Researching | Progress of detection technology of nitrogen dioxide and organic nitrates

Journal of Atmospheric and Environmental Optics, Volume. 19, Issue 3, 265(2024)

Progress of detection technology of nitrogen dioxide and organic nitrates

TONG Jinzhao^1,2, LIN Chuan², HU Renzhi^2、*, XIE Pinhua^1,2,3,4, WU Tao², WANG Jiawei^1,2, and CHEN Liang^1,2

Author Affiliations

¹School of Environmental Science and Optoelectronic Technology, University of Science and Technology of China,Hefei 230026, China

²Key Laboratory of Environmental Optics and Technology, Anhui Institute of Optics and Fine Mechanics, HFIPS,Chinese Academy of Sciences, Hefei 230031, China

³Innovation Center for Excellence in Regional Atmospheric Environment, Institute of Urban Environment,Chinese Academy of Sciences, Xiamen 361000, China

⁴University of Chinese Academy of Sciences, Beijing 100049, China

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Figures&Tables (16)

References (121)

Paper Information

Figures & Tables(16)

Fig. 1. Schematic of the chemical reaction of NO₂ in the atmosphere

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Fig. 2. Schematic of the chemical reaction of ONs in the atmosphere

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Fig. 3. Schematic of the Chemiluminescence nitrogen oxide analyzer^[29]

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Fig. 4. Schematic of the Spectrophotometry NO_x system^[17]

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Fig. 5. Schematic of the DOAS system^[67]

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Fig. 6. Schematic of the LIF system^[68]

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Fig. 7. Schematic of the TDLAS system^[22]

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Fig. 8. Schematic of the CAPS system^[80]

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Fig. 9. Schematic of the CRDS system^[88]

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Fig. 10. Schematic of the IBBCEAS system^[90]

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Fig. 11. Schematics of the experimental set-ups installed around the SAPHIR chamber^[34]

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Fig. 12. Schematics of the experimental set-ups installed around the CESAM chamber^[100]

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Table 1. The technology of measurement of NO₂ and the corresponding research groups

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Table 1. The technology of measurement of NO₂ and the corresponding research groups

Technology	Research Group	Target gas	Accuracy/%	Limit of detection/10^-9	Time resolution	References
CL	Eco Physics, FRA	NO₂, NO	±7.0	0.01	3 min	[34]
	Thermo Electron, USA	NO₂, NO		0.40	1 min	[31]
	Thermo Fisher 42i, USA	NO₂, NO	±7.0	0.05	2 min	[101]
	Eco Physics, FRA	NO₂, NO	±10.0	0.01	90 s	[102]
	Thermo Fisher 42c, USA	NO₂, NO	±7.0	0.40	1 min	[101]
	Teledyne API, USA	NO₂, NO	±6.0	0.45	1 min	[29]
	Eco Physics, FRA	NO₂, NO	±7.0	0.054	1 min	[23]
	Air Quality Design, UK	NO₂, NO	±6.0	0.15	1 min	[29]
SP	Institute of Chemical Research, China	NO₂	±3.4	18.0	15 min	[40]
SP	Research Center for Eco-Environmental Sciences, China	NO₂		5.00	24 h	[37]
DOAS	Kern for schungsanlage Juelich GmbH, Germany	NO₂, NO₃	±10.0	0.08		[48]
	Korea Research Institute of Standards and Science, Korea	NO₂	±8.0	0.50		[51]
	Anhui Institute of Optics and Fine Mechanics, China	NO₂	±6.0	0.14	30 s	[55]
	Kwangju Inst Sci & Technol, Korea	NO₂	±10.0	0.61	3 min	[103]
LIF	University of California, USA	NO₂	±5.0	0.015	10 s	[10]
	Portland State University, USA	NO₂		0.45	20 s	[8]
	Pennsylvania State University, USA	NO₂	±15.0	0.28	2.5 min	[104]
	University of California, USA	NO₂		0.145	1 min	[105]
	The University of Tokyo, Japan	NO₂		0.094	1 min	[23]
	Nagoya University, Japan	NO₂	±14.0	0.14	60 s	[68]
	Portland State University, USA	NO₂		2.00	60 s	[72]
	Nagoya University, Japan	NO₂		0.03	10 s	[106]
	Universita' degli studi di L'Aquila, Italy	NO₂		0.01	60 s	[107]
	Harvard University, USA	NO₂	±10.0	0.04	60 s	[108]
	Nagoya University, Japan	NO₂		9.80	60 s	[109]
	Environmental Protection Agency, USA	NO₂		5.00	90 s	[70]
	University of California, USA	NO₂	±5.0	0.015	10 s	[10]
	Osaka Prefecture University, Japan	NO₂	±10.0	7.00	60 s	[73]
	University of California, USA	NO₂	±15	0.09	10 s	[15]
TDLAS	Concord, Ontario, Canada	NO₂		0.025	3 min	[76]
TDLAS	State University of New York, USA	NO₂	±5.0	0.03	1 min	[22]
CAPS	Unisearch Associates, Canada	NO₂	±15	0.15	5 min	[75]
	Center for Sensor Systems and Technology, USA	NO₂	±14	0.30	10 s	[80]
	Institute of Atmospheric Physics, China	NO₂		0.046	60 s	[32]
	Center for Sensor Systems and Technology, USA	NO₂	±10.0	0.06	10 s	[81]
	Peking university, China	NO₂		0.19	60 s	[1]
	University of Manchester, UK	NO₂	±4.0	0.055	1 s	[82]
CEAS	Anhui Institute of Optics and Fine Mechanics, China	NO₂		0.095	2 s	[97]
	Anhui University, China	NO₂	±4.0	5.30	360 s	[110]
	Anhui Institute of Optics and Fine Mechanics, China	NO₂	±4.0	0.044	30 s	[94]
	Anhui Institute of Optics and Fine Mechanics, China	NO₂		0.25	20 s	[93]
	University of Colorado, USA	NO₂	±5.0	0.08	5 s	[96]
	Anhui Institute of Optics and Fine Mechanics, China	NO₂	± 6.0	3.10	80 s	[111]
	Nanchang Hangkong University, China	NO₂	±5.0	2.00	120 s	[95]
	University of Manchester, UK	NO₂		0.24	80 s	[91]
	Anhui Institute of Optics and Fine Mechanics, China	NO₂	±9.0	0.34	30 s	[98]
CRDS	University of Colorado, USA	NO₂, NO	±5.0	0.022	1 s	[2]
	Anhui Institute of Optics and Fine Mechanics, China	NO₂	±4.5	0.066	1 s	[86]
	Earth System Research Laboratory, USA	NO₂	±4.0	0.04	1 s	[20]
	Adelphi University, USA	NO₂		1.20	1 s	[84]
	University of Colorado, USA	NO₂, NO	±3.0	0.03	1 s	[85]
	South China University of Technology, China	NO₂		0.15	10 s	[112]

