Optics and Precision Engineering, Volume. 32, Issue 3, 317(2024)

Light intensity correction for light-induced thermoelastic spectroscopy based on nonlinear response of light intensity

Xiang CHEN1... Hao LIU1,2, Lu YAO1, Zhenyu XU1, Mai HU3,* and Ruifeng KAN1,* |Show fewer author(s)
Author Affiliations
  • 1Hefei Institute of Physical Science, Chinese Academy of Sciences, Hefei23003, China
  • 2University of Science and Technology of China, Hefei3006, China
  • 3The Chinese University of Hong Kong, Hong Kong999077, China
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    This study presents a method for correcting light intensity in light⁃induced thermoelastic spectroscopy (LITES) using a nonlinear light intensity response, enabling precise light intensity corrections. The DFB laser, set to a wavelength modulation mode at a frequency of 16369.75 Hz, benefits from enhanced nonlinear light intensity due to a fiber amplifier. The laser beam traverses a multi⁃pass cell before focusing on the quartz tuning fork (QTF) base, generating a thermoelastic signal. A lock⁃in amplifier demodulates the harmonic signal, and polynomial fitting of the harmonic signal's baseline extracts harmonics related to both concentration and light intensity. Experimental data reveal a strong linear correlation (coefficient > 0.998) between the baseline amplitude of the harmonic signal and light intensity as it varies from 22.03 mW to 3.16 mW, with normalized harmonic signal amplitude variation under 0.37%. In methane detection, the system demonstrates a robust linear response across a broad concentration range, with harmonic signal noise ratios indicating a detection threshold as low as 0.22×10-6. This research offers a novel approach for LITES light intensity correction, significantly enhancing system stability for prolonged measurements.

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    Xiang CHEN, Hao LIU, Lu YAO, Zhenyu XU, Mai HU, Ruifeng KAN. Light intensity correction for light-induced thermoelastic spectroscopy based on nonlinear response of light intensity[J]. Optics and Precision Engineering, 2024, 32(3): 317

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    Paper Information

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    Received: Oct. 17, 2023

    Accepted: --

    Published Online: Apr. 2, 2024

    The Author Email: HU Mai (maihu@cuhk.edu.hk), KAN Ruifeng (kanruifeng@aiofm.ac.cn)

    DOI:10.37188/OPE.20243203.0317

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