIX A: SPECIFIC METHODS TO OBTAIN MODEL PARAMETERS
The model parameters for a single TIS are obtained by fitting the reflectance spectra (calculated by TMM) with the Lorentz model in Eq. (2). In detail, we first acquire the resonance frequency , reflectance at (reflectance dip), and half-width of TIS resonance from the reflectance spectrum. These parameters together with are all real quantities. According to the standard Lorentz model in Eq. (2), we have
So we have the following equation for the model parameter:
The signs (positive and negative) in Eq. (A3) are determined by the relative values of and (). For the structure in Fig. 3(a), where , when , we have . The period number of with which is satisfied can be denoted as . If , there must be because increases as decreases. We find that when , the value of reflectance is near zero. Therefore, for , we always have . For , we have and .
For the structure in Fig. 3(b), where , when , we have . The period number of with which is satisfied can be denoted as . If , there must be because decreases as increases. We find that when , the value of reflectance is near zero. Therefore, for , we always have . For , we have and .
The Author Email: Yufei Wang (yufeiwang@semi.ac.cn), Haitao Jiang (jiang-haitao@tongji.edu.cn), Guiqiang Du (dgqql@sdu.edu.cn), Yong Sun (yongsun@tongji.edu.cn)