Ultrafast Science, Volume. 3, Issue 1, 0004(2023)

Realizing Attosecond Core-Level X-ray Spectroscopy for the Investigation of Condensed Matter Systems

Adam M. Summers1,2、†, Stefano Severino1、†, Maurizio Reduzzi1, Themistoklis P. H. Sidiropoulos1, Daniel E. Rivas1,3, Nicola Di Palo1, Hung-Wei Sun1, Ying-Hao Chien1, Iker León1, Bárbara Buades1, Seth L. Cousin1, Stephan M. Teichmann1, Tobias Mey4, Klaus Mann4, Barbara Keitel5, Elke Plönjes5, Dmitri K. Efetov1, Heinrich Schwoerer6, and Jens Biegert1,7、*
Author Affiliations
  • 1ICFO - Institut de Ciencies Fotoniques, The Barcelona Institute of Science and Technology, 08860 Castelldefels, Barcelona, Spain.
  • 2Linac Coherent Light Source, SLAC National Accelerator Laboratory, Menlo Park, CA 94025, USA.
  • 3European XFEL, Holzkoppel 4, 22869 Schenefeld, Germany.
  • 4Institut für Nanophotonik Göttingen e.V., Hans-Adolf-Krebs-Weg 1, 37077 Göttingen, Germany.
  • 5Deutsches Elektronen-Synchrotron, Notkestraße 85, 22607 Hamburg, Germany.
  • 6Max-Planck-Institut für Struktur und Dynamik der Materie, 22761 Hamburg, Germany.
  • 7ICREA, Pg. Lluís Companys 23, 08010 Barcelona, Spain.
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    Unraveling the exact nature of nonequilibrium and correlated interactions is paramount for continued progress in many areas of condensed matter science. Such insight is a prerequisite to develop an engineered approach for smart materials with targeted properties designed to address standing needs such as efficient light harvesting, energy storage, or information processing. For this goal, it is critical to unravel the dynamics of the energy conversion processes between carriers in the earliest time scales of the excitation dynamics. We discuss the implementation and benefits of attosecond soft x-ray core-level spectroscopy up to photon energies of 600 eV for measurements in solid-state systems. In particular, we examine how the pairing between coherent spectral coverage and temporal resolution provides a powerful new insight into the quantum dynamic interactions that determine the macroscopic electronic and optical response. We highlight the different building blocks of the methodology and point out the important aspects for its application from condensed matter studies to materials as thin as 25 nm. Furthermore, we discuss the technological developments in the field of tabletop attosecond soft x-ray sources with time-resolved measurements at the near and extended edge simultaneously and investigate the exciting prospective of extending such technique to the study of 2-dimensional materials.

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    Adam M. Summers, Stefano Severino, Maurizio Reduzzi, Themistoklis P. H. Sidiropoulos, Daniel E. Rivas, Nicola Di Palo, Hung-Wei Sun, Ying-Hao Chien, Iker León, Bárbara Buades, Seth L. Cousin, Stephan M. Teichmann, Tobias Mey, Klaus Mann, Barbara Keitel, Elke Plönjes, Dmitri K. Efetov, Heinrich Schwoerer, Jens Biegert. Realizing Attosecond Core-Level X-ray Spectroscopy for the Investigation of Condensed Matter Systems[J]. Ultrafast Science, 2023, 3(1): 0004

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    Paper Information

    Category: Research Articles

    Received: Aug. 14, 2022

    Accepted: Nov. 3, 2022

    Published Online: Dec. 4, 2023

    The Author Email: Biegert Jens (jens.biegert@icfo.eu)

    DOI:10.34133/ultrafastscience.0004

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