Journal of Applied Optics, Volume. 44, Issue 4, 726(2023)
Second-order nonlinear optical response based on codoped C32 multipole moments modulation
Figures & Tables(8)
Fig. 1. Optimized geometric structures of C32, C28B2N2 and C28B2P2 series
Fig. 2. Frontier molecular orbital energy distribution of C32 and different isomers
Fig. 4. Research results of second-order NLO properties of different isomers
Fig. 5. Functional relationship between harmonic light intensity and polarization angle Ψ
Fig. 6. Comparison of UV-Vis absorption spectra of C32, NB-1 and PB-1
Fig. 7. Molecular orbitals and main transition forms of PB-1 and NB-1
Table 1. Crucial excited states, excitation energies ΔE, transition dipole moment Δμ, transition dipole moment between two excited states Δμij, oscillator strength f and the first hyperpolarizability βSOS under two-level/three-level model of PB-1 and NB-1
View tableView in ArticleTable 1. Crucial excited states, excitation energies ΔE, transition dipole moment Δμ, transition dipole moment between two excited states Δμij, oscillator strength f and the first hyperpolarizability βSOS under two-level/three-level model of PB-1 and NB-1
关键态 ΔE/eV Δμ/×10−30 C·m f Δμij/ ×10−30 C·m βSOS/ ×10−51 C3·m3·J−2 PB-1 3 1.53 4.83 0.016 0.47 30.813 30 4.13 8.19 0.177 NB-1 2 1.45 9.40 0.016 - 23.660
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Ruirui TIAN, Peiyu YANG, Bojin HU, Yiyang LI, Can XU. Second-order nonlinear optical response based on codoped C32 multipole moments modulation[J]. Journal of Applied Optics, 2023, 44(4): 726
Paper Information
Category: Research Articles
Received: Sep. 23, 2022
Accepted: --
Published Online: Aug. 10, 2023
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