Table 2. The technology of ONs and the corresponding research groups

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Table 2. The technology of ONs and the corresponding research groups

Method	Research Group	Target gas	Limit of detection/10^-12	Reference
GC-ECD	National Center for Atmospheric Research, USA	PANs		[14]
TD-LIF	University of California, Berkeley, USA	PNs, ANs, HNs, HNO₃	NO₂: 90	[15]
	University of California, USA	NO₂, ONs	ON: 45	[25]
	Universita' degli studi di L'Aquila, Italy	NO₂, PNs, ANs, HNO₃	NO₂: 9.8, PNs: 18.4 ANs: 28.1, HNO₃: 49.7	[7]
	University of California, Berkeley, USA	NO₂, PNs	NO₂: 70	[114]
TD-CAPS	Osaka Prefecture University, Japan	NO₂, PNs, ONs	PNs: 21 ONs: 21	[13]
TD-CIMS	National Center for Atmospheric Research, USA	PNs、N₂O₅	PAN: 7×, PPN: 4 PiBN: 3, N₂O₅: 12	[26]
TD-CEAS	Peking University, China	NO₂, PNs, ANs	NO₂: 97	[11]
TD-CRDS	Division of Atmospheric Chemistry, Germany	NO₂, PNs, ANs	NO₂: 20	[117]
	Anhui Institute of Optics and Fine Mechanics, China	NO₂, ONs	NO₂: 90	[118]
	University of Calgary, Canada	NO₂, PAN	NO₂: 20	[27]
	Max-Planck-Institut für Chemie, Germany	NO₂, NO₃, N₂O₅, PNs, ANs	NO₂: 25 PNs: 40 ANs: 45	[116]
	University of Calgary, Canada	ANs, PNs	ANs: 100, PNs: 100	[12]
	Reed College, Portland, USA	NO₂, PNs, ANs, HNO₃	NO₂: 480 PNs: 660 ANs: 660, HNO₃: 660	[119]

Table 3. The instrument comparison of measurements in chamber SAPHIR

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Table 3. The instrument comparison of measurements in chamber SAPHIR

Research Group	Method	Position	Accuracy (1σ)/%	Limit of detection/10^-12	Time Resolution	Correlation (R²)
Eco Physics, FR	PC-CLD	Underneath the chamber	±7	10	3 min
Berkeley, USA	LIF	Below the chamber	±5	100	10 s	0.99
NOAA, USA	CRDS	Underneath the chamber	±6	80	1 s	0.96
University of Leicester, UK	BBCRDS	Below the chamber	±11		1 min	0.93
University College Cork, Ireland	IBBCEAS	Inside chamber	±18	600	5 s	0.93

Table 4. The instrument comparison of measurements in chamber CESAM

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Table 4. The instrument comparison of measurements in chamber CESAM

Research Group

Method

Accuracy/%

Limit of detection

Time Resolution/s

Correlation

(R²)

Université du Littoral

Côté d'Opale, FR

IBBCEAS

±8

160 × 10^-12

120

University of York,

UK

FTIR

±10

5 × 10^-9

300

0.93

HORIBA APNA,

JPN

CL

±10

400 × 10^-12

60

0.99

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Jinzhao TONG, Chuan LIN, Renzhi HU, Pinhua XIE, Tao WU, Jiawei WANG, Liang CHEN. Progress of detection technology of nitrogen dioxide and organic nitrates[J]. Journal of Atmospheric and Environmental Optics, 2024, 19(3): 265

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Paper Information

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Received: Apr. 8, 2022

Accepted: --

Published Online: Jul. 17, 2024

The Author Email: HU Renzhi (rzhu@aiofm.ac.cn)

DOI:10.3969/j.issn.1673-6141.2024.03.001

Topics

laser devices and laser physics

Lasers and Laser Optics

laser manufacturing

Instrumentation, Measurement and Metrology