Infrared and Laser Engineering, Volume. 53, Issue 11, 20240224(2024)

Nonlinear optical properties of SnSe2 quantum dot composite gel glass

Chan ZHENG1,2、*, Di WANG1, Li HUANG1, Xueqing XIAO1, and Xingfang HUANG1
Author Affiliations
  • 1School of Materials Science and Engineering, Fujian University of Technology, Fuzhou 350118, China
  • 2Institute of Biology and Chemistry, Fujian University of Technology, Fuzhou 350118, China
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    Figures & Tables(10)
    Preparation process of SnSe2 QD composite gel glass
    (a)-(b) The TEM image of SnSe2 QDs (the inset is the electron diffraction pattern of SnSe2 quantum dots); (c) The HRTEM image of SnSe2 QDs; (d) Statistical plot of particle size of SnSe2 QDs
    ( (a) Digital photo of blank glass (left) and SnSe2 QD composite gel glass (right); (b) SEM image of the cross section of SnSe2 QD composite gel glass; (c)-(f) EDX energy spectrum of O, Si, Se and Sn elements in SnSe2 QD composite gel glass
    The Raman spectrum of SnSe2 QDs and SnSe2 QD composite gel glass
    (a)-(b) Absorption spectra of SnSe2 QDs and SnSe2 QD composite gel glass; (c)-(d) Band gap width calculation diagram of SnSe2 QDs and its composite gel glass
    (a)-(b) OA Z-scan curves of the SnSe2 QD composite gel glass under ps and ns excitation; (c)-(d) OA Z-scan curves of the blank gel glass under ps and ns excitation
    OA Z-scan curves of the SnSe2 QDs and corresponding composite gel glasses under ps and ns excitations
    (a) Two dimensional transient absorption color spectrum of the SnSe2 QD composite gel glass; (b) Transient absorption spectra curve of SnSe2 QD composite gel glass; (c) The decay kinetics curve of the probe wavelength at 532 nm; (d) The relaxation time τ1 (bottom) and τ2 (upper) at different probe wavelength of SnSe2 QD composite gel glass
    • Table 1. β, Imχ(3), FOM, and Is of SnSe2 QD composite gel glass and other reported materials

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      Table 1. β, Imχ(3), FOM, and Is of SnSe2 QD composite gel glass and other reported materials

      Input engergy/materialsβ/×10−10 m·W−1Imχ(3)/×10−12 esuFOM/×10−12 esuIs /×1011 W·m−2Reference
      4 μJ−4.4×10−3−1.24×10−26.18×10−33.2This work
      5 μJ−5.5×10−3−1.55×10−27.73×10−34.4This work
      6 μJ−8.5×10−3−2.40×10−211.9×10−38.9This work
      7 μJ−11×10−3−3.11×10−215.5×10−39.2This work
      20 μJ1.54.241.66N/AThis work
      40 μJ1.263.561.40N/AThis work
      60 μJ1.13.111.22N/AThis work
      80 μJ1.33.671.44N/AThis work
      Pd NPS−5.14×10−2N/AN/A3.59[22]
      Ag2S QDS−0.48N/AN/A0.28[23]
      MXene flake1.1×10−31.95×10−22.44×10−3N/A[24]
      Nb2C QDs1.1×10−22.76N/AN/A[25]
      graphene QDs1.70.57×10−2N/AN/A[26]
      BP QDsN/AN/AN/A0.33[27]
      CsPbBr3 QDs0.320.26N/AN/A[28]
    • Table 2. The ultrafast relaxation times of SnSe2 QD composite gel glass and the reported materials

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      Table 2. The ultrafast relaxation times of SnSe2 QD composite gel glass and the reported materials

      MaterialsWavelength/nmUltrafast relaxation timeReference
      PumpProbeτ1/psτ2/ps
      SnSe2 QDs36053213.36288.64This work
      VP nanosheets4205401.185[29]
      BP nanosheets4005209.494.2[30]
      InP/ZnS QDs4005622173[31]
      Co-TCPP(Fe) MOF4005133.5733.5[32]
      WS2 QDs4006005.3132[33]
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    Chan ZHENG, Di WANG, Li HUANG, Xueqing XIAO, Xingfang HUANG. Nonlinear optical properties of SnSe2 quantum dot composite gel glass[J]. Infrared and Laser Engineering, 2024, 53(11): 20240224

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    Paper Information

    Category: 非线性光学

    Received: Jul. 3, 2024

    Accepted: --

    Published Online: Dec. 13, 2024

    The Author Email: ZHENG Chan (czheng@fjut.edu.cn)

    DOI:10.3788/IRLA20240224

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