Journal of the European Optical Society-Rapid Publications, Volume. 19, Issue 1, 2023008(2023)

Novel time-resolved CARS implementation for application in microscopy

Pieter H. Neethling1,*... Ruan Viljoen1, Alexander M. Heidt2, Dirk Spangenberg1,2, Thomas Feurer2 and Erich G. Rohwer1 |Show fewer author(s)
Author Affiliations
  • 1Laser Research Institute, Stellenbosch University, 7600 Stellenbosch, South Africa
  • 2Institute for Applied Physics, University of Bern, 3012 Bern, Switzerland
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    References(13)

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    [3] M.K. Petti, J.P. Lomont, M. Maj, M.T. Zanni. Two-dimensional spectroscopy is being used to address core scientific questions in biology and materials science. J. Phys. Chem. B, 122, 1771(2018).

    [4] A. Ghosh, J.S. Ostrander, M.T. Zanni. Watching proteins wiggle: Mapping structures with two-dimensional infrared spectroscopy. Chem. Rev., 117, 10726(2017).

    [5] P.V. Kolesnichenko, J.O. Tollerud, J.A. Davis. Background-free time-resolved coherent Raman spectroscopy (CSRS and CARS): Heterodyne detection of low-energy vibrations and identification of excited-state contributions. APL Photon., 4, 56102(2019).

    [6] H.U. Stauffer, J.D. Miller, M.N. Slipchenko. Time-and frequency-dependent model of time-resolved Coherent Anti-Stokes Raman scattering (CARS) with a picosecond-duration probe pulse. J. Chem. Phys., 140, 24316(2014).

    [7] A.M. Heidt, J. Rothhardt, A. Hartung, H. Bartelt, E.G. Rohwer, J. Limpert, A. Tünnermann. High quality sub-two cycle pulses from compression of supercontinuum generated in all-normal dispersion photonic crystal fiber. Opt. Exp., 19, 3775(2011).

    [8] D.M. Spangenberg, E. Rohwer, M. Brügmann, T. Feurer. Extending time-domain ptychography to generalized phase-only transfer functions. Opt. Lett., 45, 300-303(2020).

    [9] R. Viljoen, P. Neethling, D. Spangenberg, A. Heidt, H.M. Frey, T. Feurer, E. Rohwer. Implementation of temporal ptychography algorithm, i2PIE, for improved single-beam coherent anti-Stokes Raman scattering measurements. JOSA B, 37, A259-A265(2020).

    [10] A. Rampur, D.M. Spangenberg, B. Sierro, P. Hänzi, M. Klimczak, A.M. Heidt. Perspective on the next generation of ultra-low noise fiber supercontinuum sources and their emerging applications in spectroscopy, imaging, and ultrafast photonics. Appl. Phys. Lett., 118, 240504(2021).

    [11] M. Motzkus, L. Brückner, T. Buckup. Enhancement of coherent anti-Stokes Raman signal via tailored probing in spectral focusing. Opt. Lett., 40, 5204-5207(2015).

    [12] J.W. Perry, A.M. Woodward, J.C. Stephenson. Picosecond Coherent Anti-Stokes Raman Scattering (CARS) study of vibrational dephasing of carbon disulfide and benzene in solution. Laser Appl. Chem. Biophys., 620, 7(1986).

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    Pieter H. Neethling, Ruan Viljoen, Alexander M. Heidt, Dirk Spangenberg, Thomas Feurer, Erich G. Rohwer. Novel time-resolved CARS implementation for application in microscopy[J]. Journal of the European Optical Society-Rapid Publications, 2023, 19(1): 2023008

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    Paper Information

    Category: Research Articles

    Received: Dec. 12, 2022

    Accepted: Feb. 27, 2023

    Published Online: Aug. 31, 2023

    The Author Email: Neethling Pieter H. (pietern@sun.ac.za)

    DOI:10.1051/jeos/2023008

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