Acta Optica Sinica, Volume. 36, Issue 2, 216001(2016)
Effect of Size Distribution of Quantum Dots with Low Doping Concentration on Photoluminescence Emission Spectrum
A general expression of the photoluminescence (PL)-spectral shape depending on the size distribution of quantum dots (QDs) in the condition of low doping concentration is presented, using the effective mass approximation and supposing a Gaussian distribution of QD sizes. Effect of the size fluctuation on the PL-broadened line is discussed. As an example, the PL-broadened lines of both IV-VI CdSe QDs and II-VI PbSe QDs are calculated. There is evidence to show that the calculated PL intensity, PL-peak wavelength and full width at half maximum of the PL-broadened line are in consistent with the experimental measurements. The size distribution of QDs has primary effect on the PL-broadened line. The PL-broadened line is an inhomogeneous broadening.
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Cheng Cheng, Li Zhiwei. Effect of Size Distribution of Quantum Dots with Low Doping Concentration on Photoluminescence Emission Spectrum[J]. Acta Optica Sinica, 2016, 36(2): 216001
Category: Materials
Received: Aug. 3, 2015
Accepted: --
Published Online: Jan. 25, 2016
The Author Email: Cheng Cheng (chengch@zjut.edu.cn)